Three-body Interactions In Proton-helium Angular Scattering

H++He scattering at 0.5 MeV has been investigated using a coincidence technique that completely determines the three-body transverse momentum exchange in single ionization collisions. Three scattering regions could be distinctly recognized that are dominated by proton helium-nucleus, proton-electron, or electron helium-nucleus interactions. Calculations and the experimental data show that the coupling between the electronic and nuclear degrees of freedom is required to understand the dynamics for more than 97% of the ionizing collisions. © 1989 The American Physical Society

Complete Single-Ionization Momentum Spectra for Strong Perturbation Collisions

The combination of recoil ion and ionized electron momentum spectroscopy provides an unparalleled method to investigate the details of ion-atom collision dynamics in kinematically complete experiments. To predict single ionization scattering behavior at the level now realized by experiment, the classical trajectory three-body Monte Carlo method has been used to obtain complete momenta information for the ionized electron, recoil ion, and projectile in the collision plane defined by the incident projectile and outgoing recoil ion. Strongly coupled systems were considered where the charge state of the projectile divided by the speed of the collision [Formula Presented] is greater than unity. Illustrated are 3.6-MeV/nucleon [Formula Presented] and 9.5-MeV/nucleon [Formula Presented] collisions on He where experimental data are available. The theoretical results are in good agreement with these data and calculations have been performed for 165-keV/nucleon and 506-keV/nucleon [Formula Presented] to compare results for the same [Formula Presented] perturbation strengths, but at much lower velocities. In all cases the ejected electrons are found to be preferentially emitted opposite to the recoil ion in the projectile-recoil collision plane. The 165-keV/nucleon [Formula Presented] spectra are especially rich in that electron capture strongly contributes to the overall electron loss process. Here, the electron capture to the continuum (ECC) spectrum is observed to have not only the known asymmetry in the longitudinal direction, but also has an almost complete asymmetry in the collision plane opposite to the recoil ion. Collision plane spectra differential in the transverse momenta of the recoil ion depict the transition from soft electrons for low transverse recoil momenta, to two-center, and ECC electrons for increasing transverse recoil ion momenta. © 1998 The American Physical Society

Dependence Of Binary Encounter Electron Production On The Charge State Of The Recoil Ion

We study the dependence of the production of binary encounter electrons on the charge state of recoil ions for 2.4 MeV u-l Xe21+ on He and Ar. Doubly differential cross sections of electron emission are calculated with the ncrMC method. We find that the contributions to the binary electron cross section from various recoil ion charge states reach a maximum near Ar5+ for the Ar target. In the case of the He target; double ionization dominates over single ionization for alt ejected electron energies above 100 eV. However, an unexpected local drop of double ionization in the binary peak region has been observed. This decrease is found to be related to a two-step, sequential removal of the two electrons. © 1993 IOP Publishing Ltd

Quantum Interference In Clothed-ion-atom Binary Peak Structures

An impulse approximation for ionizing collisions of clothed ions with atoms is used to explain the origin of an anomalous oscillation in the ejected electron spectrum in the region of the binary peak. In addition, measurements which evidence this feature for 1-MeV/u U21+ ions colliding with helium are presented. It is shown that this behavior arises from interference structures in the elastic differential cross section for the scattering of target electrons from the impinging ion and that it is associated with the well-known phenomenon of rainbow scattering. © 1991 The American Physical Society

Time Resolved Experiments at the Frankfurt 14 GHz ECR Ion Source

To investigate the basic production processes of highly charged ions and combined phenomena of an ECRIS plasma (e. g. influence of secondary electrons and plasma instabilities) time resolved experiments have been carried out at the Frankfurt 14 GHz ECRIS [1] (see also the contributions to this workshop by O. Hohn et al. and V. Mironov et al.). We report time resolved measurements of the extracted ion currents by pulsing the biased disk voltage [2]. The measurements have shown that the extracted ion currents respond too fast to explain the "biased disk effect" (i. e. the intensity increase of highly charged ions) by enhanced ion breeding. Furthermore the influence of the pulsed biased disk on plasma instabilities has been investigated. It has also been shown that this method can be used to extract pulsed ion beams from an ECRIS

