Short-time water caging and transient electron-OH couplings in liquid phase

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Small Atomic Displacements Recorded in Bismuth by the Optical Reflectivity of Femtosecond Laser-Pulse Excitations

International audienceSubtle atomic motion in a Bi crystal excited by a 35 fs-laser pulse has been recovered from the transient reflectivity of an optical probe measured with an accuracy of 10^-5. Analysis shows that a novel effect reported here—an initial negative drop in reflectivity—relates to a delicate coherent displacement of atoms by the polarization force during the pulse. We also show that reflectivity oscillations with a frequency coinciding with that of cold Bi are related to optical phonons excited by the electron temperature gradient through electron-phonon coupling

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International audienceA Reply to the Comment by Oleg V. Misochko, Masahiro Kitajima, and Kunie Ishioka

Polarization Control in Two-Color Above-Threshold Ionization of Atomic Helium

Two-color multiphoton ionization of atomic helium was investigated by combining extreme ultraviolet (XUV) radiation from the Free Electron Laser in Hamburg with an intense synchronized optical laser. In the photoelectron spectrum, lines associated with direct ionization and above-threshold ionization show strong variations of their amplitudes as a function of both the intensity of the optical dressing field and the relative orientation of the linear polarization vectors of the two fields. The polarization dependence provides direct insight into the symmetry of the outgoing electrons in above-threshold ionization. In the high field regime, the monochromaticity of the XUV radiation enables the unperturbed observation of nonlinear processes in the optical field