A quantum photonics model for non-classical light generation using integrated nanoplasmonic cavity-emitter systems

The implementation of non-classical light sources is becoming increasingly important for various quantum applications. A particularly interesting approach is to integrate such functionalities on a single chip as this could pave the way towards fully scalable quantum photonic devices. Several approaches using dielectric systems have been investigated in the past. However, it is still not understood how on-chip nanoplasmonic antennas, interacting with a single quantum emitter, affect the quantum statistics of photons reflected or transmitted in the guided mode of a waveguide. Here we investigate a quantum photonic platform consisting of an evanescently coupled nanoplasmonic cavity-emitter system and discuss the requirements for non-classical light generation. We develop an analytical model that incorporates quenching due to the nanoplasmonic cavity to predict the quantum statistics of the transmitted and reflected guided waveguide light under weak coherent pumping. The analytical predictions match numerical simulations based on a master equation approach. It is moreover shown that for resonant excitation the degree of anti-bunching in transmission is maximized for an optimal cavity modal volume $V_{c}$ and cavity-emitter distance $s$. In reflection, perfectly anti-bunched light can only be obtained for specific $(V_{c},s)$ combinations. Finally, our model also applies to dielectric cavities and as such can guide future efforts in the design and development of on-chip non-classical light sources using dielectric and nanoplasmonic cavity-emitter systems

Visible quantum plasmonics from metallic nanodimers

We report theoretical evidence that bulk nonlinear materials weakly interacting with highly localized plasmonic modes in ultra-sub-wavelength metallic nanostructures can lead to nonlinear effects at the single plasmon level in the visible range. In particular, the two-plasmon interaction energy in such systems is numerically estimated to be comparable with the typical plasmon linewidths. Localized surface plasmons are thus predicted to exhibit a purely nonclassical behavior, which can be clearly identified by a sub-Poissonian second-order correlation in the signal scattered from the quantized plasmonic field under coherent electromagnetic excitation. We explicitly show that systems sensitive to single-plasmon scattering can be experimentally realized by combining electromagnetic confinement in the interstitial region of gold nanodimers with local infiltration or deposition of ordinary nonlinear materials. We also propose configurations that could allow to realistically detect such an effect with state-of-the-art technology, overcoming the limitations imposed by the short plasmonic lifetime

A single-photon transistor using nano-scale surface plasmons

It is well known that light quanta (photons) can interact with each other in nonlinear media, much like massive particles do, but in practice these interactions are usually very weak. Here we describe a novel approach to realize strong nonlinear interactions at the single-photon level. Our method makes use of recently demonstrated efficient coupling between individual optical emitters and tightly confined, propagating surface plasmon excitations on conducting nanowires. We show that this system can act as a nonlinear two-photon switch for incident photons propagating along the nanowire, which can be coherently controlled using quantum optical techniques. As a novel application, we discuss how the interaction can be tailored to create a single-photon transistor, where the presence or absence of a single incident photon in a ``gate'' field is sufficient to completely control the propagation of subsequent ``signal'' photons.Comment: 20 pages, 4 figure

Plasmonic Waveguides to Enhance Quantum Electrodynamic Phenomena at the Nanoscale

The emerging field of plasmonics can lead to enhanced light matter interactions at extremely nanoscale regions. Plasmonic (metallic) devices promise to efficiently control both classical and quantum properties of light. Plasmonic waveguides are usually used to excite confined electromagnetic modes at the nanoscale that can strongly interact with matter. The analysis of these nanowaveguides exhibits similarities with their low frequency microwave counterparts. In this article, we review ways to study plasmonic nanostructures coupled to quantum optical emitters from a classical electromagnetic perspective. These quantum emitters are mainly used to generate single photon quantum light that can be employed as a quantum bit or qubit in the envisioned quantum information technologies. We demonstrate different ways to enhance a diverse range of quantum electrodynamic phenomena based on plasmonic configurations by using the classical dyadic tensor Green function formalism. More specifically, spontaneous emission and superradiance are analyzed by using the Green function based field quantization. The exciting new field of quantum plasmonics will lead to a plethora of novel optical devices for communications and computing applications operating in the quantum realm, such as efficient single-photon sources, quantum sensors, and compact on-chip nanophotonic circuits

Interaction and coherence of a plasmon-exciton polariton condensate

Polaritons are quasiparticles arising from the strong coupling of electromagnetic waves in cavities and dipolar oscillations in a material medium. In this framework, localized surface plasmon in metallic nanoparticles defining optical nanocavities have attracted increasing interests in the last decade. This interest results from their sub-diffraction mode volume, which offers access to extremely high photonic densities by exploiting strong scattering cross-sections. However, high absorption losses in metals have hindered the observation of collective coherent phenomena, such as condensation. In this work we demonstrate the formation of a non-equilibrium room temperature plasmon-exciton-polariton condensate with a long range spatial coherence, extending a hundred of microns, well over the excitation area, by coupling Frenkel excitons in organic molecules to a multipolar mode in a lattice of plasmonic nanoparticles. Time-resolved experiments evidence the picosecond dynamics of the condensate and a sizeable blueshift, thus measuring for the first time the effect of polariton interactions in plasmonic cavities. Our results pave the way to the observation of room temperature superfluidity and novel nonlinear phenomena in plasmonic systems, challenging the common belief that absorption losses in metals prevent the realization of macroscopic quantum states.Comment: 23 pages, 5 figures, SI 7 pages, 5 figure

CHARACTERIZATION OF FLUORESCENCE FROM QUANTUM DOTS ON NANOSTRUCTURED METAL SURFACES

The behavior of fluorescent materials coupled to surface plasmon supporting surfaces and structures is an area of active research due to their fluorescence enhancing properties. The inherent field enhancements present near structures and interfaces where surface plasmons are excited provide great potential for increasing the response of many optical interactions. While many studies focus on the application of plasmonic nanoparticles or finite metallic structures the use of dielectric structures on a continuous metallic film has received little attention. A comprehensive experimental study using dielectric gratings on gold films is presented illustrating the fundamental properties of fluorescence enhancement on such structures. A process for fabrication of samples using Electron Beam Lithography is demonstrated and comparisons between various quantum dot deposition methods are made to determine the best conditions for surface coating. Conditions for optimization of the fluorescence enhancement phenomena for practical application are explored for gratings with square function profile illustrating the influence of gratings on fluorescence behavior and identifying conditions for optimal enhancement. Complementing these results, an understanding of the underlying physical phenomena is developed by differentiation between enhanced emission and enhanced absorption effects using measurements of fluorescence decay lifetime and emission spectra. Using these observations a thorough description of these systems and the requirements for their practical application is illustrated