57 research outputs found

    Superconductivity without Fe or Ni in the phosphides BaIr2P2 and BaRh2P2

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    Heat capacity, resistivity, and magnetic susceptibility measurements confirm bulk superconductivity in single crystals of BaIr2_2P2_2 (Tc_c=2.1K) and BaRh2_2P2_2 (Tc_c = 1.0 K). These compounds form in the ThCr2_2Si2_2 (122) structure so they are isostructural to both the Ni and Fe pnictides but not isoelectronic to either of them. This illustrates the importance of structure for the occurrence of superconductivity in the 122 pnictides. Additionally, a comparison between these and other ternary phosphide superconductors suggests that the lack of interlayer P−PP-P bonding favors superconductivity. These stoichiometric and ambient pressure superconductors offer an ideal playground to investigate the role of structure for the mechanism of superconductivity in the absence of magnetism.Comment: Published in Phys Rev B: Rapid Communication

    Magnetic, thermal and transport properties of Cd doped CeIn3_3

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    We have investigated the effect of Cd substitution on the archetypal heavy fermion antiferromagnet CeIn3_3 via magnetic susceptibility, specific heat and resistivity measurements. The suppression of the Neel temperature, TN_{N}, with Cd doping is more pronounced than with Sn. Nevertheless, a doping induced quantum critical point does not appear to be achievable in this system. The magnetic entropy at TNT_N and the temperature of the maximum in resistivity are also systematically suppressed with Cd, while the effective moment and the Curie-Weiss temperature in the paramagnetic state are not affected. These results suggest that Cd locally disrupts the AFM order on its neighboring Ce moments, without affecting the valence of Ce. Moreover, the temperature dependence of the specific heat below TNT_N is not consistent with 3D magnons in pure as well as in Cd-doped CeIn3_3, a point that has been missed in previous investigations of CeIn3_3 and that has bearing on the type of quantum criticality in this system

    Wilson ratio in Yb-substituted CeCoIn5

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    We have investigated the effect of Yb substitution on the Pauli limited, heavy fermion superconductor, CeCoIn5_5. Yb acts as a non-magnetic divalent substituent for Ce throughout the entire doping range, equivalent to hole doping on the rare earth site. We found that the upper critical field in (Ce,Yb)CoIn5_5 is Pauli limited, yet the reduced (H,T) phase diagram is insensitive to disorder, as expected in the purely orbitally limited case. We use the Pauli limiting field, the superconducting condensation energy and the electronic specific heat coefficient to determine the Wilson ratio (RWR_{W}), the ratio of the specific heat coefficient to the Pauli susceptibility in CeCoIn5_5. The method is applicable to any Pauli limited superconductor in the clean limit.Comment: 5 pages, 1 table, 4 figure

    Fermi-surface topology of the iron pnictide LaFe2_2P2_2

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    We report on a comprehensive de Haas--van Alphen (dHvA) study of the iron pnictide LaFe2_2P2_2. Our extensive density-functional band-structure calculations can well explain the measured angular-dependent dHvA frequencies. As salient feature, we observe only one quasi-two-dimensional Fermi-surface sheet, i.e., a hole-like Fermi-surface cylinder around Γ\Gamma, essential for s±s_\pm pairing, is missing. In spite of considerable mass enhancements due to many-body effects, LaFe2_2P2_2 shows no superconductivity. This is likely caused by the absence of any nesting between electron and hole bands.Comment: 5 pages, 4 figure

    Unusual metamagnetism in CeIrIn5_5

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    We report a high field investigation (up to 45 T) of the metamagnetic transition in CeIrIn5_5 with resistivity and de-Haas-van-Alphen (dHvA) effect measurements in the temperature range 0.03-1 K. As the magnetic field is increased the resistivity increases, reaches a maximum at the metamagnetic critical field, and falls precipitously for fields just above the transition, while the amplitude of all measurable dHvA frequencies are significantly attenuated near the metamagnetic critical field. However, the dHvA frequencies and cyclotron masses are not substantially altered by the transition. In the low field state, the resistivity is observed to increase toward low temperatures in a singular fashion, a behavior that is rapidly suppressed above the transition. Instead, in the high field state, the resistivity monotonically increases with temperature with a dependence that is more singular than the iconic Fermi-liquid, temperature-squared, behavior. Both the damping of the dHvA amplitudes and the increased resistivity near the metamagnetic critical field indicate an increased scattering rate for charge carriers consistent with critical fluctuation scattering in proximity to a phase transition. The dHvA amplitudes do not uniformly recover above the critical field, with some hole-like orbits being entirely suppressed at high fields. These changes, taken as a whole, suggest that the metamagnetic transition in CeIrIn5_5 is associated with the polarization and localization of the heaviest of quasiparticles on the hole-like Fermi surface.Comment: 29 pages, 9 figure

