1,497 research outputs found
Optical properties of small polarons from dynamical mean-field theory
The optical properties of polarons are studied in the framework of the
Holstein model by applying the dynamical mean-field theory. This approach
allows to enlighten important quantitative and qualitative deviations from the
limiting treatments of small polaron theory, that should be considered when
interpreting experimental data. In the antiadiabatic regime, accounting on the
same footing for a finite phonon frequency and a finite electron bandwidth
allows to address the evolution of the optical absorption away from the
well-understood molecular limit. It is shown that the width of the multiphonon
peaks in the optical spectra depends on the temperature and on the frequency in
a way that contradicts the commonly accepted results, most notably in the
strong coupling case. In the adiabatic regime, on the other hand, the present
method allows to identify a wide range of parameters of experimental interest,
where the electron bandwidth is comparable or larger than the broadening of the
Franck-Condon line, leading to a strong modification of both the position and
the shape of the polaronic absorption. An analytical expression is derived in
the limit of vanishing broadening, which improves over the existing formulas
and whose validity extends to any finite-dimensional lattice. In the same
adiabatic regime, at intermediate values of the interaction strength, the
optical absorption exhibits a characteristic reentrant behavior, with the
emergence of sharp features upon increasing the temperature -- polaron
interband transitions -- which are peculiar of the polaron crossover, and for
which analytical expressions are provided.Comment: 16 pages, 6 figure
Statistical Mechanics and Information-Theoretic Perspectives on Complexity in the Earth System
Peer reviewedPublisher PD
Common solar wind drivers behind magnetic storm-magnetospheric substorm dependency
The dynamical relationship between magnetic storms and magnetospheric
substorms presents one of the most controversial problems of contemporary
geospace research. Here, we tackle this issue by applying a causal inference
approach to two corresponding indices in conjunction with several relevant
solar wind variables. We demonstrate that the vertical component of the
interplanetary magnetic field is the strongest and common driver of both,
storms and substorms, and explains their the previously reported association.
These results hold during both solar maximum and minimum phases and suggest
that, at least based on the analyzed indices, there is no statistical evidence
for a direct or indirect dependency between substorms and storms. A physical
mechanism by which substorms drive storms or vice versa is, therefore,
unlikely.Comment: 18 pages, 6 figure
Characterization of the first true coaxial 18-fold segmented n-type prototype detector for the GERDA project
The first true coaxial 18-fold segmented n-type HPGe prototype detector
produced by Canberra-France for the GERDA neutrinoless double beta-decay
project was tested both at Canberra-France and at the Max-Planck-Institut fuer
Physik in Munich. The main characteristics of the detector are given and
measurements concerning detector properties are described. A novel method to
establish contacts between the crystal and a Kapton cable is presented.Comment: 21 pages, 16 Figures, to be submitted to NIM
A global disorder of imprinting in the human female germ line
Imprinted genes are expressed differently depending on whether they are carried by a chromosome of maternal or paternal origin. Correct imprinting is established by germline-specific modifications; failure of this process underlies several inherited human syndromes. All these imprinting control defects are cis-acting, disrupting establishment or maintenance of allele-specific epigenetic modifications across one contiguous segment of the genome. In contrast, we report here an inherited global imprinting defect. This recessive maternal-effect mutation disrupts the specification of imprints at multiple, non-contiguous loci, with the result that genes normally carrying a maternal methylation imprint assume a paternal epigenetic pattern on the maternal allele. The resulting conception is phenotypically indistinguishable from an androgenetic complete hydatidiform mole, in which abnormal extra-embryonic tissue proliferates while development of the embryo is absent or nearly so. This disorder offers a genetic route to the identification of trans-acting oocyte factors that mediate maternal imprint establishment
Polaronic excitations in CMR manganite films
In the colossal magnetoresistance manganites polarons have been proposed as
the charge carrier state which localizes across the metal-insulator transition.
