Experimental demonstration of stimulated polarization wave in a chain of nuclear spins

A stimulated wave of polarization, which implements a simple mechanism of quantum amplification, is experimentally demonstrated in a chain of four J-coupled nuclear spins, irradiated by a weak radio-frequency transverse field. The "quantum domino" dynamics, a wave of flipped spins triggered by a flip of the first spin, has been observed in fully $^{13}$C-labeled sodium butyrate.Comment: 8 pages including 3 figure

Projective measurement in nuclear magnetic resonance

It is demonstrated that nuclear magnetic resonance experiments using pseudopure spin states can give possible outcomes of projective quantum measurement and probabilities of such outcomes. The physical system is a cluster of six dipolar-coupled nuclear spins of benzene in a liquid-crystalline matrix. For this system with the maximum total spin S=3, the results of measuring $S_X$ are presented for the cases when the state of the system is one of the eigenstates of $S_Z$.Comment: 9 pages incluing 3 figure

Preparation of pseudopure state in a cluster of dipolar-coupled spins with "unresolved" spectrum

A method of creating pseudopure spin states in large clusters of coupled spins is described. It is based on filtering multiple-quantum coherence of the highest order followed by a time-reversal period and partial saturation. Experimental demonstration is presented for a cluster of six dipolar-coupled proton spins of a benzene molecule in liquid crystalline matrix, and the details of spin dynamics are studied numerically.Comment: 15 pages, 3 figures, submitted to Phys. Rev.

Selective excitation of homogeneous spectral lines

It is possible, for homogeneously broadened lines, to excite selectively the response signals, which are orders of magnitude narrower than the original lines. The new type of echo, which allows detecting such signals, and the formalism, useful for understanding the phenomenon, as well as the experimental examples from NMR spectroscopy are presented.Comment: 19 pages, 8 figure

NMR Simulation of an Eight-State Quantum System

The propagation of excitation along a one-dimensional chain of atoms is simulated by means of NMR. The physical system used as an analog quantum computer is a nucleus of 133-Cs (spin 7/2) in a liquid crystalline matrix. The Hamiltonian of migration is simulated by using a special 7-frequency pulse, and the dynamics is monitored by following the transfer of population from one of the 8 spin energy levels to the other.Comment: 10 pages, 3 figure