Ultrafast Laser Nanostructured ITO Acts as Liquid Crystal Alignment Layer and Higher Transparency Electrode

Electrodes with higher transparency that can also align liquid crystals (LCs) are of high importance for improved costs and energy consumption of LC displays. Here we demonstrate for the first time alignment of liquid crystals on femtosecond laser nanostructured indium tin oxide (ITO) coated glass exhibiting also higher transparency due to the less interface reflections. The nano paterns were created by fs laser directlly on ITO films without any additional spin coating materials or lithography procces. Nine regions of laser-induced nanostructures were fabricated with different alignment orientations and various pulse energy levels on top of the ITO. The device interfacial anchoring energy was found to be comparable to the anchoring energy of nematic LC on photosensitive polymers. The device exhibits contrast of 30:1 and relaxation time of 330ms expected for thick LC devices. The measured transparency of the LC device with two ITO nanograting substrates is 10% higher than the uniform ITO film based LC devices. The alignment methodology presented here paves the way for improved LC displays and new structured LC photonic devices

Glass-metal nanocomposite modification by femtosecond laser irradiation

Modification on silver nanoparticles (AgNPs) is of interest for various nonlinear optics applications and optical data storage. Femtosecond laser modification allows elongation of spherical AgNPs [1]; these elongated particles possess intrinsic anisotropy [2], which results in dichroism [3]. Here we present the study of transmissivity and reflectivity of glass-metal nanocomposites (GMN) [4] irradiated with 330 fs laser pulses at 515 nm wavelength; the GMN was fabricated using technique based on ion-exchange [5]. The laser processing of the NP results in the dichroism exhibited in optical spectra of transmission and reflection. At higher energies we observed the increase of transmittance and decrease of reflectance, which is attributed to dissolution of NP into the glass lattice

Polarization sensitive anisotropic structuring of silicon by ultrashort light pulses

Imprinting of anisotropic structures on the silicon surface by double pulse femtosecond laser irradiation is demonstrated. The origin of the polarization-induced anisotropy is explained in terms of interaction of linearly polarized second pulse with the wavelength-sized symmetric crater-shaped structure generated by the linearly polarized first pulse. A wavefront sensor is fabricated by imprinting an array of micro-craters. Polarization controlled anisotropy of the structures can be also explored for data storage applications

Femtosecond laser nanostructuring for high-topological charge vortex tweezers with continuously tunable orbital angular momentum

It is well known that the light carries linear and angular momentum that can be transferred to the irradiated objects. Angular momentum of the beam is comprised of spin angular momentum (SAM) and orbital angular momentum (OAM). SAM is associated to the beam's polarization and is always intrinsic. OAM comes from the azimuthal phase variations of the beam and can be both extrinsic and intrinsic. The beam with helical phase phi = l.Phi, where phi is phase, Phi is polar angle and l is positive or negative integer number, possesses well-defined OAM with l.h [1]. Such beams are often referred to as optical vortices and are exploited in optical tweezer experiments enabling the rotation of trapped particles. Changing the wavefront's helicity, also the geometry of the beam is changed. The higher is |l|, the larger is the diameter of the beam. In order to change the total angular momentum of the beam, either the shape of the beam or the photon density has to be changed. As a result, the experiments which require fixed beam size and intensity are limited to fixed OAM. Recently, we implemented optical tweezers with tunable angular momentum, there OAM could be changed from -1 to 1 by controlling ellipticity of the incident laser beam. Here we extend this technology and demonstrate the generation of optical vortices of high topological charge up to 100 (Fig. 1(a)-(i)) using femtosecond laser written polarization converters (the S-waveplate) [2]

Engineering anisotropy in glass with ultrafast laser assisted nanostructuring

Recent applications of femtosecond laser assisted self-assembled nanostructures will be overviewed. Specifically, polarization sensitive optical elements and 5-dimensional optical data storage with practically unlimited life-time will be demonstrated and discussed

Functional birefringent elements imprinted by femtosecond laser nanostructuring of multi-component glass

A decade ago, a new type of self-organization process was observed in the bulk of SiO2 glass after irradiation with ultrashort laser pulses [1]. Under certain irradiation conditions, highly ordered nanostructures with features smaller than 20 nm could be formed in the irradiated volume. The sub-wavelength arrangement of these structures results in form birefringence, which was recently exploited for demonstrating a variety of functional optical elements in silica glass [2]. Despite excellent physical and chemical properties of fused silica, the applications of this glass are limited due to the expensive manufacturing process associated with high melting temperature. Recently the evidence of laser-induced nanogratings in glasses other than SiO2 was reported, including GeO2 glass [3], binary titanium silicate glass (ULE, Corning) and multicomponent borosilicate glass (Borofloat 33, Schott) [4]. However, birefringence induced in borosilicate glass was more than one order of magnitude lower than in pure SiO2 glass

Revealing the nanoparticles aspect ratio in the glass-metal nanocomposites irradiated with femtosecond laser

We studied a femtosecond laser shaping of silver nanoparticles embedded in soda-lime glass. Comparing experimental absorption spectra with the modeling based on Maxwell Garnett approximation modified for spheroidal inclusions, we obtained the mean aspect ratio of the re-shaped silver nanoparticles as a function of the laser fluence. We demonstrated that under our experimental conditions the spherical shape of silver nanoparticles changed to a prolate spheroid with the aspect ratio as high as 3.5 at the laser fluence of 0.6J/cm2. The developed approach can be employed to control the anisotropy of the glass-metal composites

Optical vortex production mediated by azimuthal index of radial polarization

[EN]Special light beams are becoming more and more interesting due to their applications in particle manipulation, micromachining, telecommunications or light matter-interaction. Both spin and orbital angular momenta of light are exploited often in combination with spatially varying linear polarization profiles (e.g. radial or azimuthal distributions). In this work we study the interaction between those polarization profiles and the spin-orbit angular momenta, finding the relation involved in the mode coupling. We find that this manipulation can be used for in-line production of collinear optical vortices with different topological charges, which can be filtered or combined with controlled linear polarization. The results are valid for continuous wave and ultrashort pulses, as well as for collimated and focused beams. We theoretically demonstrate the proposal, which is further confirmed with numerical simulations and experimental measurements with ultrashort laser pulses.This work was partially funded by Junta de Castilla y León (SA287P18) and FEDER Funds; Spanish Ministerio de Economía y Competitividad (MINECO) (FIS2017-87970-R, EQC2018-004117-P); European Research Council (ENIGMA)

Femtosecond laser printed microoptics in hydrogenated amorphous silicon

Conventional optics (e.g. lenses or mirrors) manipulates the phase via optical path difference by controlling thickness or refractive index of material. Recently, a promising type of optics emerged which exploits geometric phase shift, when a lightwave is transformed by parameter other than optical path difference, e.g. polarization. Here, wavefront is modified by introducing spatially varying anisotropy and is a result of Panchatraman-Berry phase [1]. Theoretically any phase pattern can be achieved solely by means of geometric phase with efficiencies reaching 100% [2]. This allows continuous optical phase shifts and without phase resets, in stark contrast to conventional elements, wherein phase profiles are encoded as discrete optical path variations in refractive index or thickness, limiting performance. The geometric phase optics is a promising alternative for controlling and manipulating light, but it stumbles on the lack of adequate fabrication technology