Mechanisms of hydrological responses to volcanic eruptions in the Asian monsoon and westerlies-dominated subregions

Explosive volcanic eruptions affect surface climate, especially in monsoon regions, but responses vary in different regions and to volcanic aerosol injection (VAI) in different hemispheres. Here, we use six ensemble members from the last-millennium experiment of the Coupled Model Intercomparison Project Phase 5 to investigate the mechanisms of regional hydrological responses to different hemispheric VAIs in the Asian monsoon region (AMR). Northern hemispheric VAI (NHVAI) leads to an intensified aridity over the AMR after northern hemispheric VAI (NHVAI); spatially, a distinct inverse response pattern to the climatological conditions emerges, with an intensified aridity in the relatively wettest area (RWA) but a weakened aridity in the relatively driest area (RDA) of the AMR. Southern hemispheric VAI (SHVAI) shows a weakened aridity over the AMR, but the spatial response pattern is not that clear due to small aerosol magnitude. The mechanism of the hydrological impact relates to the indirect change of atmospheric circulation due to the direct radiative effect of volcanic aerosols. The decreased thermal contrast between the land and the ocean after NHVAI results in a weakened East Asian summer monsoon and South Asian summer monsoon. This changes the moisture transport and cloud formation in the monsoon and westerlies-dominated subregions. The subsequent radiative effect and physical feedbacks of local clouds lead to different hydrological effects in different areas. Results here indicate that future volcanic eruptions may temporarily alleviate the uneven distribution of precipitation in the AMR, which should be considered in the near-term climate predictions and future strategies of local adaptation to global warming. The local hydrological responses and mechanisms found here can also provide a reference for stratospheric aerosol engineering

The effect of regional changes in anthropogenic aerosols on rainfall of the East Asian summer monsoon

The response of East Asian Summer Monsoon (EASM) precipitation to long term changes in regional anthropogenic aerosols (sulphate and black carbon) is explored in an atmospheric general circulation model, the atmospheric component of the UK High-Resolution Global Environment Model v1.2 (HiGAM). Separately, sulphur dioxide (SO2) and black carbon (BC) emissions in 1950 and 2000 over East Asia are used to drive model simulations, while emissions are kept constant at year 2000 level outside this region. The response of the EASM is examined by comparing simulations driven by aerosol emissions representative of 1950 and 2000. The aerosol radiative effects are also determined using an off-line radiative transfer model. During June, July and August, the EASM was not significantly changed as either SO2 or BC emissions increased from 1950 to 2000 levels. However, in September, precipitation is significantly decreased by 26.4% for sulphate aerosol and 14.6% for black carbon when emissions are at the 2000 level. Over 80% of the decrease is attributed to changes in convective precipitation. The cooler land surface temperature over China in September (0.8 °C for sulphate and 0.5 °C for black carbon) due to increased aerosols reduces the surface thermal contrast that supports the EASM circulation. However, mechanisms causing the surface temperature decrease in September are different between sulphate and BC experiments. In the sulphate experiment, the sulphate direct and the 1st indirect radiative effects contribute to the surface cooling. In the BC experiment, the BC direct effect is the main driver of the surface cooling, however, a decrease in low cloud cover due to the increased heating by BC absorption partially counteracts the direct effect. This results in a weaker land surface temperature response to BC changes than to sulphate changes. The resulting precipitation response is also weaker, and the responses of the monsoon circulation are different for sulphate and black carbon experiments. This study demonstrates a mechanism that links regional aerosol emission changes to the precipitation changes of the EASM, and it could be applied to help understand the future changes in EASM precipitation in CMIP5 simulations

Dust-wind interactions can intensify aerosol pollution over eastern China.

Eastern China has experienced severe and persistent winter haze episodes in recent years due to intensification of aerosol pollution. In addition to anthropogenic emissions, the winter aerosol pollution over eastern China is associated with unusual meteorological conditions, including weaker wind speeds. Here we show, based on model simulations, that during years with decreased wind speed, large decreases in dust emissions (29%) moderate the wintertime land-sea surface air temperature difference and further decrease winds by -0.06 (±0.05) m s-1 averaged over eastern China. The dust-induced lower winds enhance stagnation of air and account for about 13% of increasing aerosol concentrations over eastern China. Although recent increases in anthropogenic emissions are the main factor causing haze over eastern China, we conclude that natural emissions also exert a significant influence on the increases in wintertime aerosol concentrations, with important implications that need to be taken into account by air quality studies

