587 research outputs found
Introducing the Fission-Fusion Reaction Process: Using a Laser-Accelerated Th Beam to produce Neutron-Rich Nuclei towards the N=126 Waiting Point of the r Process
We propose to produce neutron-rich nuclei in the range of the astrophysical
r-process around the waiting point N=126 by fissioning a dense
laser-accelerated thorium ion bunch in a thorium target (covered by a CH2
layer), where the light fission fragments of the beam fuse with the light
fission fragments of the target. Via the 'hole-boring' mode of laser Radiation
Pressure Acceleration using a high-intensity, short pulse laser, very
efficiently bunches of 232Th with solid-state density can be generated from a
Th layer, placed beneath a deuterated polyethylene foil, both forming the
production target. Th ions laser-accelerated to about 7 MeV/u will pass through
a thin CH2 layer placed in front of a thicker second Th foil closely behind the
production target and disintegrate into light and heavy fission fragments. In
addition, light ions (d,C) from the CD2 production target will be accelerated
as well to about 7 MeV/u, inducing the fission process of 232Th also in the
second Th layer. The laser-accelerated ion bunches with solid-state density,
which are about 10^14 times more dense than classically accelerated ion
bunches, allow for a high probability that generated fission products can fuse
again. In contrast to classical radioactive beam facilities, where intense but
low-density radioactive beams are merged with stable targets, the novel
fission-fusion process draws on the fusion between neutron-rich, short-lived,
light fission fragments both from beam and target. The high ion beam density
may lead to a strong collective modification of the stopping power in the
target, leading to significant range enhancement. Using a high-intensity laser
as envisaged for the ELI-Nuclear Physics project in Bucharest (ELI-NP),
estimates promise a fusion yield of about 10^3 ions per laser pulse in the mass
range of A=180-190, thus enabling to approach the r-process waiting point at
N=126.Comment: 13 pages, 6 figure
The excitation spectrum of mesoscopic proximity structures
We investigate one aspect of the proximity effect, viz., the local density of
states of a superconductor-normal metal sandwich. In contrast to earlier work,
we allow for the presence of an arbitrary concentration of impurities in the
structure. The superconductor induces a gap in the normal metal spectrum that
is proportional to the inverse of the elastic mean free path l_N for rather
clean systems. For a mean free path much shorter than the thickness of the
normal metal, we find a gap size proportional to l_N that approaches the
behavior predicted by the Usadel equation (diffusive limit). We also discuss
the influence of interface and surface roughness, the consequences of a
non-ideal transmittivity of the interface, and the dependence of our results on
the choice of the model of impurity scattering.Comment: 7 pages, 8 figures (included), submitted to PR
Diamagnetic response of cylindrical normal metal - superconductor proximity structures with low concentration of scattering centers
We have investigated the diamagnetic response of composite NS proximity
wires, consisting of a clean silver or copper coating, in good electrical
contact to a superconducting niobium or tantalum core. The samples show strong
induced diamagnetism in the normal layer, resulting in a nearly complete
Meissner screening at low temperatures. The temperature dependence of the
linear diamagnetic susceptibility data is successfully described by the
quasiclassical Eilenberger theory including elastic scattering characterised by
a mean free path l. Using the mean free path as the only fit parameter we found
values of l in the range 0.1-1 of the normal metal layer thickness d_N, which
are in rough agreement with the ones obtained from residual resistivity
measurements. The fits are satisfactory over the whole temperature range
between 5 mK and 7 K for values of d_N varying between 1.6 my m and 30 my m.
Although a finite mean free path is necessary to correctly describe the
temperature dependence of the linear response diamagnetic susceptibility, the
measured breakdown fields in the nonlinear regime follow the temperature and
thickness dependence given by the clean limit theory. However, there is a
discrepancy in the absolute values. We argue that in order to reach
quantitative agreement one needs to take into account the mean free path from
the fits of the linear response. [PACS numbers: 74.50.+r, 74.80.-g]Comment: 10 pages, 9 figure
Surface Enhanced Second Harmonic Generation from Macrocycle, Catenane, and Rotaxane Thin Films: Experiments and Theory
Surface enhanced second harmonic generation (SE SHG) experiments on molecular structures, macrocycles, catenanes, and rotaxanes, deposited as monolayers and multilayers by vacuum sublimation on silver, are reported. The measurements show that the molecules form ordered thin films, where the highest degree of order is observed in the case of macrocycle monolayers and the lowest in the case of rotaxane multilayers. The second harmonic generation activity is interpreted in terms of electric field induced second harmonic (EFISH) generation where the electric field is created by the substrate silver atoms. The measured second order nonlinear optical susceptibility for a rotaxane thin film is compared with that obtained by considering only EFISH contribution to SHG intensity. The electric field on the surface of a silver layer is calculated by using the Delphi4 program for structures obtained with TINKER molecular mechanics/dynamics simulations. An excellent agreement is observed between the calculated and the measured SHG susceptibilities.
