1,548 research outputs found
Dielectric breakdown induced by picosecond laser pulses
The damage thresholds of transparent optical materials were investigated. Single picosecond pulses at 1.06 microns, 0.53 microns and 0.35 microns were obtained from a mode locked Nd-YAG oscillator-amplifier-frequency multiplier system. The pulses were Gaussian in space and time and permitted the determination of breakdown thresholds with a reproducibility of 15%. It was shown that the breakdown thresholds are characteristic of the bulk material, which included nine alkali halides, five different laser host materials, KDP, quartz, sapphire and calcium fluoride. The extension of the damage data to the ultraviolet is significant, because some indication was obtained that two- and three-photon absorption processes begin to play a role in determining the threshold. Throughout the visible region of the spectrum the threshold is still an increasing function of frequency, indicating that avalanche ionization is the dominant factor in determining the breakdown threshold. This was confirmed by a detailed study of the damage morphology with a high resolution microscope just above the threshold. The influence of self focusing is discussed, and evidence for beam distortion below the power threshold for complete self focusing is presented, confirming the theory of Marburger
Hyperpolarizabilities for the one-dimensional infinite single-electron periodic systems: II. Dipole-dipole versus current-current correlations
Based on Takayama-Lin-Liu-Maki model, analytical expressions for the
third-harmonic generation, DC Kerr effect, DC-induced second harmonic optical
Kerr effect, optical Kerr effect or intensity-dependent index of refraction and
DC-electric-field-induced optical rectification are derived under the static
current-current() correlation for one-dimensional infinite chains. The
results of hyperpolarizabilities under correlation are then compared
with those obtained using the dipole-dipole () correlation. The comparison
shows that the conventional correlation, albeit quite successful for
the linear case, is incorrect for studying the nonlinear optical properties of
periodic systems.Comment: 11 pages, 5 figure
Causal vs. Noncausal Description of Nonlinear Wave Mixing; Resolving the Damping-Sign Controversy
Frequency-domain nonlinear wave mixing processes may be described either
using response functions whereby the signal is generated after all interactions
with the incoming fields, or in terms of scattering amplitudes where all fields
are treated symetrically with no specific time ordering. Closed Green's
function expressions derived for the two types of signals have different
analytical properties. The recent controversy regarding the sign of radiative
damping in the linear (Kramers Heisenberg) formula is put in a broader context
Quantum theory of light and noise polarization in nonlinear optics
We present a consistent quantum theory of the electromagnetic field in
nonlinearly responding causal media, with special emphasis on
media. Starting from QED in linearly responding causal media, we develop a
method to construct the nonlinear Hamiltonian expressed in terms of the complex
nonlinear susceptibility in a quantum mechanically consistent way. In
particular we show that the method yields the nonlinear noise polarization,
which together with the linear one is responsible for intrinsic quantum
decoherence.Comment: 4 pages, no figure
Nonlinear optical response in doped conjugated polymers
Exciton effects on conjugated polymers are investigated in soliton lattice
states. We use the Su-Schrieffer-Heeger model with long-range Coulomb
interactions. The Hartree-Fock (HF) approximation and the single-excitation
configuration- interaction (single-CI) method are used to obtain optical
absorption spectra. The third-harmonic generation (THG) at off-resonant
frequencies is calculated as functions of the soliton concentration and the
chain length of the polymer. The magnitude of the THG at the 10 percent doping
increases by the factor about 10^2 from that of the neutral system. This is
owing to the accumulation of the oscillator strengths at the lowest exciton
with increasing the soliton concentration. The increase by the order two is
common for several choices of Coulomb interaction strengths.Comment: Accepted for publication in J. Phys.: Condens. Matte
A time-dependent density functional theory scheme for efficient calculations of dynamic (hyper)polarizabilities
We present an efficient perturbative method to obtain both static and dynamic
polarizabilities and hyperpolarizabilities of complex electronic systems. This
approach is based on the solution of a frequency dependent Sternheimer
equation, within the formalism of time-dependent density functional theory, and
allows the calculation of the response both in resonance and out of resonance.
Furthermore, the excellent scaling with the number of atoms opens the way to
the investigation of response properties of very large molecular systems. To
demonstrate the capabilities of this method, we implemented it in a real-space
(basis-set free) code, and applied it to benchmark molecules, namely CO, H2O,
and paranitroaniline (PNA). Our results are in agreement with experimental and
previous theoretical studies, and fully validate our approach.Comment: 9 pages, 4 figure
Ultrafast Electronic Disordering During Femtosecond Laser Melting of GaAs
We have observed an ultrarapid electronic phase transformation to a centrosymmetric electronic state during laser excitation of GaAs with intense femtosecond pulses. Reflection second-harmonic intensity from the upper 90 atomic layers vanishes within 100 fs; reflectivity rises within 0.5 ps to a steady value characteristic of a metallic molten phase, long before phonon emission can heat the lattice to the melting temperature
Structure of multiphoton quantum optics. II. Bipartite systems, physical processes, and heterodyne squeezed states
Extending the scheme developed for a single mode of the electromagnetic field
in the preceding paper ``Structure of multiphoton quantum optics. I. Canonical
formalism and homodyne squeezed states'', we introduce two-mode nonlinear
canonical transformations depending on two heterodyne mixing angles. They are
defined in terms of hermitian nonlinear functions that realize heterodyne
superpositions of conjugate quadratures of bipartite systems. The canonical
transformations diagonalize a class of Hamiltonians describing non degenerate
and degenerate multiphoton processes. We determine the coherent states
associated to the canonical transformations, which generalize the non
degenerate two--photon squeezed states. Such heterodyne multiphoton squeezed
are defined as the simultaneous eigenstates of the transformed, coupled
annihilation operators. They are generated by nonlinear unitary evolutions
acting on two-mode squeezed states. They are non Gaussian, highly non
classical, entangled states. For a quadratic nonlinearity the heterodyne
multiphoton squeezed states define two--mode cubic phase states. The
statistical properties of these states can be widely adjusted by tuning the
heterodyne mixing angles, the phases of the nonlinear couplings, as well as the
strength of the nonlinearity. For quadratic nonlinearity, we study the
higher-order contributions to the susceptibility in nonlinear media and we
suggest possible experimental realizations of multiphoton conversion processes
generating the cubic-phase heterodyne squeezed states.Comment: 16 pages, 23 figure
Hole Doping Effects on Spin-gapped Na2Cu2TeO6 via Topochemical Na Deficiency
We report the magnetic susceptibility and NMR studies of a spin-gapped
layered compound
Na2Cu2TeO6 (the spin gap 250 K), the hole doping effect on the
Cu2TeO6 plane via a topochemical Na deficiency by soft chemical treatment, and
the static spin vacancy effect by nonmagnetic impurity Zn substitution for Cu.
A finite Knight shift at the Te site was observed for pure
Na2Cu2TeO6.
The negative hyperfine coupling constant is an evidence for
the existence of a superexchange pathway of the Cu-O-Te-O-Cu bond. It turned
out that both the Na deficiency and Zn impurities induce a Curie-type magnetism
in the uniform spin susceptibility in an external magnetic field of 1 T, but
only the Zn impurities enhance the low-temperature Na nuclear
spin-lattice relaxation rate whereas the Na deficiency suppresses it. A spin
glass behavior was observed for the Na-deficient samples but not for the
Zn-substituted samples. The dynamics of the unpaired moments of the doped holes
are different from that of the spin vacancy in the spin-gapped Cu2TeO6 planes.Comment: 4 pages, 7 figures, to be published in J. Phys. Soc. Jpn. Vol. 75,
No. 8 (2006
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