180 research outputs found
Hysteresis in the Mott Transition between Plasma and Insulating Gas
We show that hysteresis can occur in the transition between a neutral plasma
and the insulating gas consisting of neutral pairs bound by Coulomb attraction.
Since the transition depends sensitively on the screening length in the plasma,
regions of bistability occur in density--temperature phase space. We present
numerical results which indicate where these regions occur for systems such as
spin-polarized hydrogen, positronium gas, and excitons in a semiconductor.Comment: 9 pages (Latex/RevTex), 6 postscript figures which are in compressed
and uuencoded file, prepared using the utility "uufiles" and separately
submitted. They should be automatically included with the text when it is
downloaded. Figures also available in hard copy from the authors
([email protected]; [email protected]); paper submitted to
Phys. Rev.
Excitation-assisted inelastic processes in trapped Bose-Einstein condensates
We find that inelastic collisional processes in Bose-Einstein condensates
induce local variations of the mean-field interparticle interaction and are
accompanied by the creation/annihilation of elementary excitation. The physical
picture is demonstrated for the case of three body recombination in a trapped
condensate. For a high trap barrier the production of high energy trapped
single particle excitations results in a strong increase of the loss rate of
atoms from the condensate.Comment: 4 pages, no figure
Cold Collision Frequency Shift of the 1S-2S Transition in Hydrogen
We have observed the cold collision frequency shift of the 1S-2S transition
in trapped spin-polarized atomic hydrogen. We find , where is the sample density. From this
we derive the 1S-2S s-wave triplet scattering length, nm,
which is in fair agreement with a recent calculation. The shift provides a
valuable probe of the distribution of densities in a trapped sample.Comment: Accepted for publication in PRL, 9 pages, 4 PostScript figures,
ReVTeX. Updated connection of our measurement to theoretical wor
Bragg spectroscopy of a Bose-Einstein condensate
Properties of a Bose-Einstein condensate were studied by stimulated,
two-photon Bragg scattering. The high momentum and energy resolution of this
method allowed a spectroscopic measurement of the mean-field energy and of the
intrinsic momentum uncertainty of the condensate. The coherence length of the
condensate was shown to be equal to its size. Bragg spectroscopy can be used to
determine the dynamic structure factor over a wide range of energy and momentum
transfers.Comment: 4 pages, 3 figure
Electromagnetic response of a static vortex line in a type-II superconductor : a microscopic study
The electromagnetic response of a pinned Abrikosov fluxoid is examined in the
framework of the Bogoliubov-de Gennes formalism. The matrix elements and the
selection rules for both the single photon (emission - absorption) and two
photon (Raman scattering) processes are obtained. The results reveal striking
asymmetries: light absorption by quasiparticle pair creation or single
quasiparticle scattering can occur only if the handedness of the incident
radiation is opposite to that of the vortex core states. We show how these
effects will lead to nonreciprocal circular birefringence, and also predict
structure in the frequency dependence of conductivity and in the differential
cross section of the Raman scattering.Comment: 14 pages (RevTex
Fulleretic well-defined scaffolds: Donorâfullerene alignment through metal coordination and its effect on photophysics
Herein, we report the first example of a crystalline metalâdonorâfullerene framework, in which control of the donorâfullerene mutual orientation was achieved through chemical bond formation, in particular, by metal coordination. The 13C crossâpolarization magicâangle spinning NMR spectroscopy, Xâray diffraction, and timeâresolved fluorescence spectroscopy were performed for comprehensive structural analysis and energyâtransfer (ET) studies of the fulleretic donorâacceptor scaffold. Furthermore, in combination with photoluminescence measurements, the theoretical calculations of the spectral overlap function, Förster radius, excitation energies, and band structure were employed to elucidate the photophysical and ET processes in the prepared fulleretic material. We envision that the wellâdefined fulleretic donorâacceptor materials could contribute not only to the basic science of fullerene chemistry but would also be used towards effective development of organic photovoltaics and molecular electronics
Correlating the nanostructure and electronic properties of InAs nanowires
The electronic properties and nanostructure of InAs nanowires are correlated
by creating multiple field effect transistors (FETs) on nanowires grown to have
low and high defect density segments. 4.2 K carrier mobilities are ~4X larger
in the nominally defect-free segments of the wire. We also find that dark field
optical intensity is correlated with the mobility, suggesting a simple route
for selecting wires with a low defect density. At low temperatures, FETs
fabricated on high defect density segments of InAs nanowires showed transport
properties consistent with single electron charging, even on devices with low
resistance ohmic contacts. The charging energies obtained suggest quantum dot
formation at defects in the wires. These results reinforce the importance of
controlling the defect density in order to produce high quality electrical and
optical devices using InAs nanowires.Comment: Related papers at http://pettagroup.princeton.ed
Hierarchical CorannuleneâBased Materials: Energy Transfer and SolidâState Photophysics
We report the first example of a donorâacceptor corannulene-containing hybrid material with rapid ligand-to-ligand energy transfer (ET). Additionally, we provide the first time-resolved photoluminescence (PL) data for any corannulene-based compounds in the solid state. Comprehensive analysis of PL data in combination with theoretical calculations of donorâacceptor exciton coupling was employed to estimate ET rate and efficiency in the prepared material. The ligand-to-ligand ET rate calculated using two models is comparable with that observed in fullerene-containing materials, which are generally considered for molecular electronics development. Thus, the presented studies not only demonstrate the possibility of merging the intrinsic properties of Ï-bowls, specifically corannulene derivatives, with the versatility of crystalline hybrid scaffolds, but could also foreshadow the engineering of a novel class of hierarchical corannulene-based hybrid materials for optoelectronic devices
Quantum saturation and condensation of excitons in CuO: a theoretical study
Recent experiments on high density excitons in CuO provide evidence for
degenerate quantum statistics and Bose-Einstein condensation of this nearly
ideal gas. We model the time dependence of this bosonic system including
exciton decay mechanisms, energy exchange with phonons, and interconversion
between ortho (triplet-state) and para (singlet-state) excitons, using
parameters for the excitonic decay, the coupling to acoustic and low-lying
optical phonons, Auger recombination, and ortho-para interconversion derived
from experiment. The single adjustable parameter in our model is the
optical-phonon cooling rate for Auger and laser-produced hot excitons. We show
that the orthoexcitons move along the phase boundary without crossing it (i.e.,
exhibit a ``quantum saturation''), as a consequence of the balance of entropy
changes due to cooling of excitons by phonons and heating by the non-radiative
Auger two-exciton recombination process. The Auger annihilation rate for
para-para collisions is much smaller than that for ortho-para and ortho-ortho
collisions, explaining why, under the given experimental conditions, the
paraexcitons condense while the orthoexcitons fail to do so.Comment: Revised to improve clarity and physical content 18 pages, revtex,
figures available from G. Kavoulakis, Physics Department, University of
Illinois, Urban
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