Proton acceleration by irradiation of isolated spheres with an intense laser pulse
We report on experiments irradiating isolated plastic spheres with a peak laser intensity of 2-3 x 10(20) W cm(-2). With a laser focal spot size of 10 mu m full width half maximum (FWHM) the sphere diameter was varied between 520 nm and 19.3 mu m. Maximum proton energies of similar to 25 MeV are achieved for targets matching the focal spot size of 10 mu m in diameter or being slightly smaller. For smaller spheres the kinetic energy distributions of protons become nonmonotonic, indicating a change in the accelerating mechanism from ambipolar expansion towards a regime dominated by effects caused by Coulomb repulsion of ions. The energy conversion efficiency from laser energy to proton kinetic energy is optimized when the target diameter matches the laser focal spot size with efficiencies reaching the percent level. The change of proton acceleration efficiency with target size can be attributed to the reduced cross-sectional overlap of subfocus targets with the laser. Reported experimental observations are in line with 3D3V particle in cell simulations. They make use of well-defined targets and point out pathways for future applications and experiments.DFG via the Cluster of Excellence Munich-Centre for Advanced Photonics (MAP) Transregio SFB TR18NNSA DE-NA0002008Super-MUC pr48meIvo CermakCGC Instruments in design and realization of the Paul trap systemIMPRS-APSLMUexcellent Junior Research FundDAAD|ToIFEEuropean Union's Horizon research and innovation programme 633053Physic
Rough Surface Effect on Meissner Diamagnetism in Normal-layer of N-S Proximity-Contact System
Rough surface effect on the Meissner diamagnetic current in the normal layer
of proximity contact N-S bi-layer is investigated in the clean limit. The
diamagnetic current and the screening length are calculated by use of
quasi-classical Green's function. We show that the surface roughness has a
sizable effect, even when a normal layer width is large compared with the
coherence length . The effect is as large as that
of the impurity scattering and also as that of the finite reflection at the N-S
interface.Comment: 12 pages, 3 figures. To be published in J. Phys. Soc. Jpn. Vol.71-
Conductance of Distorted Carbon Nanotubes
We have calculated the effects of structural distortions of armchair carbon
nanotubes on their electrical transport properties. We found that the bending
of the nanotubes decreases their transmission function in certain energy ranges
and leads to an increased electrical resistance. Electronic structure
calculations show that these energy ranges contain localized states with
significant - hybridization resulting from the increased curvature
produced by bending. Our calculations of the contact resistance show that the
large contact resistances observed for SWNTs are likely due to the weak
coupling of the NT to the metal in side bonded NT-metal configurations.Comment: 5 pages RevTeX including 4 figures, submitted to PR
Performance of ab initio and density functional methods for conformational equilibria of CnH2n+2 alkane isomers (n=2-8)
Conformational energies of n-butane, n-pentane, and n-hexane have been
calculated at the CCSD(T) level and at or near the basis set limit.
Post-CCSD(T) contribution were considered and found to be unimportant. The data
thus obtained were used to assess the performance of a variety of density
functional methods. Double-hybrid functionals like B2GP-PLYP and B2K-PLYP,
especially with a small Grimme-type empirical dispersion correction, are
capable of rendering conformational energies of CCSD(T) quality. These were
then used as a `secondary standard' for a larger sample of alkanes, including
isopentane and the branched hexanes as well as key isomers of heptane and
octane. Popular DFT functionals like B3LYP, B3PW91, BLYP, PBE, and PBE0 tend to
overestimate conformer energies without dispersion correction, while the M06
family severely underestimates GG interaction energies. Grimme-type dispersion
corrections for these overcorrect and lead to qualitatively wrong conformer
orderings. All of these functionals also exhibit deficiencies in the conformer
geometries, particularly the backbone torsion angles. The PW6B95 and, to a
lesser extent, BMK functionals are relatively free of these deficiencies.
Performance of these methods is further investigated to derive conformer
ensemble corrections to the enthalpy function, , and the Gibbs
energy function, , of these alkanes. While
is only moderately sensitive to the level of theory, exhibits more pronounced sensitivity. Once again, double hybrids
acquit themselves very well.Comment: J. Phys. Chem. A, revised [Walter Thiel festschrift
Classical, non-linear, internal dynamics of large, isolated, vibrationally excited molecules
This work reports numerical experiments intended to clarify the internal
equilibration process in large molecules, following vibrational excitation. A
model of amorphous and oxygenated hydrocarbon macromolecule (about 500
atoms)--simulating interstellar dust-- is built up by means of a chemical
simulation code. Its structure is optimized, and its normal modes determined.
About 4.5 eV of potential energy is then deposited locally by perturbing one of
the C-H peripheral bonds, thus simulating the capture of a free H atom by a
dangling C bond. The ensuing relaxation of the system is followed for up to 300
ps, using a molecular mechanics code. When steady state is reached, spectra and
time correlation functions of kinetic energy and bond length fluctuations
indicate that most normal modes have been activated, but the motion remains
quasi-periodic or regular. By contrast, when the molecule is violently excited
or embedded in a thermal bath (modelled by Langevin dynamics), the same markers
clearly depict chaotic motions. Thus it appears that even such a large system
of oscillators is unable to provide the equivalent of a thermal bath to any one
of these, unless there are strong resonances between some of them. In general,
therefore, an energy of a few eV's deposited in an isolated molecule will not
be immediately thermalized. This conclusion is of consequence for the
interpretation of astronomical UIB spectra.
Key Words:IS dust--UIBs--Excitation, relaxation processes.Comment: 19 pages, 9 figures, J. of Phys. B 2002, vol 35(17
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