Growth-mode investigation of epitaxial EuS on InAs(100)

A persistent challenge in the field of spintronics is the search for suitable materials that enable the circumvention of the impedance mismatch preventing efficient spin-injection from metallic ferromagnetic conductors into semiconductors. One promising material is europium sulfide (EuS), a ferromagnetic semiconductor below the Curie temperature of 16.5 K. Investigation and optimization of the conditions required for high-quality growth of epitaxial EuS films on suitable substrates are thus of particular interest for the creation of efficient devices. We present the results of a growth-mode study employing atomic force microscopy and spot-profile analysis low-energy electron diffraction (SPA-LEED) of epitaxial EuS thin films deposited by electron-beam evaporation on InAs(100) substrates with varying combinations of, respectively, growth and annealing temperatures, Tg and Ta, from room temperature to 400 °C. We observed Stranski-Krastanov-like growth featuring low-roughness surfaces with root mean square values between 0.4 – 0.9 nm for all temperature combinations. An increased tendency for nucleation into grains and islands was observed for higher Ta from 300 – 400 °C. The corresponding nucleation mode, defined by varying degrees of 2D and 3D nucleation, was dependent on Tg. A 2D island growth mode was observed for Tg = 150 °C and Ta = 400 °C featuring a sharp and bright SPA-LEED pattern. This suggests the formation of a highly ordered, smooth surface for these growth conditions thereby providing a good starting point for optimization attempts for potential future devices

Scanning near-field optical microscopy measurements and simulations of regularly arranged silver nanoparticles

Silver nanoparticles on a glass substrate are experimentally investigated by aperture scanning near-field optical microscopy (a-SNOM). To understand the experimental results, finite-element-method simulations are performed building a theoretical model of the a-SNOM geometry. We systematically vary parameters like aperture size, aluminum-coating thickness, tip cone angle, and tip-surface distance and discuss their influence on the near-field enhancement. All these investigations are performed comparatively for constant-height and constant-gap scanning modes. In the end, we establish a reliable and stable optical model for simulating a-SNOM measurements, which is capable of reproducing trends observed in experimental data

Mapping near-field plasmonic interactions of silver particles with scanning near-field optical microscopy measurements

A scanning near-field optical microscope (SNOM) is a powerful tool to investigate optical effects that are smaller than Abbe’s limit. Its greatest strength is the simultaneous measurement of high-resolution topography and optical nearfield data that can be correlated to each other. However, the resolution of an aperture SNOM is always limited by the probe. It is a technical challenge to fabricate small illumination tips with a well-defined aperture and high transmission. The aperture size and the coating homogeneity will define the optical resolution and the optical image whereas the tip size and shape influence the topographic accuracy. Although the technique has been developing for many years, the correlation between simulated near-field data and measurement is still not convincing. To overcome this challenge, the mapping of near-field plasmonic interactions of silver nanoparticles is investigated. Different nanocluster samples with diverse distributions of silver particles are characterized via SNOM in illumination and collection mode. This will lead to topographical and optical images that can be used as an input for SNOM simulations with the aim of estimating optical artifacts. Including tip, particles, and substrate, our finite-elementmethod (FEM) simulations are based on the realistic geometry. Correlating the high- precision SNOM measurement and the detailed simulation of a full image scan will enable us to draw conclusions regarding near-field enhancements caused by interacting particles

Ultrafast transport of laser-excited spin polarized carriers in Au/Fe/MgO(001)

A time domain approach to probe hot carrier-induced spin dynamics is demonstrated. The experiments are performed in epitaxial Au/Fe/MgO(001), where spin-polarized hot carriers are excited in the Fe layer by 35 fs laser pulses. They propagate to the Au surface where the transient spin polarization is detected by magneto-induced second harmonic generation. Different energies of majority and minority hot carriers excited in the exchange-split Fe band structure lead to their spindependent lifetimes in Au. Accordingly, two spin-polarized current contributions which propagate superdiffusively at different velocities result in a spin current pulse of about 100 fs duration.Comment: 5 pages, 4 figure

