460 research outputs found
The rare genus Leptofoenus Smith, 1862 (Hymenoptera: Pteromalidae, Leptofoeninae): new records, and aspects of its distribution
Despite being the largest and most remarkable species of Chalcidoidea, species of Leptofoeninae are very rarely collected. Here, we expand the distribution range extension of the Leptofoenus howardi (Ashmead, 1895) for RondĂŽnia and Minas Gerais, Leptofoenus stephanoides (Roman, 1920) for RondĂŽnia, EspĂrito Santo and SĂŁo Paulo and Leptofoenus westwoodi (Ashmead, 1895) for Roraima, Amazonas, RondĂŽnia, Bahia, Minas Gerais, Rio de Janeiro and Rio Grande do Sul
Aeration and rheology of buttercream icings
Buttercream icings â 4 phase materials comprising sugar, butter (an emulsion) and air â are widely used for coating and decorating sweet goods. The aeration of 2:1 w/w sugar-butter mixtures was investigated in 2 benchtop planetary mixers and the rheology of the resultant viscoplastic material was quantified using lubricated compressive testing (squeeze flow and upsetting) over extensional shear rates of 10â3â100 sâ1. The aeration dynamics exhibited asymptotic behaviour which fitted a simple phenomenological model well. Optical microscopy and X-ray microtomography indicated that the air was incorporated as small bubbles of similar size to the sugar particles or as voids generated by the mixer wires. The measured yield stress was strongly dependent on the air volume fraction, Ï. The flow behaviour for one batch could be reasonably described as a Herschel-Bulkley fluid whereas a second batch gave overall better agreement with a modified power-law description: in both cases the viscous friction term decreased strongly with Ï.Fil: Fernandes, R.R.. University of Cambridge; Reino UnidoFil: Calver, K.E.. University of Cambridge; Reino UnidoFil: Hayes, D.. University of Cambridge; Reino UnidoFil: Murphy, A.E.. University of Cambridge; Reino UnidoFil: Meza, Barbara Erica del Valle. Consejo Nacional de Investigaciones CientĂficas y TĂ©cnicas. Centro CientĂfico TecnolĂłgico Conicet - Santa Fe. Instituto de Desarrollo TecnolĂłgico para la Industria QuĂmica. Universidad Nacional del Litoral. Instituto de Desarrollo TecnolĂłgico para la Industria QuĂmica; ArgentinaFil: Orona, Jesica Daiana. Consejo Nacional de Investigaciones CientĂficas y TĂ©cnicas. Centro CientĂfico TecnolĂłgico Conicet - Santa Fe. Instituto de Desarrollo TecnolĂłgico para la Industria QuĂmica. Universidad Nacional del Litoral. Instituto de Desarrollo TecnolĂłgico para la Industria QuĂmica; ArgentinaFil: Zorrilla, Susana. Consejo Nacional de Investigaciones CientĂficas y TĂ©cnicas. Centro CientĂfico TecnolĂłgico Conicet - Santa Fe. Instituto de Desarrollo TecnolĂłgico para la Industria QuĂmica. Universidad Nacional del Litoral. Instituto de Desarrollo TecnolĂłgico para la Industria QuĂmica; ArgentinaFil: Walton, H.C.. University of Cambridge; Reino UnidoFil: Wilson, D Ian. University of Cambridge; Reino UnidoFil: Peralta, Juan Manuel. Consejo Nacional de Investigaciones CientĂficas y TĂ©cnicas. Centro CientĂfico TecnolĂłgico Conicet - Santa Fe. Instituto de Desarrollo TecnolĂłgico para la Industria QuĂmica. Universidad Nacional del Litoral. Instituto de Desarrollo TecnolĂłgico para la Industria QuĂmica; Argentin
Possible Unconventional Superconductivity In Substituted Bafe 2 As 2 Revealed By Magnetic Pair-breaking Studies
