6,709 research outputs found
The development of liquid crystal lasers for application in fluorescence microscopy
Lasers can be found in many areas of optical medical imaging and their properties have enabled the rapid advancement of many imaging techniques and modalities. Their narrow linewidth, relative brightness and coherence are advantageous in obtaining high quality images of biological samples. This is particularly beneficial in fluorescence microscopy. However, commercial imaging systems depend on the combination of multiple independent laser sources or use tuneable sources, both of which are expensive and have large footprints. This thesis demonstrates the use of liquid crystal (LC) laser technology, a compact and portable alternative, as an exciting candidate to provide a tailorable light source for fluorescence microscopy.
Firstly, to improve the laser performance parameters such that high power and high specification lasers could be realised; device fabrication improvements were presented. Studies exploring the effect of alignment layer rubbing depth and the device cell gap spacing on laser performance were conducted. The results were the first of their kind and produced advances in fabrication that were critical to repeatedly realising stable, single-mode LC laser outputs with sufficient power to conduct microscopy. These investigations also aided with the realisation of laser diode pumping of LC lasers. Secondly, the identification of optimum dye concentrations for single and multi-dye systems were used to optimise the LC laser mixtures for optimal performance. These investigations resulted in novel results relating to the gain media in LC laser systems. Collectively, these advancements yielded lasers of extremely low threshold, comparable to the lowest reported thresholds in the literature.
A portable LC laser system was integrated into a microscope and used to perform fluorescence microscopy. Successful two-colour imaging and multi-wavelength switching ability of LC lasers were exhibited for the first time. The wavelength selectivity of LC lasers was shown to allow lower incident average powers to be used for comparable image quality. Lastly, wavelength selectivity enabled the LC laser fluorescence microscope to achieve high enough sensitivity to conduct quantitative fluorescence measurements. The development of LC lasers and their suitability to fluorescence microscopy demonstrated in this thesis is hoped to push towards the realisation of commercialisation and application for the technology
Crystal Structures of Metal Complexes
This reprint contains 11 papers published in a Special Issue of Molecules entitled "Crystal Structures of Metal Complexes". I will be very happy if readers will be interested in the crystal structures of metal complexes
Direct measurement of coating thermal noise in the AEI 10m prototype
A thermal noise interferometer for the characterization of thermal noise in high reflectivity mirrors has been commissioned and first direct measurements of coating thermal noise have been performed. This serves as an important step in the improvement of current and future gravitational wave detectors
Wavelength Tunable MECSELs
Membrane external-cavity surface-emitting lasers (MECSELs) represent a relatively new category of semiconductor laser that have potential to be attractive tunable light sources for various applications. Potential advantages over similar lasers include improved active region heat extraction, access to novel wavelength regimes, and wider tuning ranges. Semiconductor membranes with varying quantum well architectures were investigated in this thesis. Additionally, varying cavity configurations and intracavity elements were investigated with the goal of satisfying application-specific properties required for implementation
The 2023 terahertz science and technology roadmap
Terahertz (THz) radiation encompasses a wide spectral range within the electromagnetic spectrum that extends from microwaves to the far infrared (100 GHzââŒ30 THz). Within its frequency boundaries exist a broad variety of scientific disciplines that have presented, and continue to present, technical challenges to researchers. During the past 50 years, for instance, the demands of the scientific community have substantially evolved and with a need for advanced instrumentation to support radio astronomy, Earth observation, weather forecasting, security imaging, telecommunications, non-destructive device testing and much more. Furthermore, applications have required an emergence of technology from the laboratory environment to production-scale supply and in-the-field deployments ranging from harsh ground-based locations to deep space. In addressing these requirements, the research and development community has advanced related technology and bridged the transition between electronics and photonics that high frequency operation demands. The multidisciplinary nature of THz work was our stimulus for creating the 2017 THz Science and Technology Roadmap (Dhillon et al 2017 J. Phys. D: Appl. Phys. 50 043001). As one might envisage, though, there remains much to explore both scientifically and technically and the field has continued to develop and expand rapidly. It is timely, therefore, to revise our previous roadmap and in this 2023 version we both provide an update on key developments in established technical areas that have important scientific and public benefit, and highlight new and emerging areas that show particular promise. The developments that we describe thus span from fundamental scientific research, such as THz astronomy and the emergent area of THz quantum optics, to highly applied and commercially and societally impactful subjects that include 6G THz communications, medical imaging, and climate monitoring and prediction. Our Roadmap vision draws upon the expertise and perspective of multiple international specialists that together provide an overview of past developments and the likely challenges facing the field of THz science and technology in future decades. The document is written in a form that is accessible to policy makers who wish to gain an overview of the current state of the THz art, and for the non-specialist and curious who wish to understand available technology and challenges. A such, our experts deliver a 'snapshot' introduction to the current status of the field and provide suggestions for exciting future technical development directions. Ultimately, we intend the Roadmap to portray the advantages and benefits of the THz domain and to stimulate further exploration of the field in support of scientific research and commercial realisation
Laser Technologies for Applications in Quantum Information Science
Scientific progress in experimental physics is inevitably dependent on continuing advances in the underlying technologies. Laser technologies enable controlled coherent and dissipative atom-light interactions and micro-optical technologies allow for the implementation of versatile optical systems not accessible with standard optics.
