25 research outputs found
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Sub-seasonal variations in lower stratospheric water vapor
Observations of water vapor with high temporal and spatial resolution and good horizontal coverage just above the tropical tropopause have been scarce, but a preliminary version of such data has been developed using radiance measurements of the Microwave Limb Sounder. These data reveal distinct variations with periods in the ranges 10-25 days and 30-70 days, consistent with (respectively) slow Kelvin waves and the tropical intraseasonal oscillation
Simulation study for measurement of horizontal wind profiles in the polar stratosphere and mesosphere using ground-based observations of ozone and carbon monoxide lines in the 230–250 GHz region
Meteorological and atmospheric models are being extended up to 80 km altitude but there are very few observing techniques that can measure stratospheric–mesospheric winds at altitudes between 20 and 80 km to verify model datasets. Here we demonstrate the feasibility of horizontal wind profile measurements using ground-based passive millimetre-wave spectroradiometric observations of ozone lines centred at 231.28, 249.79, and 249.96 GHz. Vertical profiles of horizontal winds are retrieved from forward and inverse modelling simulations of the line-of-sight Doppler-shifted atmospheric emission lines above Halley station (75°37′ S, 26°14′ W), Antarctica. For a radiometer with a system temperature of 1400 K and 30 kHz spectral resolution observing the ozone 231.28 GHz line we estimate that 12 h zonal and meridional wind profiles could be determined over the altitude range 25–74 km in winter, and 28–66 km in summer. Height-dependent measurement uncertainties are in the range 3–8 m s−1 and vertical resolution  ∼  8–16 km. Under optimum observing conditions at Halley a temporal resolution of 1.5 h for measuring either zonal or meridional winds is possible, reducing to 0.5 h for a radiometer with a 700 K system temperature. Combining observations of the 231.28 GHz ozone line and the 230.54 GHz carbon monoxide line gives additional altitude coverage at 85 ± 12 km. The effects of clear-sky seasonal mean winter/summer conditions, zenith angle of the received atmospheric emission, and spectrometer frequency resolution on the altitude coverage, measurement uncertainty, and height and time resolution of the retrieved wind profiles have been determined
The impact of the mixing properties within the Antarctic stratospheric vortex on ozone loss in spring
Calculations of equivalent length from an artificial advected tracer provide new insight into the isentropic transport processes occurring within the Antarctic stratospheric vortex. These calculations show two distinct regions of approximately equal area: a strongly mixed vortex core and a broad ring of weakly mixed air extending out to the vortex boundary. This broad ring of vortex air remains isolated from the core between late winter and midspring. Satellite measurements of stratospheric H2O confirm that the isolation lasts until at least mid-October. A three-dimensional chemical transport model simulation of the Antarctic ozone hole quantifies the ozone loss within this ring and demonstrates its isolation. In contrast to the vortex core, ozone loss in the weakly mixed broad ring is not complete. The reasons are twofold. First, warmer temperatures in the broad ring prevent continuous polar stratospheric cloud (PSC) formation and the associated chemical processing (i.e., the conversion of unreactive chlorine into reactive forms). Second, the isolation prevents ozone-rich air from the broad ring mixing with chemically processed air from the vortex core. If the stratosphere continues to cool, this will lead to increased PSC formation and more complete chemical processing in the broad ring. Despite the expected decline in halocarbons, sensitivity studies suggest that this mechanism will lead to enhanced ozone loss in the weakly mixed region, delaying the future recovery of the ozone hole
MLS Measurements of Stratospheric Hydrogen Cyanide During the 2015-2016 El Niño Event
It is known from ground-based measurements made during the 1982-1983 and 1997-1998 El Niño events that atmospheric hydrogen cyanide (HCN) tends to be higher during such years than at other times. The Microwave Limb Sounder (MLS) on the Aura satellite has been measuring HCN mixing ratios since launch in 2004; the measurements are ongoing at the time of writing. The winter of 2015- 2016 saw the largest El Niño event since 1997-1998. We present MLS measurements of HCN in the lower stratosphere for the Aura mission to date, comparing the 2015- 2016 El Niño period to the rest of the mission. HCN in 2015- 2016 is higher than at any other time during the mission, but ground-based measurements suggest that it may have been even more elevated in 1997-1998. As the MLS HCN data are essentially unvalidated, we show them alongside data from the MIPAS and ACE-FTS instruments; the three instruments agree reasonably well in the tropical lower stratosphere. Global HCN emissions calculated from the Global Fire Emissions Database (GFED v4.1) database are much greater during large El Niño events and are greater in 1997- 1998 than in 2015-2016, thereby showing good qualitative agreement with the measurements. Correlation between El Niño-Southern Oscillation (ENSO) indices, measured HCN, and GFED HCN emissions is less clear if the 2015-2016 event is excluded. In particular, the 2009-2010 winter had fairly strong El Niño conditions and fairly large GFED HCN emissions, but very little effect is observed in the MLS HCN
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Intraseasonal variations of water vapor in the tropical upper troposphere and tropopause region
We show the signature of the tropical intraseasonal oscillation (TIO) in upper tropospheric moisture and dynamical fields, roughly between 200 and 100 hPa. Relationships among these fields are examined using lag-correlation analysis and using multivariate extended empirical orthogonal functions (MEEOFs), which maximize the shared explained variance among several fields for both spatial and temporal variations. The MEEOFs show that all of the fields respond to the TIO and that the TIO is the dominant factor influencing each of the fields on these timescales. Convection associated with the TIO moistens the upper troposphere up to about 150 hPa, as expected; the behavior at 100 hPa is more complex. Over the longitude range where the TIO is associated with convection, roughly 60°-180°E, 100-hPa temperature and water vapor tend to be reduced above convection on TIO timescales. East of 180°, though, the temperature and water vapor variations at 100 hPa become decoupled. The water vapor variations, like those of 200-hPa velocity potential, appear to speed up at about 180°E