Transition From Quantum To Quasi-classical Behaviour Of The Binary Encounter Peak In Collisions Of 0.6 To 3.6 Mev Amu“¹ I23+ And Xe21+ With He And Ar

Double differentia] cross sections are reported for the production of binary encounter electrons in collisions of 0.6 MeV amu-1 I23+ and 1.4, 2.4, and 3.6 MeV amu-1 Xe21+ projectiles incident on He and Ar targets. Electron energy spectra were measured between 0: and 45: in the case of the two lower projectile energies, and between 17.5° and 60- for the two higher projectile energies. The data are compared with quantum mechanical impulse approximation and classical trajectory Monte Carlo calculations. While the quantum model calculation predicts a rapid disappearance of diffraction effects in the binary encounter peak with increasing projectile energy, these remain visible in the experimental results up to the highest energy measured. The necessity of including multiple target ionization involving inner shell electrons in the theoretica] description of the collision process is demonstrated by the classical trajectory Monte Carlo calculation, which accounts well for the shape of the 2.4 and 3.6 MeV amu-1 cross sections, except at angles where diffraction effects are manifest. Systematic shifts of the binary encounter peak position towards lower energies with increasing emission angle were observed for all projectile energies. © 1993 IOP Publishing Ltd

Carbon K-shell Photo Ionization of CO: Molecular frame angular Distributions of normal and conjugate shakeup Satellites

We have measured the molecular frame angular distributions of photoelectrons emitted from the Carbon K shell of fixed-in-space CO molecules for the case of simultaneous excitation of the remaining molecular ion. Normal and conjugate shake up states are observed. Photo electrons belonging to normal \Sigma -satellite lines show an angular distribution resembling that observed for the main photoline at the same electron energy. Surprisingly a similar shape is found for conjugate shake up states with \Pi -symmetry. In our data we identify shake rather than electron scattering (PEVE) as the mechanism producing the conjugate lines. The angular distributions clearly show the presence of a \Sigma -shape resonance for all of the satellite lines.Comment: 8 pages, 2 figure

Complete Momentum Balance for Single Ionization of Helium by Fast Ion Impact: Experiment

The collision dynamics of He single ionization by [Formula Presented] impact was explored using the reaction microscope of the Gesellschaft für Schwerionenforschung, a high-resolution integrated multielectron recoil-ion momentum spectrometer. The complete three-particle final-state momentum distribution (nine Cartesian components [Formula Presented]) was imaged with a resolution of [Formula Presented] by measuring the three momentum components of the emitted electron and the recoiling target ion in coincidence. The projectile energy loss has been determined on a level of [Formula Presented] and projectile scattering angles as small as [Formula Presented] became accessible. The experimental data which are compared with results of classical trajectory Monte Carlo calculations reveal an unprecedented insight into the details of the electron emission and the collision dynamics for ionization of helium by fast heavy-ion impact. © 1997 The American Physical Society

Interatomic Coulombic Decay following Photoionization of the Helium Dimer: Observation of Vibrational Structure

Using synchrotron radiation we simultaneously ionize and excite one helium atom of a helium dimer (He_2) in a shakeup process. The populated states of the dimer ion (i.e. He^[*+](n = 2; 3)-He) are found to deexcite via interatomic coulombic decay. This leads to the emission of a second electron from the neutral site and a subsequent coulomb explosion. In this letter we present a measurement of the momenta of fragments that are created during this reaction. The electron energy distribution and the kinetic energy release of the two He^+ ions show pronounced oscillations which we attribute to the structure of the vibrational wave function of the dimer ion.Comment: 8 pages, 5 figure