This thesis reports on important advances in both technologies with targeted applications ranging from Rydberg-state mediated quantum simulation and computation with individual atoms in arrays of optical tweezers to high-resolution spectroscopy of highly-charged ions.
A wide range of advances in laser technologies are reported: The long-term stability and maintainability of external-cavity diode laser systems is improved significantly by introducing a mechanically adjustable lens mount. Tapered-amplifier modules based on a similar lens mount are developed. The diode laser systems are complemented by digital controllers for laser frequency and intensity stabilisation. The controllers offer a bandwidth of up to 1.25 MHz and a noise performance set by the commercial STEMlab platform. In addition, shot-noise limited photodetectors optimised for intensity stabilisation and Pound-Drever-Hall frequency stabilisation as well as a fiber based detector for beat notes in the MHz-regime are developed. The capabilities of the presented techniques are demonstrated by analysing the performance of a laser system used for laser cooling of Rb85 at a wavelength of 780 nm. A reference laser system is stabilised to a spectroscopic reference provided by modulation transfer spectroscopy. This spectroscopy scheme is analysed finding optimal operation at high modulation indices. A suitable signal is generated with a compact and cost-efficient module. A scheme for laser offset-frequency stabilisation based on an optical phase-locked loop is realised. All frequency locks derived from the reference laser system offer a Lorentzian linewidth of 60 kHz (FWHM) in combination with a long-term stability of 130 kHz peak-to-peak within 10 days. Intensity stabilisation based on acousto-optic modulators in combination with the digital controller allows for real-time intensity control on microsecond time scales complemented by a sample and hold feature with a response time of 150 ns.
High demands on the spectral properties of the laser systems are put forward for the coherent excitation of quantum states. In this thesis, the performance of active frequency stabilisation is enhanced by introducing a novel current modulation technique for diode lasers. A flat response from DC to 100 MHz and a phase lag below 90° up to 25 MHz are achieved extending the bandwidth available for laserfrequency stabilisation. Applying this technique in combination with a fast proportional-derivative controller, two laser fields with a relative phase noise of 42 mrad for driving rubidium ground state transitions are realised. A laser system for coherent Rydberg excitation via a two-photon scheme provides light at 780 nm and at 480 nm via frequency-doubling from 960 nm. An output power of 0.6 W at 480 nm from a single-mode optical fiber is obtained . The frequencies of both laser systems are stabilised to a high-finesse reference cavity resulting in a linewidth of 1.02 kHz (FWHM) at 960 nm. Numerical simulations quantify the effect of the finite linewidth on the coherence of Rydberg Rabi-oscillations. A laser system similar to the 480 nm Rydberg system is developed for spectroscopy on highly charged bismuth.
Advanced optical technologies are also at the heart of the micro-optical generation of tweezer arrays that offer unprecedented scalability of the system size. By using an optimised lens system in combination with an automatic evaluation routine, a tweezer array with several thousand sites and trap waists below 1 ÎŒm is demonstrated. A similar performance is achieved with a microlens array produced in an additive manufacturing process. The microlens design is optimised for the manufacturing process. Furthermore, scattering rates in dipole traps due to suppressed resonant light are analysed proving the feasibility of dipole trap generation using tapered amplifier systems
Electrically tunable VO2-metal metasurface for mid-infrared switching, limiting, and nonlinear isolation
We demonstrate an electrically controlled metal-VO2 metasurface for the
mid-wave infrared that simultaneously functions as a tunable optical switch, an
optical limiter with a tunable limiting threshold, and a nonlinear optical
isolator with a tunable operating range. The tunability is achieved via Joule
heating through the metal comprising the metasurface, resulting in an
integrated optoelectronic device. As an optical switch, the device has an
experimental transmission ratio of ~100 when varying the bias current.