    Fermi surface evolution through a heavy fermion superconductor-to-antiferromagnet transition: de Haas-van Alphen effect in Cd-substituted CeCoIn5_5

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    We report the results of de-Haas-van-Alphen (dHvA) measurements in Cd doped CeCoIn5_5 and LaCoIn5_5. Cd doping is known to induce an antiferromagnetic order in the heavy fermion superconductor CeCoIn5_5, whose effect can be reversed with applied pressure. We find a slight but systematic change of the dHvA frequencies with Cd doping in both compounds, reflecting the chemical potential shift due to the addition of holes. The frequencies and effective masses are close to those found in the nominally pure compounds with similar changes apparent in the Ce and La compounds with Cd substitution. We observe no abrupt changes to the Fermi surface in the high field paramagnetic state for x∼xcx \sim x_c corresponding to the onset of antiferromagnetic ordering at H=0 in CeCo(In1−x_{1-x}Cdx_x)5_5. Our results rule out f−f-electron localization as the mechanism for the tuning of the ground state in CeCoIn5_5 with Cd doping

    Anomalous dissipation in the mixed state of underdoped cuprates close to the superconductor-insulator boundary

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    We present a comparative study of Nernst effect and resistivity in underdoped samples of Bi2_2Sr2_2CuO6+δ_{6+\delta} and La2−x_{2-x}Srx_{x}CuO4_4. The Nernst effect presents a peak in a region of the H-T diagram where resistivity shows a non-metallic temperature dependence. Our results illustrate that the mechanism of dissipation in the mixed state of underdoped cuprates is poorly understood. Large quantum superconducting fluctuations and vanishing vortex viscosity are among suggested explanations for an enhanced Nernst signal close to the superconductor-insulator boundary.Comment: 5 pages including 3 figure

    SC-to-AFM transition in CeCo(In1-xCdx)5: De Haas-van Alphen Measurements

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    The results of de-Haas-van-Alphen (dHvA) measurements on Cd doped CeCoIn5 in the high magnetic field paramagnetic phase are reported. The replacement of trivalent In by divalent Cd is known to induce an antiferromagnetic order coexisting with superconductivity in this heavy fermion superconductor. We find a small but systematic change in the dHvA frequencies with Cd doping, reflecting the chemical potential shift due to the removal of conduction electrons. The frequencies and effective masses are close to those found in the undoped compound. We observe no abrupt change in the electron Fermi surface (FS) volume in the high field paramagnetic phase for x \u3e x c corresponding to the onset of antiferromagnetic ordering at zero magnetic field in CeCo(In1xCdx)5. Our results show that no significant change of the Fermi surface volume occurs to cause the AFM onset inside the SC state in CeCoIn5 with Cd doping. Only slight changes causing the Band 15 electron FS to be more cylindrical are observed making nesting more likely. © Published under licence by IOP Publishing Ltd

    Effects of proximity to an electronic topological transition on normal state transport properties of the high-Tc superconductors

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    Within the time dependent Ginzburg-Landau theory, the effects of the superconducting fluctuations on the transport properties above the critical temperature are characterized by a non-zero imaginary part of the relaxation rate gamma of the order parameter. Here, we evaluate Im gamma for an anisotropic dispersion relation typical of the high-Tc cuprate superconductors (HTS), characterized by a proximity to an electronic topological transition (ETT). We find that Im gamma abruptly changes sign at the ETT as a function of doping, in agreement with the universal behavior of the HTS. We also find that an increase of the in-plane anisotropy, as is given by a non-zero value of the next-nearest to nearest hopping ratio r=t'/t, increases the value of | Im gamma | close to the ETT, as well as its singular behavior at low temperature, therefore enhancing the effect of superconducting fluctuations. Such a result is in qualitative agreement with the available data for the excess Hall conductivity for several cuprates and cuprate superlattices.Comment: to appear in Phys. Rev.

    Entropy of vortex cores on the border of the superconductor-to-insulator transition in an underdoped cuprate

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    We present a study of Nernst effect in underdoped La2−xSrxCuO4La_{2-x}Sr_xCuO_4 in magnetic fields as high as 28T. At high fields, a sizeable Nernst signal was found to persist in presence of a field-induced non-metallic resistivity. By simultaneously measuring resistivity and the Nernst coefficient, we extract the entropy of vortex cores in the vicinity of this field-induced superconductor-insulator transition. Moreover, the temperature dependence of the thermo-electric Hall angle provides strong constraints on the possible origins of the finite Nernst signal above TcT_c, as recently discovered by Xu et al.Comment: 5 Pages inculding 4 figure
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