The possible existence of a sign-changing gap symmetry in BaFe 2 As 2 -derived superconductors (SC) has been an exciting topic of research in the last few years. To further investigate this subject we combine Electron Spin Resonance (ESR) and pressure-dependent transport measurements to investigate magnetic pair-breaking effects on BaFe 1.9 M 0.1 As 2 (M = Mn, Co, Cu, and Ni) single crystals. An ESR signal, indicative of the presence of localized magnetic moments, is observed only for M = Cu and Mn compounds, which display very low SC transition temperature (T c) and no SC, respectively. From the ESR analysis assuming the absence of bottleneck effects, the microscopic parameters are extracted to show that this reduction of T c cannot be accounted by the Abrikosov-Gorkov pair-breaking expression for a sign-preserving gap function. Our results reveal an unconventional spin- and pressure-dependent pair-breaking effect and impose strong constraints on the pairing symmetry of these materials.4Kamihara, Y., Watanabe, T., Hirano, M., Hosono, H., Iron-based layered superconductor La[O12xFx]FeAs (x 5 0. 05-0. 12) with Tc 5 26 K (2008) J. Am. Chem. Soc., 130, p. 3296Rotter, M., Spin density wave anomaly at 140 K in the ternary iron arsenide BaFe2As2 (2008) Phys. Rev. B, 78, pp. 020503RIshida, K., Nakai, Y., Hosono, H., To what extent iron-pnictide new superconductors have been clarified: A progress report (2009) J. Phys. Soc. Japan, 78, p. 062001Hirschfeld, P.J., Korshunov, M.M., Mazin, I.I., Gap symmetry and structure of Fe-based superconductors (2011) Rep. Prog. Phys., 74, p. 124508Chubukov, A.V., Pairing mechanism in fe-based superconductors (2012) Annu. Rev. Cond. Mat. Phys., 3, p. 57Bittar, E.M., Co-substitution effects on the fe valence in the BaFe2As2 superconducting compound: A study of hard x-ray absorption spectroscopy (2011) Phys. Rev. Lett., 107, p. 267402Granado, E., Pressure and chemical substitution effects in the local atomic structure of BaFe2As2 (2011) Phys. Rev. B, 83, p. 184508Wadati, H., Elfimov, I., Sawatzky, G.A., Where are the extra d electrons in transition-metal-substituted iron pnictides? (2010) Phys. Rev. Lett., 105, p. 157004Ideta, S., Dependence of carrier doping on the impurity potential in transition-metal-substituted feas-based superconductors (2013) Phys. Rev. Lett., 110, p. 107007Berlijn, T., Lin, C.-H., Garber, W., Ku, W., Do transition-metal substitutions dope carriers in iron-based superconductors? (2012) Phys. Rev. Lett., 108, p. 207003Hin, Z.P., Haule, K., Kotliar, G., Kinetic frustration and the nature of the magnetic and paramagnetic states in iron pnictides and iron chalcogenides (2011) Nature Materials, 10, pp. 932a-935aRosa, P.F.S., Evolution of Eu21 spin dynamics in Ba12xEuxFe2As2 (2012) Phys. Rev. B, 86, p. 165131Rosa, P.F.S., (2014) Site Specific Spin Dynamics in BaFe2As2: Tuning the Ground State by Orbital Differentiation, , arxiv:1402. 2001v01Garitezi, T.M., Transport critical current measurements on a Cu-substituted BaFe2As2 superconductor (2014) J. Appl. Phys., 115, pp. 17D704Rosa, P.F.S., Pressure effects on magnetic pair-breaking in Mn- and Eusubstituted BaFe2As2 (2014) J. Appl. Phys., 115, pp. 17D702Thaler, A., Physical and magnetic properties of Ba(Fe12xMnx) 2As2 single crystals (2011) Phys. Rev. B, 84, p. 144528Et Al., A., Pressure effects on the electron-doped high Tc superconductor BaFe22xCoxAs2 (2008) J Phys. Cond. Mat., 20, p. 472201Et Al., D., Pressure versus concentration tuning of the superconductivity in Ba(Fe12xCox) 2As2 (2010) J. Phys. Soc. Japan, 79, p. 124705Yamaichi, S., Katagiri, T., Sasagawa, T., Uniaxial pressure effects on the transport properties in Ba(Fe12xCox) 2As2 single crystals (2013) Physica C, 494, pp. 62-64Canfield, P.C., Budko, S.L., Ni, N., Yan, J.Q., Kracher, A., Decoupling of the superconducting and magnetic/structural phase transitions in electron-doped BaFe2As2 (2009) Phys. Rev. B, 80, pp. 060501RKirshenbaum, K., Saha, S.R., Ziemak, S., Drye, T., Paglione, J., Universal pairbreaking in transition metal-substituted iron-pnictide superconductors (2012) Phys. Rev. B, 86, pp. 140505ROnari, S., Kontani, H., Violation of AndersonaĆ Theorem for the Sign-Reversing s-Wave State of Iron-Pnictide Superconductors (2009) Phys. Rev. Lett., 103, p. 177001Li, J., Superconductivity suppression of Ba0. 