Generation and quantum control of giant plasmon pulses by transient quantum coherence

Amplified ultrashort laser pulses are useful in many fields of science and engineering. Pushing the frontiers of ultrashort pulse generation will lead to new applications in biomedical imaging, communications and sensing. We propose a new, quantum approach to ultrashort pulse generation using transient quantum coherence which predicts order of magnitude stronger pulses generated with lower input energy than in the steady-state regime, reducing the practical heating limitations. This femtosecond quantum-coherent analog of nanosecond Q-switching is not limited by the pulse duration constraints of the latter, and, in principle, may be used for a variety of lasers including x-ray and plasmon nanolasers. We apply this approach to generation of giant plasmon pulses and achieve quantum control of plasmon relaxation dynamics by varying the drive pulse delay, amplitude and duration. We provide insights into the control mechanisms, and discuss future implementations and applications of this new source of ultrashort nanooptical fields

Quantum-Coherence-Enhanced Surface Plasmon Amplification by Stimulated Emission of Radiation

We investigate surface plasmon amplification in a silver nanoparticle coupled to an externally driven three-level gain medium, and show that quantum coherence significantly enhances the generation of surface plasmons. Surface plasmon amplification by stimulated emission of radiation is achieved in the absence of population inversion on the spasing transition, which reduces the pump requirements. The coherent drive allows us to control the dynamics, and holds promise for quantum control of nanoplasmonic devices.Comment: 5 pages, 4 figure