5,339 research outputs found
Tilting light's polarization plane to spatially separate the ultrafast nonlinear response of chiral molecules
Distinguishing between the left- and right-handed versions of a chiral molecule (enantiomers) is vital, but also inherently difficult. Traditional optical methods using elliptically/circularly polarized light rely on linear effects which arise beyond the electric-dipole approximation, posing major limitations for ultrafast spectroscopy. Here we show how to turn an ultrashort elliptical pulse into an efficient chiro-optical tool: by tilting its polarization plane towards its propagation direction. This forward tilt can be achieved by focusing the beam tightly, creating structured light which exhibits a nontrivial polarization pattern in space. Using state-of-the-art computational modelling, we show that our structured field realizes a near-field interferometer for efficient chiral recognition that separates the nonlinear optical response of left- and right-handed molecules in space. Our work provides a simple, yet highly efficient, way of spatially structuring the polarization of light to image molecular chirality, with extreme enantio-efficiency and on ultrafast time scales
Effect oF Ligand's Nature on Chemical Deposition by Sodium Sulphate of Sodium thin CdSe Films
The work was financially supported by program 211 of the Government of the Russian Federation (No. 02.A03.21.0006.
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Multipolar second-harmonic generation from high-Q quasi-BIC states in subwavelength resonators
We put forward the multipolar model which captures the physics behind linear and nonlinear response driven by high-quality (high-Q) supercavity modes in subwavelength particles. We show that the formation of such trapped states associated with bound states in the continuum (quasi-BIC) can be understood through multipolar transformations of coupled leaky modes. The quasi-BIC state appears with increasing the order of the dominating multipole, where dipolar losses are completely suppressed. The efficient optical coupling to this state in the AlGaAs nanodisk is implemented via azimuthally polarized beam illumination matching its multipolar origin. We establish a one-to-one correspondence between the standard phenomenological non-Hermitian coupled-mode theory and multipolar models. The derived multipolar composition of the generated second-harmonic radiation from the AlGaAs nanodisk is then validated with full-wave numerical simulations. Back-action of the second-harmonic radiation onto the fundamental frequency is taken into account in the coupled nonlinear model with pump depletion. A hybrid metal-dielectric nanoantenna is proposed to augment the conversion efficiency up to tens of per cent due to increasing quality factors of the involved resonant states. Our findings delineate novel promising strategies in the design of functional elements for nonlinear nanophotonics applications
High-order harmonic generation in Xe, Kr, and Ar driven by a 2.1-\mu m source: high-order harmonic spectroscopy under macroscopic effects
We experimentally and numerically study the atomic response and pulse
propagation effects of high-order harmonics generated in Xe, Kr, and Ar driven
by a 2.1-\mu m infrared femtosecond light source. The light source is an
optical parametric chirped-pulse amplifier, and a modified strong-field
approximation and 3-dimensional pulse propagation code are used for the
numerical simulations. The extended cutoff in the long-wavelength driven
high-harmonic generation has revealed the spectral shaping of high-order
harmonics due to the atomic structure (or photo-recombination cross-section)
and the macroscopic effects, which are the main factors of determining the
conversion efficiency besides the driving wavelength. Using precise numerical
simulations to determine the macroscopic electron wavepacket, we are able to
extract the photo-recombination cross-sections from experimental high-order
harmonic spectra in the presence of macroscopic effects. We have experimentally
observed that the macroscopic effects shift the observed Cooper minimum of Kr
from 80 eV to 60-70 eV and wash out the Cooper minimum of Ar. Measured
high-harmonic conversion efficiencies per harmonic near the cutoff are ~10^{-9}
for all three gases.Comment: 19 pages, 8 figure
Novel spin-liquid states in the frustrated Heisenberg antiferromagnet on the honeycomb lattice
Recent experiment on a honeycomb-lattice Heisenberg antiferromagnet (AF)
BiMnO(NO) revealed a novel spin-liquid-like behavior down to
low temperature, which was ascribed to the frustration effect due to the
competition between the AF nearest- and next-nearest-neighbor interactions
and . Motivated by the experiment, we study the ordering of the
- frustrated classical Heisenberg AF on a honeycomb lattice both by
a low-temperature expansion and a Monte Carlo simulation. The model has been
known to possess a massive degeneracy of the ground state, which, however,
might be lifted due to thermal fluctuations leading to a unique ordered state,
the effect known as 'order-by-disorder'. We find that the model exhibits an
intriguing ordering behavior, particularly near the AF phase boundary. The
energy scale of the order-by-disorder is suppressed there down to extremely low
temperatures, giving rise to exotic spin-liquid states like a "ring-liquid" or
a "pancake-liquid" state accompanied by the characteristic spin structure
factor and the field-induced antiferromagnetism. We argue that the recent
experimental data are explicable if the system is in such exotic spin-liquid
states
АНАЛІЗ МОДЕЛЕЙ МЕДИЧНОГО СТРАХУВАННЯ
Purpose: to analyze the main models of health insurance in different countries.
