Efficient and spectrally bright source of polarization-entangled photons

We demonstrate an efficient fiber-coupled source of nondegenerate polarization entangled photons at 795 and 1609 nm using bidirectionally pumped parametric down-conversion in bulk periodically poled lithium niobate. The single-mode source has an inferred bandwidth of 50 GHz and a spectral brightness of 300 pairs/s/GHz/mW of pump power that is suitable for narrowband applications such as entanglement transfer from photonic to atomic qubits.Comment: 8 pages, 7 figures, submitted to Phys. Rev.

Two-photon coincident-frequency-entanglement via extended phase matching

We demonstrate a new class of frequency-entangled states generated via spontaneous parametric down-conversion under extended phase matching conditions. Biphoton entanglement with coincident signal and idler frequencies is observed over a broad bandwidth in periodically poled KTiOPO$_4$. We demonstrate high visibility in Hong-Ou-Mandel interferometric measurements under pulsed pumping without spectral filtering, which indicates excellent frequency indistinguishability between the down-converted photons. The coincident-frequency entanglement source is useful for quantum information processing and quantum measurement applications.Comment: 4 pages, 3 figures, submitted to PR

Practical decoy state method in quantum key distribution with heralded single photon source

We propose a practical decoy state method with heralded single photon source for quantum key distribution (QKD). In the protocol, 3 intensities are used and one can estimate the fraction of single-photon counts. The final key rate over transmission distance is simulated under various parameter sets. Due to the lower dark count than that of a coherent state, it is shown that a 3-intensity decoy-state QKD with a heralded source can work for a longer distance than that of a coherent state.Comment: 10 pages, 4 Postscript figure

Efficient generation of tunable photon pairs at 0.8 and 1.6 micrometer

We demonstrate efficient generation of collinearly propagating, highly nondegenerate photon pairs in a periodically-poled lithium niobate cw parametric downconverter with an inferred pair generation rate of 1.4*10^7/s/mW of pump power. Detection of an 800-nm signal photon triggers a thermoelectrically-cooled 20%-efficient InGaAs avalanche photodiode for the detection of the 1600-nm conjugate idler photon. Using single-mode fibers as spatial mode filters, we obtain a signal-conditioned idler-detection probability of about 3.1%.Comment: 8 pages, 3 figure

Efficient upconversion of sub-THz radiation in a high-Q whispering gallery resonator

We demonstrate efficient upconversion of sub-THz radiation into the optical domain in a high-Q whispering gallery mode resonator with quadratic optical nonlinearity. The 5x10^{-3} power conversion efficiency of continuous wave 100GHz signal is achieved with only 16 mW of optical pump.Comment: This revision is limited to discussion of only optical WGMs coupled with the external Rf field. Discussion of RF WGMs is now posted separatel

Supramolecular interactions in clusters of polar and polarizable molecules

We present a model for molecular materials made up of polar and polarizable molecular units. A simple two state model is adopted for each molecular site and only classical intermolecular interactions are accounted for, neglecting any intermolecular overlap. The complex and interesting physics driven by interactions among polar and polarizable molecules becomes fairly transparent in the adopted model. Collective effects are recognized in the large variation of the molecular polarity with supramolecular interactions, and cooperative behavior shows up with the appearance, in attractive lattices, of discontinuous charge crossovers. The mean-field approximation proves fairly accurate in the description of the gs properties of MM, including static linear and non-linear optical susceptibilities, apart from the region in the close proximity of the discontinuous charge crossover. Sizeable deviations from the excitonic description are recognized both in the excitation spectrum and in linear and non-linear optical responses. New and interesting phenomena are recognized near the discontinuous charge crossover for non-centrosymmetric clusters, where the primary photoexcitation event corresponds to a multielectron transfer.Comment: 14 pages, including 11 figure

A photonic quantum information interface

Quantum communication is the art of transferring quantum states, or quantum bits of information (qubits), from one place to another. On the fundamental side, this allows one to distribute entanglement and demonstrate quantum nonlocality over significant distances. On the more applied side, quantum cryptography offers, for the first time in human history, a provably secure way to establish a confidential key between distant partners. Photons represent the natural flying qubit carriers for quantum communication, and the presence of telecom optical fibres makes the wavelengths of 1310 and 1550 nm particulary suitable for distribution over long distances. However, to store and process quantum information, qubits could be encoded into alkaline atoms that absorb and emit at around 800 nm wavelength. Hence, future quantum information networks made of telecom channels and alkaline memories will demand interfaces able to achieve qubit transfers between these useful wavelengths while preserving quantum coherence and entanglement. Here we report on a qubit transfer between photons at 1310 and 710 nm via a nonlinear up-conversion process with a success probability greater than 5%. In the event of a successful qubit transfer, we observe strong two-photon interference between the 710 nm photon and a third photon at 1550 nm, initially entangled with the 1310 nm photon, although they never directly interacted. The corresponding fidelity is higher than 98%.Comment: 7 pages, 3 figure

Quantum Transduction of Telecommunications-band Single Photons from a Quantum Dot by Frequency Upconversion

The ability to transduce non-classical states of light from one wavelength to another is a requirement for integrating disparate quantum systems that take advantage of telecommunications-band photons for optical fiber transmission of quantum information and near-visible, stationary systems for manipulation and storage. In addition, transducing a single-photon source at 1.3 {\mu}m to visible wavelengths for detection would be integral to linear optical quantum computation due to the challenges of detection in the near-infrared. Recently, transduction at single-photon power levels has been accomplished through frequency upconversion, but it has yet to be demonstrated for a true single-photon source. Here, we transduce the triggered single-photon emission of a semiconductor quantum dot at 1.3 {\mu}m to 710 nm with a total detection (internal conversion) efficiency of 21% (75%). We demonstrate that the 710 nm signal maintains the quantum character of the 1.3 {\mu}m signal, yielding a photon anti-bunched second-order intensity correlation, g^(2)(t), that shows the optical field is composed of single photons with g^(2)(0) = 0.165 < 0.5.Comment: 7 pages, 4 figure

Nanoparticles for highly efficient multiphoton fluorescence bioimaging

In this paper, we demonstrate for the first time that the new class of fluoride-based inorganic upconverting nanoparticles, NaYF4:Er3+, Yb3+, are the most efficient multiphoton excited fluorescent nanoparticles developed to date. The near-infrared-to-visible conversion efficiency of the aforementioned nanoparticles surpasses that of CdSe quantum dots and gold nanorods, which are the commercially available inorganic fluorescent nanoprobes presently used for multiphoton fluorescence bioimaging. The results presented here open new perspectives for the implementation of fluorescence tomography by multiphoton fluorescence imaging