65 research outputs found
Hour-glass magnetic spectrum in a stripe-less insulating transition metal oxide
An hour-glass shaped magnetic excitation spectrum appears to be an universal
characteristic of the high-temperature superconducting cuprates. Fluctuating
charge stripes or alternative band structure approaches are able to explain the
origin of these spectra. Recently, an hour- glass spectrum has been observed in
an insulating cobaltate, thus, favouring the charge stripe scenario. Here we
show that neither charge stripes nor band structure effects are responsible for
the hour-glass dispersion in a cobaltate within the checkerboard charge ordered
regime of La2-xSrxCoO4. The search for charge stripe ordering reflections
yields no evidence for charge stripes in La1.6Sr0.4CoO4 which is supported by
our phonon studies. With the observation of an hour-glass-shaped excitation
spectrum in this stripe-less insulating cobaltate, we provide experimental
evidence that the hour-glass spectrum is neither necessarily connected to
charge stripes nor to band structure effects, but instead, probably intimately
coupled to frustration and arising chiral or non-collinear magnetic
correlations
Impact of high solar zenith angles on dynamical and chemical processes in a coupled chemistry-climate model
International audienceActinic fluxes at high solar zenith angles (SZAs) are important for atmospheric chemistry, especially under twilight conditions in polar winter and spring. The results of a sensitivity experiment employing the fully coupled 3D chemistry-climate model ECHAM4.L39(DLR)/CHEM have been analysed to quantify the impact of SZAs greater than 87.5° on dynamical and chemical processes in the lower stratosphere, in particular their influence on the ozone layer. Although the actinic fluxes at SZAs larger than 87.5° are small, ozone concentrations are significantly affected because daytime photolytic ozone destruction is switched on earlier, especially the conversion of Cl2 and Cl2O2 into ClO at the end of polar night in the lower stratosphere. Comparing climatological mean ozone column values of a simulation considering SZAs up to 93° with those of the sensitivity run with SZAs confined to 87.5° total ozone is reduced by about 20% in the polar Southern Hemisphere, i.e., the ozone hole is "deeper'' if twilight conditions are considered in the model because there is 2?3 weeks more time for ozone destruction. This causes an additional cooling of the polar lower stratosphere (50 hPa) up to ?4 K with obvious consequences for chemical processes. In the Northern Hemisphere the impact of high SZAs cannot be determined on the basis of climatological mean values due to the pronounced dynamic variability of the stratosphere in winter and spring
Incommensurate antiferromagnetic fluctuations in single-crystalline LiFeAs studied by inelastic neutron scattering
We present an inelastic neutron scattering study on single-crystalline LiFeAs
devoted to the characterization of the incommensurate antiferromagnetic
fluctuations at . Time-of-flight
measurements show the presence of these magnetic fluctuations up to an energy
transfer of 60 meV, while polarized neutrons in combination with longitudinal
polarization analysis on a triple-axis spectrometer prove the pure magnetic
origin of this signal. The normalization of the magnetic scattering to an
absolute scale yields that magnetic fluctuations in LiFeAs are by a factor
eight weaker than the resonance signal in nearly optimally Co-doped
BaFeAs, although a factor two is recovered due to the split peaks owing
to the incommensurability. The longitudinal polarization analysis indicates
weak spin space anisotropy with slightly stronger out-of-plane component
between 6 and 12 meV. Furthermore, our data suggest a fine structure of the
magnetic signal most likely arising from superposing nesting vectors.Comment: 9 pages, 8 figure
Magnetic Blue Phase in the Chiral Itinerant Magnet MnSi
Chiral nematic liquid crystals sometimes form blue phases characterized by
spirals twisting in different directions. By combining model calculations with
neutron-scattering experiments, we show that the magnetic analogue of blue
phases does form in the chiral itinerant magnet MnSi in a large part of the
phase diagram. The properties of this blue phase explain a number of previously
reported puzzling features of MnSi such as partial magnetic order and a
two-component specific-heat and thermal-expansion anomaly at the magnetic
transition
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