469 research outputs found
Crystal-field effects in the mixed-valence compounds Yb2M3Ga9 (M= Rh, Ir)
Magnetic susceptibility, heat capacity, and electrical resistivity
measurements have been carried out on single crystals of the intermediate
valence compounds Yb2Rh3Ga9 and Yb2Ir3Ga9. These measurements reveal a large
anisotropy due apparently to an interplay between crystalline electric field
(CEF) and Kondo effects. The temperature dependence of magnetic susceptibility
can be modelled using the Anderson impurity model including CEF within an
approach based on the Non-Crossing Approximation.Comment: Accepted to Phys. Rev.
Field-induced magnetic transitions in the quasi-two-dimensional heavy-fermion antiferromagnets Ce_{n}RhIn_{3n+2} (n=1 or 2)
We have measured the field-dependent heat capacity in the tetragonal
antiferromagnets CeRhIn and CeRhIn, both of which have an
enhanced value of the electronic specific heat coefficient
mJ/mol-Ce K above . For the specific heat data at zero
applied magnetic field are consistent with the existence of an anisotropic
spin-density wave opening a gap in the Fermi surface for CeRhIn while
CeRhIn shows behavior consistent with a simple antiferromagnetic
magnon. From these results, the magnetic structure, in a manner similar to the
crystal structure, appears more two-dimensional in CeRhIn than in
CeRhIn where only about 12% of the Fermi surface remains ungapped
relative to 92% for CeRhIn. When both compounds behave in a
manner expected for heavy fermion systems as both and the electronic
heat capacity decrease as field is applied. When the field is applied in the
tetragonal basal plane (), CeRhIn and CeRhIn have very
similar phase diagrams which contain both first- and second-order field-induced
magnetic transitions .Comment: 15 pages, 4 figure
Radiative transfer effects in primordial hydrogen recombination
The calculation of a highly accurate cosmological recombination history has
been the object of particular attention recently, as it constitutes the major
theoretical uncertainty when predicting the angular power spectrum of Cosmic
Microwave Background anisotropies. Lyman transitions, in particular the
Lyman-alpha line, have long been recognized as one of the bottlenecks of
recombination, due to their very low escape probabilities. The Sobolev
approximation does not describe radiative transfer in the vicinity of Lyman
lines to a sufficient degree of accuracy, and several corrections have already
been computed in other works. In this paper, the impact of some previously
ignored radiative transfer effects is calculated. First, the effect of Thomson
scattering in the vicinity of the Lyman-alpha line is evaluated, using a full
redistribution kernel incorporated into a radiative transfer code. The effect
of feedback of distortions generated by the optically thick deuterium
Lyman-alpha line blueward of the hydrogen line is investigated with an analytic
approximation. It is shown that both effects are negligible during cosmological
hydrogen recombination. Secondly, the importance of high-lying, non overlapping
Lyman transitions is assessed. It is shown that escape from lines above
Ly-gamma and frequency diffusion in Ly-beta and higher lines can be neglected
without loss of accuracy. Thirdly, a formalism generalizing the Sobolev
approximation is developed to account for the overlap of the high-lying Lyman
lines, which is shown to lead to negligible changes to the recombination
history. Finally, the possibility of a cosmological hydrogen recombination
maser is investigated. It is shown that there is no such maser in the purely
radiative treatment presented here.Comment: 23 pages, 4 figures, to be submitted to PR
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Life in the Atacama — Year 2: Geologic reconnaissance through long-range roving and implications on the search for life
The Life in the Atacama-2004 project, which included geological, morphological, and mineralogical mapping through combined satellite, field-based, and microscopic perspectives and long-range roving, led to the localization of potential habitats
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Spectroscopic results from the Life in the Atacama (LITA) project 2004 field season
Analysis of spectroscopy datasets from rover field tests in the Atacama Desert (Chile), focusing on the composition of the surface and identification of potential habitats for life
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Searching for life with rovers: exploration methods and science results from the 2004 field campaign of the “Life in the Atacama” project and applications to future Mars Missions