Asian summer monsoon response to greenhouse gases and anthropogenic aerosols

The Asian monsoon-affected area is one of the most vulnerable regions in the world facing hydroclimate changes. Anthropogenic climate change, particularly the emissions of greenhouse gases (GHGs) and aerosols, exerts significant impacts on monsoon rainfall and circulation. Understanding the effects of external forcing on monsoon rainfall is essential for improving the predictability, constraining the uncertainty, and assessing the climate risks. In this dissertation, I use a combination of observations, outputs from multiple Coupled Model Intercomparison Project - Phase 5 (CMIP5) models, and idealized atmospheric general circulation model (AGCM) experiments to examine the Asian summer monsoon variability and change. The main focus is understanding the responses to GHGs and anthropogenic aerosols and their differences for both the historical period and future projections. The Asian monsoon is an interactive system influenced by multiple natural and anthropogenic factors. GHGs and aerosols induce significantly different changes in monsoon rainfall through both thermodynamical and dynamical processes. These changes can be further separated into the fast adjustments related to radiation and cloud processes and the slow response due to changes in sea surface temperature (SST). This thesis provides a detailed analysis of the multiple physical processes entangled in the total response, advancing our mechanistic understanding of the effects of external forcing on the Asian monsoon system and the associated uncertainties. In Chapter 2, I first analyze the monsoon-ENSO (El Nino - Southern Oscillation) relationship in observations and CMIP5 models to determine the role of natural variability. Separating the natural and forced components shows that natural variability plays a dominant role in the 20th century, however enhanced monsoon rainfall associated with global warming may contribute to a weakened ENSO-monsoon relation in the 21st century. In Chapter 3, I examine the physical mechanisms causing the changes of the Asian summer monsoon during the 20th and 21st century using observations and CMIP5 models, attributing the rainfall changes to the relative roles of thermodynamic and dynamic processes. CMIP5 models show a distinct drying of the Asian summer monsoon rainfall during the historical period but strong wetting for future projections, which can be explained by the strong aerosol-induced dynamical weakening during the 20th century and the thermodynamic enhancement due to GHGs in the 21st century. In Chapters 4 and 5, I further use multiple AGCMs to separate the total monsoon response into a fast adjustment component independent of the sea surface temperature (SST) responses, and a slow response component associated with SST feedbacks. For GHGs (Chapter 4), the fast and slow monsoon circulation changes largely oppose each other, leading to an overall weak response and large inter-model spread. For aerosols (Chapter 5), the strongly weakened monsoon circulation over land due to aerosols is largely driven by the fast adjustments related to aerosol-radiation and aerosol-cloud interactions. Finally in Chapter 6, I design idealized AGCM experiments with prescribed SSTs using the Community Atmosphere Model (CAM5) and the Geophysical Fluid Dynamic Laboratory Model (GFDL-AM3) to investigate the relative roles of uniform SST warming/cooling as well as global and regional SST patterns in shaping the differing monsoon responses. While GHGs-induced SST changes affect the monsoon largely via the uniform warming effect, for aerosols the SST spatial pattern plays the dominant role through changes in atmospheric circulation

Advances in understanding large-scale responses of the water cycle to climate change

Globally, thermodynamics explains an increase in atmospheric water vapor with warming of around 7%/°C near to the surface. In contrast, global precipitation and evaporation are constrained by the Earth's energy balance to increase at ∼2–3%/°C. However, this rate of increase is suppressed by rapid atmospheric adjustments in response to greenhouse gases and absorbing aerosols that directly alter the atmospheric energy budget. Rapid adjustments to forcings, cooling effects from scattering aerosol, and observational uncertainty can explain why observed global precipitation responses are currently difficult to detect but are expected to emerge and accelerate as warming increases and aerosol forcing diminishes. Precipitation increases with warming are expected to be smaller over land than ocean due to limitations on moisture convergence, exacerbated by feedbacks and affected by rapid adjustments. Thermodynamic increases in atmospheric moisture fluxes amplify wet and dry events, driving an intensification of precipitation extremes. The rate of intensification can deviate from a simple thermodynamic response due to in‐storm and larger‐scale feedback processes, while changes in large‐scale dynamics and catchment characteristics further modulate the frequency of flooding in response to precipitation increases. Changes in atmospheric circulation in response to radiative forcing and evolving surface temperature patterns are capable of dominating water cycle changes in some regions. Moreover, the direct impact of human activities on the water cycle through water abstraction, irrigation, and land use change is already a significant component of regional water cycle change and is expected to further increase in importance as water demand grows with global population

Preferred response of the East Asian summer monsoon to local and non-local anthropogenic sulphur dioxide emissions