The structural and electrical characterization of europium sulfide thin films prepared with E-beam evaporation

In this study, EuS thin films with varying thicknesses (15, 25, and 50 nm) were deposited onto a Si/SiO2 substrate using e-beam evaporation. Subsequently, two Ag contact electrodes with a 0.2 mm spacing were prepared via thermal evaporation using a shadow mask. To investigate the influence of film thickness and temperature on the electrical properties of EuS thin films, current-voltage (I–V) measurements were performed in a temperature range of 300–433 K for a voltage range of −2 V to +2 V. The I–V characteristics exhibited a temperature-dependent behavior, particularly showing an increase in current with rising temperature in the forward bias region. Furthermore, an improvement in the Schottky behavior was observed with increasing EuS film thickness. Additionally, the AC electrical and dielectric properties of the EuS thin film were examined in a frequency range of 4 Hz–8 MHz. Capacitance, conductance, impedance, and the Cole–Cole characteristic of EuS were analyzed in detail with respect to frequency, temperature, and film thicknesses

Proximity effecs and curie temperature enhancement in Co/EuS and Fe/EuS multilayers

Two identical Co/EuS and Fe/EuS multilayers of six periods each and with individual layers of about 4 nm thick are grown by e-beam evaporation under ultrahigh vacuum conditions. The films show polycrystalline structure with a grain size limited by the individual layer thickness. Both multilayers consist of almost continuous layers with some roughness. The surface peak-to-peak roughness is about 4–5 nm. Magnetization measurements and calculations of the loops based on a Stoner–Wohlfarth-like model allow us to determine the direct antiferromagnetic exchange coupling constant between the 3d metal and EuS at 5 K. Both samples show strong enhancement of the Curie temperature of EuS up to at least 50 K with a EuS magnetization tail, which persists up to about 100 K. The J = 7/2 character of the EuS layers is shown to be responsible for the large Curie temperature enhancement

Band-gap tuning at the strong quantum confinement regime in magnetic semiconductor EuS thin films

Ultraviolet-visible absorption spectra of nanoscaled EuS thin films reveal a blue shift of the energy between the top-valence and bottom-conduction bands. This band-gap tuning changes smoothly with decreasing film thickness and becomes significant below the exciton Bohr diameter ~3.5nm indicating strong quantum confinement effects. The results are reproduced in the framework of the potential morphing method in Hartree Fock approximation. The large values of the effective mass of the holes, due to localization of the EuS ƒ-states, limit the blue shift to about 0.35eV. This controllable band-gap tuning of magnetic semiconductor EuS renders it useful for merging spintronics and optoelectronics

Role of interactions in the magneto-plasmonic response at the geometrical threshold of surface continuity

The optical and magneto-optical behavior in periodically nanostructured surfaces at the threshold of surface continuity is revealed. We address Co films that evolve from an island-like array to a connecting network of islands that form a membrane pattern. The analysis of magneto-optical spectra as well as numerical simulations show significant differences between continuous and broken membranes that depend dramatically on the energy of the incoming radiation. Light localization increases the magneto-optical signal in the membranes. However, the generation of hot spots is not accompanied with magneto-optic enhancement. The electromagnetic field profile within the membrane system can explain the differences in the transmission and in the magneto-optic Kerr signal

Household Earnings and Income Volatility in the UK, 2009-2017

We study the volatility of sources of individual and household level income in the UK in the years 2009-2017, following the Great Recession and government austerity. We find that the volatility of (pre-tax) earnings and disposable income has fallen for the working-age in this period, largely due to fewer negative and large earnings shocks. For older individuals, we also find a fall in the volatility of private income, mainly due to fewer positive and large income shocks. Taxes and transfers help stabilise incomes, with social security cash benefits and income-dependent refundable tax credits reducing household private income volatility by around a quarter for the working age, and 40 percent for those aged 60 or over. However, over the sample period, taxes and benefits became less well correlated with earnings, reducing their ability to counteract swings in labour income. The findings illustrate the consequences of fiscal retrenchment and the cut-backs to welfare benefits on the stability of incomes