218 research outputs found
The effect of Auger heating on intraband carrier relaxation in semiconductor quantumrods
The rate at which excited charge carriers relax to their equilibrium state
affects many aspects of the performance of nanoscale devices, including
switching speed, carrier mobility and luminescent efficiency. Better
understanding of the processes that govern carrier relaxation therefore has
important technological implications. A significant increase in carrier-carrier
interactions caused by strong spatial confinement of electronic excitations in
semiconductor nanostructures leads to a considerable enhancement of Auger
effects, which can further result in unusual, Auger-process-controlled
recombination and energy-relaxation regimes. Here, we report the first
experimental observation of efficient Auger heating in CdSe quantum rods at
high pump intensities, leading to a strong reduction of carrier cooling rates.
In this regime, the carrier temperature is determined by the balance between
energy outflow through phonon emission and energy inflow because of Auger
heating. This equilibrium results in peculiar carrier cooling dynamics that
closely correlate with recombination dynamics, an effect never before seen in
bulk or nanoscale semiconductors.Comment: 7 pages, 4 figure
Unitary and Non-Unitary Matrices as a Source of Different Bases of Operators Acting on Hilbert Spaces
Columns of d^2 x N matrices are shown to create different sets of N operators
acting on -dimensional Hilbert space. This construction corresponds to a
formalism of the star-product of operator symbols. The known bases are shown to
be partial cases of generic formulas derived by using d^2 x N matrices as a
source for constructing arbitrary bases. The known examples of the SIC-POVM,
MUBs, and the phase-space description of qubit states are considered from the
viewpoint of the developed unified approach. Star-product schemes are
classified with respect to associated d^2 x N matrices. In particular, unitary
matrices correspond to self-dual schemes. Such self-dual star-product schemes
are shown to be determined by dequantizers which do not form POVM.Comment: 12 pages, 1 figure, 1 table, to appear in Journal of Russian Laser
Researc
Erratum to: Concentric Multiple Rings by Droplet Epitaxy: Fabrication and Study of the Morphological Anisotropy
We present the Molecular Beam Epitaxy fabrication of complex GaAs/AlGaAs nanostructures by Droplet Epitaxy, characterized by the presence of concentric multiple rings. We propose an innovative experimental procedure that allows the fabrication of individual portions of the structure, controlling their diameter by only changing the substrate temperature. The obtained nanocrystals show a significant anisotropy between [110] and [1–10] crystallographic directions, which can be ascribed to different activation energies for the Ga atoms migration processes
A single-photon transistor using nano-scale surface plasmons
It is well known that light quanta (photons) can interact with each other in
nonlinear media, much like massive particles do, but in practice these
interactions are usually very weak. Here we describe a novel approach to
realize strong nonlinear interactions at the single-photon level. Our method
makes use of recently demonstrated efficient coupling between individual
optical emitters and tightly confined, propagating surface plasmon excitations
on conducting nanowires. We show that this system can act as a nonlinear
two-photon switch for incident photons propagating along the nanowire, which
can be coherently controlled using quantum optical techniques. As a novel
application, we discuss how the interaction can be tailored to create a
single-photon transistor, where the presence or absence of a single incident
photon in a ``gate'' field is sufficient to completely control the propagation
of subsequent ``signal'' photons.Comment: 20 pages, 4 figure
Постать Тараса Шевченка в рецепції Ліни Костенко
У статті розглядається поетика творення Ліною Костенко образу Кобзаря крізь призму власного "я", через пережиті відчуття поета-шістдесятника, що своєю проекцією нагадують душевні терзання великого поета.В статье рассмотрена поэтика создания Линой Костенко образа Тараса Шевченко сквозь призму собственного "я", через пережитые ощущения поэта-шестидесятника, своей проекцией напоминающие душевные терзания великого поэта.The article deals with the problem of the poetics creation by Lina Kostenko Taras Shevchenko’ image through a prism her own mind, through sensations of the poet-sixtier, by the projection reminding sincere torments the great poet is considered
Continuous-wave biexciton lasing at room temperature using solution-processed quantum wells
Solution-processed inorganic and organic materials have been pursued for more than a decade as low-threshold, high-gain lasing media, motivated in large part by their tunable optoelectronic properties and ease of synthesis and processing. Although both have demonstrated stimulated emission and lasing, they have not yet approached the continuous-wave pumping regime. Two-dimensional CdSe colloidal nanosheets combine the advantage of solution synthesis with the optoelectronic properties of epitaxial two-dimensional quantum wells. Here, we show that these colloidal quantum wells possess large exciton and biexciton binding energies of 132 meV and 30 meV, respectively, giving rise to stimulated emission from biexcitons at room temperature. Under femtosecond pulsed excitation, close-packed thin films yield an ultralow stimulated emission threshold of 6 μJ cm(-2), sufficient to achieve continuous-wave pumped stimulated emission, and lasing when these layers are embedded in surface-emitting microcavities
Investigation on Photovoltaic Performance based on Matchstick-Like Cu2S–In2S3Heterostructure Nanocrystals and Polymer
In this paper, we synthesized a novel type II cuprous sulfide (Cu2S)–indium sulfide (In2S3) heterostructure nanocrystals with matchstick-like morphology in pure dodecanethiol. The photovoltaic properties of the heterostructure nanocrystals were investigated based on the blends of the nanocrystals and poly(2-methoxy-5-(2′-ethylhexoxy)-p-phenylenevinylene) (MEH-PPV). In comparison with the photovoltaic properties of the blends of Cu2S or In2S3nanocrystals alone and MEH-PPV, the power conversion efficiency of the hybrid device based on blend of Cu2S–In2S3and MEH-PPV is enhanced by ~3–5 times. This improvement is consistent with the improved exciton dissociation or separation and better charge transport abilities in type II heterostructure nanocrystals
One-Step Synthesis of Monodisperse In-Doped ZnO Nanocrystals
A method for the synthesis of high quality indium-doped zinc oxide (In-doped ZnO) nanocrystals was developed using a one-step ester elimination reaction based on alcoholysis of metal carboxylate salts. The resulting nearly monodisperse nanocrystals are well-crystallized with typically crystal structure identical to that of wurtzite type of ZnO. Structural, optical, and elemental analyses on the products indicate the incorporation of indium into the host ZnO lattices. The individual nanocrystals with cubic structures were observed in the 5% In–ZnO reaction, due to the relatively high reactivity of indium precursors. Our study would provide further insights for the growth of doped oxide nanocrystals, and deepen the understanding of doping process in colloidal nanocrystal syntheses
Effects of the Template Composition and Coating on the Photoluminescence Properties of ZnS:Mn Nanoparticles
Mn-doped ZnS nanocrystals based on low dopant concentrations (0–2%) and coated with a shell of Zn(OH)2 have been prepared via soft template and precipitation reaction. The results indicate that the ZnS:Mn nanocrystal is cubic zinc blende structure and its diameter is 3.02 nm as demonstrated by XRD. Measured by TEM, the morphology of nanocrystals is a spherical shape, and their particle size (3–5 nm) is similar to that of XRD results. Photoluminescence spectra under ultraviolet region shows that the volume ratio of alcohol to water in the template has a great effect on the luminescence properties of ZnS:Mn particles. Compared with unpassivated ZnS:Mn nanocrystals, ZnS:Mn/Zn(OH)2 core/shell nanocrystal exhibits much improved luminescence and higher absolute quantum efficiency. Meanwhile, we simply explore the formation mechanism of ZnS:Mn nanocrystals in alcohol and water system and analyze the reason why alcohol and water cluster structures can affect the luminescent properties of nanoparticle
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