Cosmogenic radionuclide production in NaI(Tl) crystals

arXiv:1411.0106v2.-- et al.The production of long-lived radioactive isotopes in materials due to the exposure to cosmic rays on Earth surface can be an hazard for experiments demanding ultra-low background conditions, typically performed deep underground. Production rates of cosmogenic isotopes in all the materials present in the experimental set-up, as well as the corresponding cosmic rays exposure history, must be both well known in order to assess the relevance of this effect in the achievable sensitivity of a given experiment. Although NaI(Tl) scintillators are being used in experiments aiming at the direct detection of dark matter since the first nineties of the last century, very few data about cosmogenic isotopes production rates have been published up to date. In this work we present data from two 12.5 kg NaI(Tl) detectors, developed in the frame of the ANAIS project, which were installed inside a convenient shielding at the Canfranc Underground Laboratory just after finishing surface exposure to cosmic rays. The very fast start of data taking allowed to identify and quantify isotopes with half-lives of the order of tens of days. Initial activities underground have been measured and then production rates at sea level have been estimated following the history of detectors; values of about a few tens of nuclei per kg and day for Te isotopes and 22Na and of a few hundreds for I isotopes have been found. These are the first direct estimates of production rates of cosmogenic nuclides in NaI crystals. A comparison of the so deduced rates with calculations using typical cosmic neutron flux at sea level and a carefully selected description of excitation functions will be also presented together with an estimate of the corresponding contribution to the background at low and high energies, which can be relevant for experiments aiming at rare events searches.This work has been supported by the Spanish Ministerio de Economía y Competitividad and the European Regional Development Fund (MINECO-FEDER) (FPA2011-23749), the Consolider-Ingenio 2010 Programme under grants MULTIDARK CSD2009-00064 and CPAN CSD2007-00042, and the Gobierno de Aragón (Group in Nuclear and Astroparticle Physics, ARAID Foundation and C. Cuesta predoctoral grant). C. Ginestra and P. Villar are supported by the MINECO Subprograma de Formación de Personal Investigador.Peer Reviewe

Measurement of the quenching factor of Na recoils in NaI(Tl)

Measurements of the quenching factor for sodium recoils in a 5 cm diameter NaI(Tl) crystal at room temperature have been made at a dedicated neutron facility at the University of Sheffield. The crystal has been exposed to 2.45 MeV mono-energetic neutrons generated by a Sodern GENIE 16 neutron generator, yielding nuclear recoils of energies between 10 and 100 keVnr. A cylindrical BC501A detector has been used to tag neutrons that scatter off sodium nuclei in the crystal. Cuts on pulse shape and time of flight have been performed on pulses recorded by an Acqiris DC265 digitiser with a 2 ns sampling time. Measured quenching factors of Na nuclei range from 19% to 26% in good agreement with other experiments, and a value of 25.2 \pm 6.4% has been determined for 10 keV sodium recoils. From pulse shape analysis, the mean times of pulses from electron and nuclear recoils have been compared down to 2 keVee. The experimental results are compared to those predicted by Lindhard theory, simulated by the SRIM Monte Carlo code, and a preliminary curve calculated by Prof. Akira Hitachi.Comment: 21 pages, 13 figure

Light yield determination in large sodium iodide detectors applied in the search for dark matter

Application of NaI(Tl) detectors in the search for galactic dark matter particles through their elastic scattering off the target nuclei is well motivated because of the long standing DAMA/LIBRA highly significant positive result on annual modulation, still requiring confirmation. For such a goal, it is mandatory to reach very low threshold in energy (at or below the keV level), very low radioactive background (at a few counts/keV/kg/day), and high detection mass (at or above the 100 kg scale). One of the most relevant technical issues is the optimization of the crystal intrinsic scintillation light yield and the efficiency of the light collecting system for large mass crystals. In the frame of the ANAIS (Annual modulation with NaI Scintillators) dark matter search project large NaI(Tl) crystals from different providers coupled to two photomultiplier tubes (PMTs) have been tested at the Canfranc Underground Laboratory. In this paper we present the estimates of the NaI(Tl) scintillation light collected using full-absorption peaks at very low energy from external and internal sources emitting gammas/electrons, and single-photoelectron events populations selected by using very low energy pulses tails. Outstanding scintillation light collection at the level of 15~photoelectrons/keV can be reported for the final design and provider chosen for ANAIS detectors. Taking into account the Quantum Efficiency of the PMT units used, the intrinsic scintillation light yield in these NaI(Tl) crystals is above 40~photoelectrons/keV for energy depositions in the range from 3 up to 25~keV. This very high light output of ANAIS crystals allows triggering below 1~keV, which is very important in order to increase the sensitivity in the direct detection of dark matter