Operating as an optical limiter, we demonstrated tunability of the limiting
threshold from 20 mW to 180 mW of incident laser power. Similar degrees of
tunability are also achieved for nonlinear optical isolation, which enables
asymmetric (nonreciprocal) transmission.Comment: Main text + supplementar
Hybridization of Surface Plasmon Polaritons and Molecular Excitations
Starke Kopplung von MolekĂŒlen mit einem rĂ€umlich begrenzten Lichtfeld fĂŒhrt zur Bildung neuer polaritonischer EigenzustĂ€nde des Systems, die sowohl molekulare als auch photonische Eigenschaften erhalten und somit ein groĂes Potenzial fĂŒr Anwendungen in der Chemie und Optoelektronik besitzen.
In dieser Arbeit wird die Kopplung zwischen OberflÀchenplasmonen Polaritonen (SPPs), die als das rÀumlich begrenzte Lichtfeld agieren, und molekularen Anregungen wie Schwingungen und polaronischen Resonanzen untersucht.
Das starke Kopplungsregime zwischen einer MolekĂŒlschwingung und einem SPP wird zum ersten Mal im mittleren Infrarot unter Verwendung der Carbonylschwingung von Poly(vinylmethylketon) Polymer und Silber als Ausbreitungsmedium von SPPs demonstriert. Die neu gebildeten Hybridmoden werden durch Experimente und numerische Modellierung untersucht, wobei Messungen der abgeschwĂ€chten Totalreflexion und der thermischen Emission sowie Berechnungen mittels der Transfermatrix und der linearen Dispersionstheorie verwendet werden. Ein Anticrossing in der Dispersion der Polariton-Zweige mit einer Energieaufspaltung bis zu 15 meV, was die Hauptsignatur des starken Kopplungsregimes ist, wird beobachtet.
Die starke Kopplung mit Zinkgalliumoxid, einem hochdotierten Halbleiter als Alternative zu Edelmetallen, wird auch untersucht. Experimentelle und simulierte Reflektometrie-Spektren sowie Dispersionsrelationen werden diskutiert, um RĂŒckschlĂŒsse auf die Eigenschaften des Systems zu ziehen. AuĂerdem wird ein Ansatz zur Verbesserung der LeitfĂ€higkeit organischer Halbleiterpolymere durch starke Kopplung ihrer polaronischen ZustĂ€nde an SPPs vorgestellt und LeitfĂ€higkeitsmessungen durchgefĂŒhrt. Ziel ist es, die Delokalisierung der HybridzustĂ€nde auszunutzen, um die LeitfĂ€higkeit zu verĂ€ndern.
Die prĂ€sentierten Ergebnisse bieten neue Einblicke in den Nutzen der Eigenschaften der Licht-Materie-Hybridisierung, um ihr volles Potenzial fĂŒr verschiedene Bereiche und Anwendungen zu erforschen.Strong coupling of molecules with a confined light field results in the formation of new polaritonic eigenstates of the system called polaritons that inherit both molecular and photonic characteristics and thus holds strong potential for applications in chemistry and optoelectronics.
In this work, coupling between propagating surface plasmon polaritons (SPPs), as confined light field, and molecular excitations, such as vibrational resonances and polaronic features, is investigated.
The strong coupling regime between a molecular vibration and a propagating SPP is demonstrated for the first time in the mid-infrared spectral range using the carbonyl stretch vibration of Poly(vinyl methyl ketone) polymer and silver as metallic medium for SPPs propagation. The newly formed hybrid modes are investigated through experiments and numerical modelling, employing attenuated-total-reflection and thermal emission measurements as well as transfer-matrix and linear dispersion theory calculations. An anticrossing behavior in the dispersion of the polariton branches with an energy splitting up to 15meV, which is a key signature of the strong coupling regime, is observed.
Strong coupling involving zinc gallium oxide, which is a highly doped semiconductor, as an alternative to noble metals is also investigated. Experimental and simulated reflectometry spectra as well as the dispersion relations are discussed so as to draw conclusions about the properties of the system. Furthermore, an approach to enhance the conductivity of organic semiconductor polymers by strongly coupling their polaronic states to SPPs is presented and four-point probe measurements are conducted. The goal is to exploit the delocalization of the hybrid states to alter the conductivity of the organic semiconductor.
