467 research outputs found
Double-beta decay Q values of 130Te, 128Te, and 120Te
The double-beta decay Q values of 130Te, 128Te, and 120Te have been
determined from parent-daughter mass differences measured with the Canadian
Penning Trap mass spectrometer. The 132Xe-129Xe mass difference, which is
precisely known, was also determined to confirm the accuracy of these results.
The 130Te Q value was found to be 2527.01(32) keV which is 3.3 keV lower than
the 2003 Atomic Mass Evaluation recommended value, but in agreement with the
most precise previous measurement. The uncertainty has been reduced by a factor
of 6 and is now significantly smaller than the resolution achieved or foreseen
in experimental searches for neutrinoless double-beta decay. The 128Te and
120Te Q values were found to be 865.87(131) keV and 1714.81(125) keV,
respectively. For 120Te, this reduction in uncertainty of nearly a factor of 8
opens up the possibility of using this isotope for sensitive searches for
neutrinoless double-electron capture and electron capture with positron
emission.Comment: 5 pages, 2 figures, submitted to Physical Review Letter
Mass measurements near the -process path using the Canadian Penning Trap mass spectrometer
The masses of 40 neutron-rich nuclides from Z = 51 to 64 were measured at an
average precision of using the Canadian Penning Trap mass
spectrometer at Argonne National Laboratory. The measurements, of fission
fragments from a Cf spontaneous fission source in a helium gas catcher,
approach the predicted path of the astrophysical process. Where overlap
exists, this data set is largely consistent with previous measurements from
Penning traps, storage rings, and reaction energetics, but large systematic
deviations are apparent in -endpoint measurements. Differences in mass
excess from the 2003 Atomic Mass Evaluation of up to 400 keV are seen, as well
as systematic disagreement with various mass models.Comment: 15 pages, 16 figures. v2 updated, published in Physical Review
C+O sub-barrier radiative capture cross-section measurements
We have performed a heavy ion radiative capture reaction between two light
heavy ions, C and O, leading to Si. The present experiment
has been performed below Coulomb barrier energies in order to reduce the phase
space and to try to shed light on structural effects. Obtained -spectra
display a previously unobserved strong feeding of intermediate states around 11
MeV at these energies. This new decay branch is not fully reproduced by
statistical nor semi-statistical decay scenarii and may imply structural
effects. Radiative capture cross-sections are extracted from the data.Comment: 4 pages, 7 figures, to appear as proceedings of FUSION 2011
conference at St-Malo, Franc
The ethics of uncertainty for data subjects
Modern health data practices come with many practical uncertainties. In this paper, I argue that data subjects’ trust in the institutions and organizations that control their data, and their ability to know their own moral obligations in relation to their data, are undermined by significant uncertainties regarding the what, how, and who of mass data collection and analysis. I conclude by considering how proposals for managing situations of high uncertainty might be applied to this problem. These emphasize increasing organizational flexibility, knowledge, and capacity, and reducing hazard
Synthetic routes, characterization and photophysical properties of luminescent, surface functionalized nanodiamonds
The functionalization of small diameter (ca. 50 nm) polycarboxylated nanodiamond particles using amide coupling methodologies in both water and acetonitrile solvent has been investigated. In this manner, the surfaces of nanodiamond particles were adorned with different luminescent moieties, including a green fluorescent 1,8-naphthalimide species (Nap-1), and a red emitting ruthenium(II) tris-bipyridine complex (Ru-1), as well as dual functionalization with both luminophores. Comprehensive characterization of the surface functionalized nanodiamonds has been achieved using a combination of dynamic light scattering, nanoparticle tracking analysis, transmission electron microscopy, X-ray photoelectron spectroscopy, zeta potential measurements, microwave plasma atomic emission spectroscopy and time-resolved photophysics. The tendency of the functionalized nanodiamonds to aggregate reflects the degree of surface substitution, yielding small aggregates with typical particle sizes ca. 150 nm. This is likely to be driven by the reduction of the zeta potential, concomitant with the conversion of surface charged carboxylate groups to neutral amide functions. The results show that luminescent nanodiamond materials can be synthesised with tuneable photophysical properties
β-delayed neutron spectroscopy using trapped radioactive ions
A novel technique for β-delayed neutron spectroscopy has been demonstrated using trapped ions. The neutron-energy spectrum is reconstructed by measuring the time of flight of the nuclear recoil following neutron emission, thereby avoiding all the challenges associated with neutron detection, such as backgrounds from scattered neutrons and γ rays and complicated detector-response functions. I+137 ions delivered from a Cf252 source were confined in a linear Paul trap surrounded by radiation detectors, and the β-delayed neutron-energy spectrum and branching ratio were determined by detecting the β- and recoil ions in coincidence. Systematic effects were explored by determining the branching ratio three ways. Improvements to achieve higher detection efficiency, better energy resolution, and a lower neutron-energy threshold are proposed. © 2013 American Physical Society
Direct measurement of resonance strengths in S 34 (α,γ) Ar 38 at astrophysically relevant energies using the DRAGON recoil separator
Background: Nucleosynthesis of mid-mass elements is thought to occur under hot and explosive astrophysical conditions. Radiative α capture on S34 has been shown to impact nucleosynthesis in several such conditions, including core and shell oxygen burning, explosive oxygen burning, and type Ia supernovae. Purpose: Broad uncertainties exist in the literature for the strengths of three resonances within the astrophysically relevant energy range (ECM=1.94-3.42MeV at T=2.2GK). Further, there are several states in Ar38 within this energy range which have not been previously measured. This work aimed to remeasure the resonance strengths of states for which broad uncertainty existed as well as to measure the resonance strengths and energies of previously unmeasured states. Methods: Resonance strengths and energies of eight narrow resonances (five of which had not been previously studied) were measured in inverse kinematics with the DRAGON facility at TRIUMF by impinging an isotopically pure beam of S34 ions on a windowless He4 gas target. Prompt γ emissions of de-exciting Ar38 recoils were detected in an array of bismuth germanate scintillators in coincidence with recoil nuclei, which were separated from unreacted beam ions by an electromagnetic mass separator and detected by a time-of-flight system and a multianode ionization chamber. Results: The present measurements agree with previous results. Broad uncertainty in the resonance strength of the ECM=2709keV resonance persists. Resonance strengths and energies were determined for five low-energy resonances which had not been studied previously, and their strengths were determined to be significantly weaker than those of previously measured resonances. Conclusions: The five previously unmeasured resonances were found not to contribute significantly to the total thermonuclear reaction rate. A median total thermonuclear reaction rate calculated using data from the present work along with existing literature values using the STARLIB rate calculator agrees with the NON-SMOKER statistical model calculation as well as the REACLIB and STARLIB library rates at explosive and nonexplosive oxygen-burning temperatures (T=3-4GK and T=1.5-2.7GK, respectively)
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