193 research outputs found
Linewidths in bound state resonances for helium scattering from Si(111)-(1x1)H
Helium-3 spin-echo measurements of resonant scattering from the Si(111)–(1 × 1)H surface, in the energy range 4–14 meV, are presented. The measurements have high energy resolution yet they reveal bound state resonance features with uniformly broad linewidths. We show that exact quantum mechanical calculations of the elastic scattering, using the existing potential for the helium/Si(111)–(1 × 1)H interaction, cannot reproduce the linewidths seen in the experiment. Further calculations rule out inelastic and other mechanisms that might give rise to losses from the elastic scattering channels. We show that corrugation in the attractive part of the atom–surface potential is the most likely origin of the experimental lineshapes
How Atomic Steps Modify Diffusion and Inter-adsorbate Forces: Empirical Evidence from Hopping Dynamics in Na/Cu(115).
We followed the collective atomic-scale motion of Na atoms on a vicinal Cu(115) surface within a time scale of pico- to nanoseconds using helium spin echo spectroscopy. The well-defined stepped structure of Cu(115) allows us to study the effect that atomic steps have on the adsorption properties, the rate for motion parallel and perpendicular to the step edge, and the interaction between the Na atoms. With the support of a molecular dynamics simulation we show that the Na atoms perform strongly anisotropic 1D hopping motion parallel to the step edges. Furthermore, we observe that the spatial and temporal correlations between the Na atoms that lead to collective motion are also anisotropic, suggesting the steps efficiently screen the lateral interaction between Na atoms residing on different terraces.This work was supported by the German-Israeli Foundation for Scientific Research and Development, the Israeli Science Foundation (Grant No. 2011185), the German Science Foundation (DFG) through contract MO 960/18-1, the Cluster of Excellence RESOLV (EXC 1069), and the European Research Council under the European Union’s seventh framework program (FP/2007-2013)/ERC Grant 307267.This is the author accepted manuscript. The final version is available from ACS via http://dx.doi.org/10.1021/acs.jpclett.5b0193
Parallel and anti-parallel echoes in beam spin echo experiments
The refocusing of velocity-dependent spin-phase is the basic phenomenon behind helium and neutron spin echo beam experiments. In this paper we present quantum and classical descriptions of the spin echo phenomenon and show that non-adiabatic transitions, such as those which take place during rotation of the magnetic field axis between the two arms of a helium spin echo setup, lead to echo conditions without reversing the magnetic field orientation between the two arms. The usual spin echo conditions, created by reversing the magnetic field orientation, do not require such non-adiabatic transitions. These two echo conditions are termed parallel and anti-parallel spin echoes, respectively. We derive the dependence of the relative intensity of the two echoes on the scattering geometry of the setup and show experimental results which verify the co-existence of the two echo conditions, the theoretically derived expressions for their relative intensity and the effect of an additional spin rotator coil introduced within the non-adiabatic transition region
Random Walks with Long-Range Self-Repulsion on Proper Time
We introduce a model of self-repelling random walks where the short-range
interaction between two elements of the chain decreases as a power of the
difference in proper time. Analytic results on the exponent are obtained.
They are in good agreement with Monte Carlo simulations in two dimensions. A
numerical study of the scaling functions and of the efficiency of the algorithm
is also presented.Comment: 25 pages latex, 4 postscript figures, uses epsf.sty (all included)
IFUP-Th 13/92 and SNS 14/9
Probability Distribution of the Shortest Path on the Percolation Cluster, its Backbone and Skeleton
We consider the mean distribution functions Phi(r|l), Phi(B)(r|l), and
Phi(S)(r|l), giving the probability that two sites on the incipient percolation
cluster, on its backbone and on its skeleton, respectively, connected by a
shortest path of length l are separated by an Euclidean distance r. Following a
scaling argument due to de Gennes for self-avoiding walks, we derive analytical
expressions for the exponents g1=df+dmin-d and g1B=g1S-3dmin-d, which determine
the scaling behavior of the distribution functions in the limit x=r/l^(nu) much
less than 1, i.e., Phi(r|l) proportional to l^(-(nu)d)x^(g1), Phi(B)(r|l)
proportional to l^(-(nu)d)x^(g1B), and Phi(S)(r|l) proportional to
l^(-(nu)d)x^(g1S), with nu=1/dmin, where df and dmin are the fractal dimensions
of the percolation cluster and the shortest path, respectively. The theoretical
predictions for g1, g1B, and g1S are in very good agreement with our numerical
results.Comment: 10 pages, 3 figure
Two-Dimensional Wetting of a Stepped Copper Surface.
Highly corrugated, stepped surfaces present regular 1D arrays of binding sites, creating a complex, heterogeneous environment to water. Rather than decorating the hydrophilic step sites to form 1D chains, water on stepped Cu(511) forms an extended 2D network that binds strongly to the steps but bridges across the intervening hydrophobic Cu(100) terraces. The hydrogen-bonded network contains pentamer, hexamer, and octomer water rings that leave a third of the stable Cu step sites unoccupied in order to bind water H down close to the step dipole and complete three hydrogen bonds per molecule.Herchel Smith fun
Dynamical Scaling from Multi-Scale Measurements
We present a new measure of the Dynamical Critical behavior: the "Multi-scale
Dynamical Exponent (MDE)"Comment: 9 pages,Latex, Request figures from [email protected]
Crossover phenomena in spin models with medium-range interactions and self-avoiding walks with medium-range jumps
We study crossover phenomena in a model of self-avoiding walks with
medium-range jumps, that corresponds to the limit of an -vector
spin system with medium-range interactions. In particular, we consider the
critical crossover limit that interpolates between the Gaussian and the
Wilson-Fisher fixed point. The corresponding crossover functions are computed
using field-theoretical methods and an appropriate mean-field expansion. The
critical crossover limit is accurately studied by numerical Monte Carlo
simulations, which are much more efficient for walk models than for spin
systems. Monte Carlo data are compared with the field-theoretical predictions
concerning the critical crossover functions, finding a good agreement. We also
verify the predictions for the scaling behavior of the leading nonuniversal
corrections. We determine phenomenological parametrizations that are exact in
the critical crossover limit, have the correct scaling behavior for the leading
correction, and describe the nonuniversal lscrossover behavior of our data for
any finite range.Comment: 43 pages, revte
Monte Carlo computation of correlation times of independent relaxation modes at criticality
We investigate aspects of universality of Glauber critical dynamics in two
dimensions. We compute the critical exponent and numerically corroborate
its universality for three different models in the static Ising universality
class and for five independent relaxation modes. We also present evidence for
universality of amplitude ratios, which shows that, as far as dynamic behavior
is concerned, each model in a given universality class is characterized by a
single non-universal metric factor which determines the overall time scale.
This paper also discusses in detail the variational and projection methods that
are used to compute relaxation times with high accuracy
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