The character of the polarons is still under debate. We present an assessment
of measurements which identify polarons in the metallic state of
La{2/3}Sr{1/3}MnO{3} (LSMO) and La{2/3}Ca{1/3}MnO{3} (LCMO) thin films. We
focus on optical spectroscopy in these films which displays a pronounced
resonance in the mid-infrared. The temperature dependent resonance has been
previously assigned to polaron excitations. These polaronic resonances are
qualitatively distinct in LSMO and LCMO and we discuss large and small polaron
scenarios which have been proposed so far. There is evidence for a large
polaron excitation in LSMO and small polarons in LCMO. These scenarios are
examined with respect to further experimental probes, specifically charge
carrier mobility (Hall-effect measurements) and high-temperature
dc-resistivity.Comment: 16 pages, 10 figure
Photoinduced IR absorption in (La(1-x)Sr(x)Mn)(1-\delta)O3: changes of the anti-Jahn-Teller polaron binding energy with doping
Photoinduced IR absorption was measured in (La(1-x)Sr(x)Mn)(1-\delta)O3. A
midinfrared peak centered at ~ 5000 cm was observed in the x=0
antiferromagnetic sample. The peak diminishes and softens as hole doping is
increased. The origin of the photoinduced absorption peak is atributted to the
photon assisted hopping of anti-Jahn-Teller polarons formed by photoexcited
charge carriers, whose binding energy decreases with increasing hole doping.
The shape of the peak indicates that the polarons are small.Comment: 5 pages, 3 figures, submitted to PR
Geometric and dynamic perspectives on phase-coherent and noncoherent chaos
Statistically distinguishing between phase-coherent and noncoherent chaotic
dynamics from time series is a contemporary problem in nonlinear sciences. In
this work, we propose different measures based on recurrence properties of
recorded trajectories, which characterize the underlying systems from both
geometric and dynamic viewpoints. The potentials of the individual measures for
discriminating phase-coherent and noncoherent chaotic oscillations are
discussed. A detailed numerical analysis is performed for the chaotic R\"ossler
system, which displays both types of chaos as one control parameter is varied,
and the Mackey-Glass system as an example of a time-delay system with
noncoherent chaos. Our results demonstrate that especially geometric measures
from recurrence network analysis are well suited for tracing transitions
between spiral- and screw-type chaos, a common route from phase-coherent to
noncoherent chaos also found in other nonlinear oscillators. A detailed
explanation of the observed behavior in terms of attractor geometry is given.Comment: 12 pages, 13 figure
Histone modifications form a cell-type-specific chromosomal bar code that persists through the cell cycle.
Chromatin configuration influences gene expression in eukaryotes at multiple levels, from individual nucleosomes to chromatin domains several Mb long. Post-translational modifications (PTM) of core histones seem to be involved in chromatin structural transitions, but how remains unclear. To explore this, we used ChIP-seq and two cell types, HeLa and lymphoblastoid (LCL), to define how changes in chromatin packaging through the cell cycle influence the distributions of three transcription-associated histone modifications, H3K9ac, H3K4me3 and H3K27me3. We show that chromosome regions (bands) of 10-50 Mb, detectable by immunofluorescence microscopy of metaphase (M) chromosomes, are also present in G1 and G2. They comprise 1-5 Mb sub-bands that differ between HeLa and LCL but remain consistent through the cell cycle. The same sub-bands are defined by H3K9ac and H3K4me3, while H3K27me3 spreads more widely. We found little change between cell cycle phases, whether compared by 5 Kb rolling windows or when analysis was restricted to functional elements such as transcription start sites and topologically associating domains. Only a small number of genes showed cell-cycle related changes: at genes encoding proteins involved in mitosis, H3K9 became highly acetylated in G2M, possibly because of ongoing transcription. In conclusion, modified histone isoforms H3K9ac, H3K4me3 and H3K27me3 exhibit a characteristic genomic distribution at resolutions of 1 Mb and below that differs between HeLa and lymphoblastoid cells but remains remarkably consistent through the cell cycle. We suggest that this cell-type-specific chromosomal bar-code is part of a homeostatic mechanism by which cells retain their characteristic gene expression patterns, and hence their identity, through multiple mitoses
Polaronic optical absorption in electron-doped and hole-doped cuprates
Polaronic features similar to those previously observed in the photoinduced
spectra of cuprates have been detected in the reflectivity spectra of
chemically doped parent compounds of high-critical-temperature superconductors,
both -type and -type. In NdCuO these features, whose
intensities depend both on doping and temperature, include local vibrational
modes in the far infrared and a broad band centered at 1000 cm.
The latter band is produced by the overtones of two (or three) local modes and
is well described in terms of a small-polaron model, with a binding energy of
about 500 cm. Most of the above infrared features are shown to survive
in the metallic phase of NdCeCu0, BiSrCuO, and
YBaCuO, where they appear as extra-Drude peaks. The occurrence
of polarons is attributed to local modes strongly coupled to carriers, as shown
by a comparison with tunneling results.Comment: File latex, 31 p., submitted to Physical Review B. Figures may be
faxed upon reques
- …