Materials and Methods. Methods of theoretical generalization, grouping are used; factor analysis; statistical comparison and generalization.
Results. Types of health insurance models are identified; their similar and different qualities are analyzed. The basic principles of combining budget and insurance funds for the provision of health services to the population are considered on the example of countries that are already making good progress in this area.
Conclusions. There are three main types of medical financing: public (budget), in which the state’s share exceeds 70 % of total funding, social funding (from national social insurance funds that do not come to the budget) and private health insurance. Each country typically uses all three types of funding, combining them in different proportions.Мета: проаналізувати основні моделі медичного страхування у різних країнах світу.
Матеріали і методи. Використано методи теоретичного узагальнення, групування; факторного аналізу; статистичного порівняння та узагальнення.
Результати. Визначено види моделей медичного страхування; проаналізовано їх подібні та відмінні якості; розглянуто основні засади поєднання бюджетних та страхових коштів для надання населенню послуг у галузі охорони здоров’я на прикладі країн, які вже мають у цій сфері належні успіхи.
Висновки. Є три основні види фінансування медицини: державне (бюджетне), за якого частка держави перевищує 70 % загального фінансування, соціальне фінансування (за рахунок загальнодержавних фондів соціального страхування, які не надходять до бюджету) та приватне медичне страхування. Кожна країна, як правило, використовує всі три види фінансування, комбінуючи їх у різних пропорціях
Interpreting Attoclock Measurements of Tunnelling Times
Resolving in time the dynamics of light absorption by atoms and molecules,
and the electronic rearrangement this induces, is among the most challenging
goals of attosecond spectroscopy. The attoclock is an elegant approach to this
problem, which encodes ionization times in the strong-field regime. However,
the accurate reconstruction of these times from experimental data presents a
formidable theoretical challenge. Here, we solve this problem by combining
analytical theory with ab-initio numerical simulations. We apply our theory to
numerical attoclock experiments on the hydrogen atom to extract ionization time
delays and analyse their nature. Strong field ionization is often viewed as
optical tunnelling through the barrier created by the field and the core
potential. We show that, in the hydrogen atom, optical tunnelling is
instantaneous. By calibrating the attoclock using the hydrogen atom, our method
opens the way to identify possible delays associated with multielectron
dynamics during strong-field ionization.Comment: 33 pages, 10 figures, 3 appendixe
HEP Applications Evaluation of the EDG Testbed and Middleware
Workpackage 8 of the European Datagrid project was formed in January 2001
with representatives from the four LHC experiments, and with experiment
independent people from five of the six main EDG partners. In September 2002
WP8 was strengthened by the addition of effort from BaBar and D0. The original
mandate of WP8 was, following the definition of short- and long-term
requirements, to port experiment software to the EDG middleware and testbed
environment. A major additional activity has been testing the basic
functionality and performance of this environment. This paper reviews
experiences and evaluations in the areas of job submission, data management,
mass storage handling, information systems and monitoring. It also comments on
the problems of remote debugging, the portability of code, and scaling problems
with increasing numbers of jobs, sites and nodes. Reference is made to the
pioneeering work of Atlas and CMS in integrating the use of the EDG Testbed
into their data challenges. A forward look is made to essential software
developments within EDG and to the necessary cooperation between EDG and LCG
for the LCG prototype due in mid 2003.Comment: Talk from the 2003 Computing in High Energy and Nuclear Physics
Conference (CHEP03), La Jolla, CA, USA, March 2003, 7 pages. PSN THCT00
Quantum corrections for pion correlations involving resonance decays
A method is presented to include quantum corrections into the calculation of
two-pion correlations for the case where particles originate from resonance
decays. The technique uses classical information regarding the space-time
points at which resonances are created. By evaluating a simple thermal model,
the method is compared to semiclassical techniques that assume exponential
decaying resonances moving along classical trajectories. Significant
improvements are noted when the resonance widths are broad as compared to the
temperature.Comment: 9 pages, 4 figure
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