250 research outputs found
Magnetic versus nonmagnetic doping effects on the magnetic ordering in the Haldane chain compound PbNi2V2O8
A study of an impurity driven phase-transition into a magnetically ordered
state in the spin-liquid Haldane chain compound PbNi2V2O8 is presented. Both,
macroscopic magnetization as well as 51V nuclear magnetic resonance (NMR)
measurements reveal that the spin nature of dopants has a crucial role in
determining the stability of the induced long-range magnetic order. In the case
of nonmagnetic (Mg2+) doping on Ni2+ spin sites (S=1) a metamagnetic transition
is observed in relatively low magnetic fields. On the other hand, the magnetic
order in magnetically (Co2+) doped compounds survives at much higher magnetic
fields and temperatures, which is attributed to a significant anisotropic
impurity-host magnetic interaction. The NMR measurements confirm the predicted
staggered nature of impurity-liberated spin degrees of freedom, which are
responsible for the magnetic ordering. In addition, differences in the
broadening of the NMR spectra and the increase of nuclear spin-lattice
relaxation in doped samples, indicate a diverse nature of electron spin
correlations in magnetically and nonmagnetically doped samples, which begin
developing at rather high temperatures with respect to the antiferromagnetic
phase transition.Comment: 10 pages, 7 figure
Optical investigation of the metal-insulator transition in
We present a comprehensive optical study of the narrow gap
semiconductor. From the optical reflectivity, measured from the far infrared up
to the ultraviolet spectral range, we extract the complete absorption spectrum,
represented by the real part of the complex optical
conductivity. With decreasing temperature below 80 K, we find a progressive
depletion of below cm, the
semiconducting optical gap. The suppressed (Drude) spectral weight within the
gap is transferred at energies and also partially piles up over a
continuum of excitations extending in the spectral range between zero and
. Moreover, the interaction of one phonon mode with this continuum leads
to an asymmetric phonon shape. Even though several analogies between
and were claimed and a Kondo-insulator scenario was also invoked for
both systems, our data on differ in several aspects from those of
. The relevance of our findings with respect to the Kondo insulator
description will be addressed.Comment: 17 pages, 5 figure
Elastic properties of FeSi
Measurements of the sound velocities in a single crystal of FeSi were
performed in the temperature range 4-300 K. Elastic constants and
deviate from a quasiharmonic behavior at high temperature; whereas,
increases anomalously in the entire range of temperature, indicating a
change in the electron structure of this materia
Enhancement of the Josephson current by magnetic field in superconducting tunnel structures with paramagnetic spacer
The dc Josephson critical current of a (S/M)IS tunnel structure in a parallel
magnetic field has been investigated (here S is a superconductor, S/M is the
proximity coupled S and paramagnet M bilayer and I is an insulating barrier).
We consider the case when, due to the Hund's rule, in the M metal the effective
molecular interaction aligns spins of the conducting electrons antiparallel to
localized spins of magnetic ions. It is predicted that for tunnel structures
under consideration there are the conditions when the destructive action of the
internal and the applied magnetic fields on Cooper pairs is weakened and the
increase of the applied magnetic field causes the field-induced enhancement of
the tunnel critical current. The experimental realization of this interesting
effect of the interplay between superconductivity and magnetism is also
discussed.Comment: 5 pages 3 figure
NMR and dc-susceptibility studies of NaVGe2O6
We report the results of measurements of the dc magnetic susceptibility
chi(T) and of the 23Na nuclear magnetic resonance (NMR) response of NaVGe2O6, a
material in which the V ions form a network of interacting one-dimensional spin
S=1 chains. The experiments were made at temperatures between 2.5 and 300 K.
The chi(T) data suggest that the formation of the expected low-temperature
Haldane phase is intercepted by an antiferromagnetic phase transition at 18 K.
The transition is also reflected in the 23Na NMR spectra and the corresponding
spin-lattice relaxation rate 1/T1(T). In the ordered phase, 1/T1(T) decreases
by orders of magnitude with decreasing temperature, indicating the formation of
a gap of the order of 12 K in the magnetic excitation spectrum.Comment: 10 pages, 15 figures; v2 with minor revisions of the tex
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