5K0. 5Fe222xMn2xAs2 single crystals by substitution of transition metal (M 5 Mn, Ru, Co, Ni, Cu, and Zn) (2012) Phys. Rev. B, 85, p. 214509Bang, Y., Choi, H.-Y., Won, H., Impurity effects on the s6-wave state of the ironbased superconductors (2009) Phys. Rev. B, 79, p. 054529Wang, Y., Kreisel, A., Hirschfeld, P.J., Mishra, V., Using controlled disorder to distinguish s6 and s11 gap structure in Fe-based superconductors (2013) Phys. Rev. B, 87, p. 094504Fernandes, R.M., Vavilov, M.G., Chubukov, A.V., Enhancement of Tc by disorder in underdoped iron pnictide superconductors (2012) Phys. Rev. B, 85, pp. 140512RNi, N., Temperature versus doping phase diagrams for Ba(Fe12xTMx) 2As2 (TM 5 Ni,Cu,Cu/Co) single crystals (2010) Phys. Rev. B, 82, p. 024519Patz, A., Ultrafast observation of critical nematic fluctuations and giant magnetoelastic coupling in iron pnictides (2014) Nature Comm., 5, p. 3229Abrikosov, A.A., Gorkov, L.P., Contribution to the theory of superconducting alloys with paramagnetic impurities (1961) Sov. Phys. JETP, 12, p. 1243Skalski, S., Betbeder-Matibet, O., Weiss, P.R., Properties of superconducting alloys containing paramagnetic impurities (1964) Phys. Rev., 136, pp. A1500-A1518Pagliuso, P.G., Electron spin resonance of Gd31 in the normal state of RNi2B2C (R 5 Y, Lu) (1998) Phys. Rev. B, 57, p. 3668Korringa, J., Nuclear magnetic relaxation and resonance line shift in metals (1950) Physica, 16, p. 601Rettori, C., Dynamic behavior of paramagnetic ions and conduction electrons in intermetallic compounds: GdxLu12xAl2 (1974) Phys. Rev. B, 10, p. 1826Davidov, D., Electron spin resonance of Gd in the intermetallic compounds YCu, YAg, and LaAg:Wave vector dependence of the exchange interaction (1973) Solid State Comm., 12, p. 621Narath, A., Weaver, H.T., Effects of electron-electron interactions on nuclear spin-lattice relaxation rates and knight shifts in alkali and noble metals (1968) Phys. Rev., 175, p. 373Shaw, R.W., Warren, W.W., Enhancement of the korringa constant in alkali metals by electron-electron interactions (1971) Phys. Rev. B, 3, p. 1562Bittar, E.M., Electron spin resonance study of the LaIn32xSnx superconducting system (2011) J. of Phys.: Cond. Matt., 23, p. 455701Maple, M.B., Dependence of s 2 f exchange on atomic number in rare earth dialuminides (1970) Solid State Comm., 8 (22), pp. 1915-1917Garitezi, T.M., Synthesis and characterization of BaFe2As2 single crystals grown by in-flux technique (2013) Brazilian Journal of Physics, 43, p. 223Alireza, P.L., Superconductivity up to 29 K in SrFe2As2 and BaFe2As2 at high pressures (2009) J. Phys. Condens. Matter, 21, p. 012208Rotter, M., Tegel, M., Johrendt, D., Superconductivity at 38 K in the Iron Arsenide Ba12xKxFe2As2 (2008) Phys. Rev. Lett., 101, p. 107006Wang, C., Thorium-dopingaĂźnduced superconductivity up to 56ĂąK in Gd12xThxFeAsO (2008) EPL, 83, p. 67006Shibata, A., Thorium-dopingaĂźnduced superconductivity up to 56ĂąK in Gd12xThxFeAsO (1986) J. Phys. Soc. Jpn., 55, p. 6Cooley, J.C., Aronson, M.C., Canfield, P.C., High pressures and the Kondo gap in Ce3Bi4Pt3 (1997) Phys. Rev. B, 55, p. 7533Oomi, G., Kagayama, T., Effect of pressure and magnetic field on the electrical resistivity of cerium kondo compounds (1996) J. Phys. Soc. Jpn., 65 (SUPPL. B), pp. 42-48Ramos, S.M., Superconducting quantum critical point in CeCoIn52xSnx (2010) Phys. Rev. Lett., 105, p. 126401Hering, E.N., PressureĂątemperatureĂącomposition phase diagram of Ce2MIn8 (2006) Physica B: Cond. Matt., 378Dyson, F.J., Electron spin resonance absorption in metals. Ii. Theory of electron diffusion and the skin effect (1955) Phys. Rev., 98, p. 349Texier, Y., Mn local moments prevent superconductivity in iron pnictides Ba(Fe12xMnx) 2As2 (2012) EPL, 99, p. 17002Leboeuf, D., (2013) NMR Study of Electronic Correlations in Mn-doped Ba(Fe12xCox) 2As2 and BaFe(As12xPx) 2, p. 4969. , arXiv1310Suzuki, H., Absence of superconductivity in the hole-doped Fe pnictide Ba(Fe12xMnx) 2As2: Photoemission and x-ray absorption spectroscopy studies (2013) Phys. Rev. B, 88, pp. 100501RKim, M.G., Effects of transition metal substitutions on the incommensurability and spin fluctuations in BaFe2As2 by elastic and inelastic neutron scattering (2012) Phys. Rev. Lett., 109, p. 167003Et Al., F., Short-range magnetic order and effective suppression of superconductivity by manganese doping in LaFe12xMnxAsO12yFy (2013) Phys. Rev. B, 87, p. 174515Golubov, A.A., Mazin, I.I., Effect of magnetic and nonmagnetic impurities on highly anisotropic superconductivity (1997) Phys. Rev. B, 55, p. 15146Openov, L.A., Combined effect of nonmagnetic and magnetic scatterers on the critical temperatures of superconductors with different anisotropies of the gap (1997) JETP Lett., 66, p. 661Efremov, D.V., Disorder-induced transition between s6 and s11 states in two-band superconductors (2011) Phys. Rev. B, 84, p. 180512Tucker, G.S., Competition between stripe and checkerboard magnetic instabilities in Mn-doped BaFe2As2 (2012) Phys. Rev. B, 86, p. 020503Fernandes, R.M., Millis, A.J., Suppression of Superconductivity by Neel-Type magnetic fluctuations in the iron pnictides (2013) Phys. Rev. Lett., 110, p. 117004Chi, S., (2013) Sign Inversion in the Superconducting Order Parameter of LiFeAs Inferred from Bogoliubov Quasiparticle Interference. ArXiv:1308. 4413v1Johnston, D.C., (2010) Adv. Phys., 59, p. 803Paglione, J., Greene, R.L., Hightemperature superconductivity in iron-based materials (2010) Nature Phys., 6, p. 645Wen, H.H., Li, S., Materials and novel superconductivity in iron pnictide superconductors (2011) Annu. Rev. Cond. Mat. Phys., 2, p. 121Stewart, G.R., Superconductivity in iron compounds (2011) Rev. Mod. Phys., 83, pp. 1589-165
Bifunctional primary amine 2-aminobenzimidazole organocatalyst anchored to trans-cyclohexane-1,2-diamine in enantioselective conjugate additions of aldehydes
Bifunctional chiral primary amine 8 containing an (S,S)-trans-cyclohexane-1,2-diamine scaffold and a 2-benzimidazole unit is used as a general organocatalyst for the Michael addition of α,α-branched aldehydes to nitroalkenes and maleimides. The reactions take place, with 20 mol % of catalyst in dichloromethane at rt for nitroalkenes and with 15 mol % catalyst loading in toluene at 10 °C for maleimides, in good yields and enantioselectivities. DFT calculations demonstrate the bifunctional character of this organocatalyst activating the aldehyde by enamine formation and the Michael acceptor by double hydrogen bonding.The Spanish Ministerio de Ciencia e InnovaciĂłn (MICINN) (projects CTQ2010-20387, and Consolider Ingenio 2010, CSD2007-00006), the Spanish Ministerio de EconomĂa y Competitividad (MINECO) (projects CTQ2013-43446-P and CTQ2014-51912-REDC), FEDER, the Generalitat Valenciana (PROMETEO 2009/039 and PROMETEOII/2014/017), the Basque Government (GV Grant IT-291-07), the FP7 Marie Curie Actions of the European Commission via the ITN ECHONET network (MCITN-2012-316379) and the Universities of Alicante and Basque Country are gratefully acknowledged for financial support. We also thank for technical and human support provided by IZO-SGI SGIker of UPV-EHU and European funding (ERDF and ESF). Financial support from Brazilian agencies CAPES-DGU (Project 200/09), CNPq, FAPERJ and UFRJ are also acknowledged. A. O. M. thanks MINECO for a FPI fellowship (BES-2014-069695)