Background analysis and status of the ANAIS dark matter project

ANAIS (Annual modulation with NaI Scintillators) is a project aiming to set up at the new facilities of the Canfranc Underground Laboratory (LSC), a large scale NaI(Tl) experiment in order to explore the DAMA/LIBRA annual modulation positive result using the same target and technique. Two 12.5 kg each NaI(Tl) crystals provided by Alpha Spectra took data at the LSC in the ANAIS-25 set-up. The comparison of the background model for the ANAIS-25 prototypes with the experimental results is presented. ANAIS crystal radiopurity goals have been achieved for Th-232 and U-238 chains, but a Pb-210 contamination out-of-equilibrium was identified, whose origin has been studied. The high light collection efficiency obtained with these prototypes allows to anticipate an energy threshold of the order of 1 keVee. A new detector, with improved performances, was received in March 2015 and very preliminary results are shown.Comment: 6 pages, 7 figure

Status and preliminary results of the ANAIS experiment at Canfranc

ANAIS (Annual Modulation with NaI's) is an experiment planned to investigate seasonal modulation effects in the signal of galactic WIMPs using up to 107 kg of NaI(Tl) in the Canfranc Underground Laboratory (Spain). A prototype using one single crystal (10.7 kg) is being developed before the installation of the complete experiment; the first results presented here show an average background level of 1.2 counts/(keV kg day) from threshold (Ethr~4 keV) up to 10 keV.Comment: 3 pages, 2 figures, talk delivered at the 7th International Workshop on Topics in Astroparticle and Underground Physics (TAUP 2001), September 2001, Laboratori Nazionali del Gran Sasso, Italy (to appear in the Conference Proceedings, Nucl. Phys. B (Proc. Suppl.)

Preliminary results of ANAIS-25

The ANAIS (Annual Modulation with NaI(Tl) Scintillators) experiment aims at the confirmation of the DAMA/LIBRA signal using the same target and technique at the Canfranc Underground Laboratory. 250 kg of ultrapure NaI(Tl) crystals will be used as a target, divided into 20 modules, each coupled to two photomultipliers. Two NaI(Tl) crystals of 12.5 kg each, grown by Alpha Spectra from a powder having a potassium level under the limit of our analytical techniques, form the ANAIS-25 set-up. The background contributions are being carefully studied and preliminary results are presented: their natural potassium content in the bulk has been quantified, as well as the uranium and thorium radioactive chains presence in the bulk through the discrimination of the corresponding alpha events by PSA, and due to the fast commissioning, the contribution from cosmogenic activated isotopes is clearly identified and their decay observed along the first months of data taking. Following the procedures established with ANAIS-0 and previous prototypes, bulk NaI(Tl) scintillation events selection and light collection efficiency have been also studied in ANAIS-25.Comment: 4 pages, 6 Figure

Bulk NaI(Tl) scintillation low energy events selection with the ANAIS-0 module

Dark matter particles scattering off some target nuclei are expected to deposit very small energies in form of nuclear recoils (below 100 keV). Because of the low scintillation efficiency for nuclear recoils vs. electron recoils, in most of the scintillating targets considered in the search for dark matter, the region below 10 keVee concentrates most of the expected dark matter signal. For this reason, very low energy threshold (at or below 2 keVee) and very low background are required. This is the case of the ANAIS (Annual modulation with NaI Scintillators) experiment. A good knowledge of the detector response function for real scintillation events, a good characterization of other anomalous or noise event populations contributing in that energy range, and the development of convenient filtering procedures for the latter are mandatory to achieve the required low background at such a low energy. In this work we will present the specific protocols developed to select bulk scintillation events in NaI(Tl), and its application to data obtained with the ANAIS-0 prototype. Slight differences in time constants are expected in scintillation pulses produced by nuclear or electron recoils in NaI(Tl), so in order to analyze the effect of these filtering procedures in the case of a recoil population attributable to dark matter, data from a neutron calibration have been used.Comment: 13 pages, 22 figure