The results presented in this thesis provide new insights into the profit from the properties of light-matter hybridization in order to explore its full potential for several areas and applications
Toward an active CMOS electronics-photonics platform based on subwavelength structured devices
The scaling trend of microelectronics over the past 50 years, quantified by Mooreâs Law, has faced insurmountable bottlenecks, necessitating the use of optical communication with its high bandwidth and energy efficiency to further improve computing performance.
Silicon photonics, compatible with CMOS platform manufacturing, presents a promising means to achieve on-chip optical links, employing highly sensitive microring resonator devices that demand electronic feedback and control due to fabrication variations. Achieving the full potential of both technologies requires tight integration to realize the ultimate benefits of both realms of technology, leading to the convergence of microelectronics and photonics.
A promising approach for achieving this convergence is the monolithic integration of electronics and photonics on CMOS platforms. A critical milestone was reached in 2015 with the demonstration of the first microprocessor featuring photonic I/O (Chen et al, Nature 2015), accomplished by integrating transistors and photonic devices on a single chip using a monolithic CMOS silicon-on-insulator (SOI) platform (GlobalFoundries 45RFSOI, 45 nm SOI process) without process modifications, thus known as the "zero-change" approach. This dissertation focuses on leveraging the fabrication capabilities of advanced monolithic electronic-photonic 45 nm CMOS platforms, specifically high-resolution lithography and small feature size doping implants, to realize photonic devices with subwavelength features that could potentially provide the next leap in integrated optical links performance, beyond microring resonator based links.
Photonic crystal (PhC) nanobeam cavities can support high-quality resonance modes while confining light in a small volume, enhancing light-matter interactions and potentially enabling ultimate efficiencies in active devices such as modulators and photodetectors. However, PhC cavities have been overshadowed by microring resonators due to two challenges. First, their fabrication demands high lithography resolution, which excludes most standard SOI photonic platforms as viable options for creating these devices. Secondly, the standing-wave nature of PhC nanobeam cavities complicates their integration into wavelength-division multiplexing (WDM) optical links, causing unwanted reflections when coupled evanescently to a bus waveguide.
In this work, we present PhC nanobeam cavities with the smallest footprint, largest intrinsic quality factor, and smallest mode volume to be demonstrated to date in a monolithic CMOS platform. The devices were fabricated in a 45 nm monolithic electronicsâphotonics CMOS platform optimized for silicon photonics, GlobalFoundries 45CLO, exhibiting a quality factor in excess of 100,000 the highest among fully cladded PhC nanobeam cavities in any SOI platform. Furthermore to eliminate reflections, we demonstrate an approach using pairs of PhC nanobeam cavities with opposite spatial mode symmetries to mimic traveling-wave-like ring behavior, enabling efficient and seamless WDM link integration. This concept was extended to realize a reflectionless microring resonator unit with two microrings operating as standing-wave cavities. Using this scheme with standing-wave microring resonators could lead to an optimum geometry for microring modulators with interdigitated p-n junctions in terms of modulation efficiency in a manner that allows for straightforward WDM cascading.
This work also presents the first demonstration of resonant-structure-based modulators in the GlobalFoundries 45CLO platform. We report the first-ever demonstration of a PhC modulator in a CMOS platform, featuring a novel design with sub-wavelength contacts on one side allowing it to benefit from the "reflection-less"' architecture. Additionally, we also report the first demonstration of microring modulators. The most efficient devices exhibited electro-optical bandwidths up to 30 GHz, and 25 Gbps non-return-to-zero (NRZ) on-off-keyed (OOK) modulation with 1 dB insertion loss and 3.1 dB extinction ratio.
Finally, as the complexity of silicon photonic systems-on-a-chip (SoC) increases to enable new applications such as low-energy data links, quantum optics, and neuromorphic computing, the need for in-situ characterization of individual components becomes increasingly important. By combining Near-field scanning optical microscopy (NSOM) with a flip-chip post-processing technique, this dissertation demonstrates a method to non-invasively perform NSOM scans of a photonic device within a large-scale CMOS-photonic circuit, without interfering with the performance and packaging of the photonics and electronics, making it a valuable tool for future development of high performance photonic circuits and systems
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