LITA develops and field tests a long-range automated rover and a science payload to search for microbial life in the Atacama. The Atacama's evolution provides a unique training ground for designing and testing exploration strategies and life detection methods for the search for life on Mars
Magnetic structure of antiferromagnetic NdRhIn5
The magnetic structure of antiferromagnetic NdRhIn5 has been determined using
neutron diffraction. It has a commensurate antiferromagnetic structure with a
magnetic wave vector (1/2,0,1/2) below T_N = 11K. The staggered Nd moment at
1.6K is 2.6mu_B aligned along the c-axis. We find the magnetic structure to be
closely related to that of its cubic parent compound NdIn3 below 4.6K. The
enhanced T_N and the absence of additional transitions below T_N for NdRhIn5
are interpreted in terms of an improved matching of the
crystalline-electric-field (CEF), magnetocrystalline, and exchange interaction
anisotropies. In comparison, the role of these competing anisotropies on the
magnetic properties of the structurally related compound CeRhIn5 is discussed.Comment: 4 pages, 4 figure
Compressibility of and (M = Rh, Ir and Co) Compounds
The lattice parameters of the tetragonal compounds CeIn and
CeIn(Rh, Ir and Co) have been studied as a function of
pressure up to 15 GPa using a diamond anvil cell under both hydrostatic and
quasihydrostatic conditions at room temperature. The addition of In
layers to the parent CeIn compound is found to stiffen the lattice as the
2-layer systems (average of bulk modulus values is 70.4 GPa) have a
larger than CeIn (67 GPa), while the 1-layer systems with the are
even stiffer (average of is 81.4 GPa). Estimating the hybridization
using parameters from tight binding calculations shows that the dominant
hybridization is in nature between the Ce and In atoms. The values of
at the pressure where the superconducting transition temperature
reaches a maximum is the same for all CeIn compounds. By
plotting the maximum values of the superconducting transition temperature
versus for the studied compounds and Pu-based superconductors, we
find a universal versus behavior when these quantities are
normalized appropriately. These results are consistent with magnetically
mediated superconductivity.Comment: Updated version resubmitted to Phys. Rev.
Heat capacity studies of Ce and Rh site substitution in the heavy fermion antiferromagnet CeRhIn_5;: Short-range magnetic interactions and non-Fermi-liquid behavior
In heavy fermion materials superconductivity tends to appear when long range
magnetic order is suppressed by chemical doping or applying pressure. Here we
report heat capacity measurements on diluted alloyes of the heavy fermion
superconductor CeRhIn_5;. Heat capacity measurements have been performed on
CeRh_{1-y}Ir_{y}In_5; (y <= 0.10) and Ce_{1-x}La_{x}Rh_{1-y}Ir_{y}In_5; (x <=
0.50) in applied fields up to 90 kOe to study the affect of doping and magnetic
field on the magnetic ground state. The magnetic phase diagram of
CeRh_{0.9}Ir_{0.1}In_5; is consistent with the magnetic structure of CeRhIn_5;
being unchanged by Ir doping. Doping of Ir in small concentrations is shown to
slightly increase the antiferromagnetic transition temperature T_{N} (T_{N}=3.8
K in the undoped sample). La doping which causes disorder on the Ce sublattice
is shown to lower T_{N} with no long range order observed above 0.34 K for
Ce_{0.50}La_{0.50}RhIn_5;. Measurements on Ce_{0.50}La_{0.50}RhIn_5; show a
coexistence of short range magnetic order and non-Fermi-liquid behavior. This
dual nature of the Ce 4f-electrons is very similar to the observed results on
CeRhIn_5; when long range magnetic order is suppressed at high pressure.Comment: 8 pages, 9 figure
An Experimental and Theoretical Study of the Variation of 4f Hybridization Across the La1-xCexIn3 Series
Crystal structures of a series of La1-xCexIn3 (x = 0.02, 0.2, 0.5, or 0.8)
intermetallic compounds have been investigated by both neutron and X-ray
diffraction, and their physical properties have been characterized by magnetic
susceptibility and specific heat measurements. Our results emphasize atypical
atomic displacement parameters (ADP) for the In and the rare-earth sites.
Depending on the x value, the In ADP presents either an "ellipsoidal"
elongation (La-rich compounds) or a "butterfly-like" distortion (Ce-rich
compounds). These deformations have been understood by theoretical techniques
based on the band theory and are the result of hybridization between conduction
electrons and 4f-electrons.Comment: 7 pages, 8 figure
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