Observation of a new chi_b state in radiative transitions to Upsilon(1S) and Upsilon(2S) at ATLAS
The chi_b(nP) quarkonium states are produced in proton-proton collisions at
the Large Hadron Collider (LHC) at sqrt(s) = 7 TeV and recorded by the ATLAS
detector. Using a data sample corresponding to an integrated luminosity of 4.4
fb^-1, these states are reconstructed through their radiative decays to
Upsilon(1S,2S) with Upsilon->mu+mu-. In addition to the mass peaks
corresponding to the decay modes chi_b(1P,2P)->Upsilon(1S)gamma, a new
structure centered at a mass of 10.530+/-0.005 (stat.)+/-0.009 (syst.) GeV is
also observed, in both the Upsilon(1S)gamma and Upsilon(2S)gamma decay modes.
This is interpreted as the chi_b(3P) system.Comment: 5 pages plus author list (18 pages total), 2 figures, 1 table,
corrected author list, matches final version in Physical Review Letter
Search for displaced vertices arising from decays of new heavy particles in 7 TeV pp collisions at ATLAS
We present the results of a search for new, heavy particles that decay at a
significant distance from their production point into a final state containing
charged hadrons in association with a high-momentum muon. The search is
conducted in a pp-collision data sample with a center-of-mass energy of 7 TeV
and an integrated luminosity of 33 pb^-1 collected in 2010 by the ATLAS
detector operating at the Large Hadron Collider. Production of such particles
is expected in various scenarios of physics beyond the standard model. We
observe no signal and place limits on the production cross-section of
supersymmetric particles in an R-parity-violating scenario as a function of the
neutralino lifetime. Limits are presented for different squark and neutralino
masses, enabling extension of the limits to a variety of other models.Comment: 8 pages plus author list (20 pages total), 8 figures, 1 table, final
version to appear in Physics Letters
Reducing heterotic M-theory to five dimensional supergravity on a manifold with boundary
This paper constructs the reduction of heterotic -theory in eleven
dimensions to a supergravity model on a manifold with boundary in five
dimensions using a Calabi-Yau three-fold. New results are presented for the
boundary terms in the action and for the boundary conditions on the bulk
fields. Some general features of dualisation on a manifold with boundary are
used to explain the origin of some topological terms in the action. The effect
of gaugino condensation on the fermion boundary conditions leads to a `twist'
in the chirality of the gravitino which can provide an uplifting mechanism in
the vacuum energy to cancel the cosmological constant after moduli
stabilisation.Comment: 16 pages, RevTe
Measurement of the inclusive isolated prompt photon cross-section in pp collisions at sqrt(s)= 7 TeV using 35 pb-1 of ATLAS data
A measurement of the differential cross-section for the inclusive production
of isolated prompt photons in pp collisions at a center-of-mass energy sqrt(s)
= 7 TeV is presented. The measurement covers the pseudorapidity ranges
|eta|<1.37 and 1.52<=|eta|<2.37 in the transverse energy range 45<=E_T<400GeV.
The results are based on an integrated luminosity of 35 pb-1, collected with
the ATLAS detector at the LHC. The yields of the signal photons are measured
using a data-driven technique, based on the observed distribution of the
hadronic energy in a narrow cone around the photon candidate and the photon
selection criteria. The results are compared with next-to-leading order
perturbative QCD calculations and found to be in good agreement over four
orders of magnitude in cross-section.Comment: 7 pages plus author list (18 pages total), 2 figures, 4 tables, final
version published in Physics Letters
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