In this study, the atmospheric component of a state-of-the-art climate model (HadGEM2-ES) that includes earth system components such as interactive chemistry and eight species of tropospheric aerosols considering aerosol direct, indirect, and semi-direct effects, has been used to investigate the impacts of local and non-local emissions of anthropogenic sulphur dioxide on the East Asian summer monsoon (EASM). The study focuses on the fast responses (including land surface feedbacks, but without sea surface temperature feedbacks) to sudden changes in emissions from Asia and Europe. The initial responses, over days 1–40, to Asian and European emissions show large differences. The response to Asian emissions involves a direct impact on the sulphate burden over Asia, with immediate consequences for the shortwave energy budget through aerosol–radiation and aerosol–cloud interactions. These changes lead to cooling of East Asia and a weakening of the EASM. In contrast, European emissions have no significant impact on the sulphate burden over Asia, but they induce mid-tropospheric cooling and drying over the European sector. Subsequently, however, this cold and dry anomaly is advected into Asia, where it induces atmospheric and surface feedbacks over Asia and the Western North Pacific (WNP), which also weaken the EASM. In spite of very different perturbations to the local aerosol burden in response to Asian and European sulphur dioxide emissions, the large scale pattern of changes in land–sea thermal contrast, atmospheric circulation and local precipitation over East Asia from days 40 onward exhibits similar structures, indicating a preferred response, and suggesting that emissions from both regions likely contributed to the observed weakening of the EASM. Cooling and drying of the troposphere over Asia, together with warming and moistening over the WNP, reduces the land–sea thermal contrast between the Asian continent and surrounding oceans. This leads to high sea level pressure (SLP) anomalies over Asia and low SLP anomalies over the WNP, associated with a weakened EASM. In response to emissions from both regions warming and moistening over the WNP plays an important role and determines the time scale of the response

Impacts of recent decadal changes in Asian aerosols on the East Asian summer monsoon: roles of aerosol–radiation and aerosol–cloud interactions

Anthropogenic aerosols (AA) can affect cloud and precipitation through aerosol–radiation interaction (ARI) and aerosol–cloud interaction (ACI). Over the past few decades, anthropogenic aerosol emissions have exhibited remarkable changes in the magnitude and in spatial pattern. The most significant changes are the increased emissions over both South Asia and East Asia. In this study, the atmospheric component of a state-of-the-art climate model that includes eight species of tropospheric aerosols, coupled to a multi-level mixed-layer ocean model, has been used to investigate the impacts of Asian anthropogenic aerosol precursor emission changes from 1970s to 2000s on large scale circulation and precipitation in boreal summer over East Asia. Results reveal significant changes in circulation and clouds over East Asia and over the tropical and western North Pacific (WNP). Increased Asian AA emissions lead to anomalous cyclonic circulation over the Maritime continent (MC) and anomalous anticyclonic circulation over the WNP, resulting in anomalous moisture transport convergence over the MC and therefore increased precipitation. They also lead to anomalous moisture flux divergence over both the WNP and large land areas of East Asia, especially over northern China, and therefore decreased precipitation there. These large scale circulation anomalies over the adjacent oceans are related to aerosol change induced ocean feedbacks, predominantly through ACI. It is the slow responses over the adjacent oceans (e.g., SST changes) through coupled atmosphere–ocean interaction in pre-monsoon seasons and summer that shape the changes of the East Asian summer monsoon and local precipitation. The results in this study suggest that increased Asian AA emissions from 1970s to 2000s may have played an important role for the observed southward shift of the Pacific intertropical convergence zone and precipitation belt, weakening of East Asian summer monsoon and reduced precipitation over northern China in East Asia during the latter half of the twentieth century

Forced decadal changes in the East Asian summer monsoon: the roles of greenhouse gases and anthropogenic aerosols

Since the mid-1990s precipitation trends over eastern China display a dipole pattern, characterized by positive anomalies in the south and negative anomalies in the north, named as the Southern-Flood-Northern-Drought (SFND) pattern. This work investigates the drivers of decadal changes of the East Asian summer monsoon (EASM), and the dynamical mechanisms involved, by using a coupled climate model (specifically an atmospheric general circulation model coupled to an ocean mixed layer model) forced by changes in (1) anthropogenic greenhouse gases (GHG), (2) anthropogenic aerosol (AA) and (3) the combined effects of both GHG and AA (All Forcing) between two periods across the mid-1990s. The model experiment forced by changes in All Forcing shows a dipole pattern of response in precipitation over China that is similar to the observed SFND pattern across the mid-1990s, which suggests that anthropogenic forcing changes played an important role in the observed decadal changes. Furthermore, the experiments with separate forcings indicate that GHG and AA forcing dominate different parts of the SFND pattern. In particular, changes in GHG increase precipitation over southern China, whilst changes in AA dominate in the drought conditions over northern China. Increases in GHG cause increased moisture transport convergence over eastern China, which leads to increased precipitation. The AA forcing changes weaken the EASM, which lead to divergent wind anomalies over northern China and reduced precipitation