11,017 research outputs found
Charge transport in nanoscale vertical organic semiconductor pillar devices
We report charge transport measurements in nanoscale vertical pillar
structures incorporating ultrathin layers of the organic semiconductor
poly(3-hexylthiophene)(P3HT). P3HT layers with thickness down to 5 nm are
gently top-contacted using wedging transfer, yielding highly reproducible,
robust nanoscale junctions carrying high current densities (up to
A/m). Current-voltage data modeling demonstrates excellent hole injection.
This work opens up the pathway towards nanoscale, ultrashort-channel organic
transistors for high-frequency and high-current-density operation.Comment: 30 pages, 8 figures, 1 tabl
Interfacial charge transfer in nanoscale polymer transistors
Interfacial charge transfer plays an essential role in establishing the
relative alignment of the metal Fermi level and the energy bands of organic
semiconductors. While the details remain elusive in many systems, this charge
transfer has been inferred in a number of photoemission experiments. We present
electronic transport measurements in very short channel ( nm)
transistors made from poly(3-hexylthiophene) (P3HT). As channel length is
reduced, the evolution of the contact resistance and the zero-gate-voltage
conductance are consistent with such charge transfer. Short channel conduction
in devices with Pt contacts is greatly enhanced compared to analogous devices
with Au contacts, consistent with charge transfer expectations. Alternating
current scanning tunneling microscopy (ACSTM) provides further evidence that
holes are transferred from Pt into P3HT, while much less charge transfer takes
place at the Au/P3HT interface.Comment: 19 preprint pages, 6 figure
Roadmap on semiconductor-cell biointerfaces.
This roadmap outlines the role semiconductor-based materials play in understanding the complex biophysical dynamics at multiple length scales, as well as the design and implementation of next-generation electronic, optoelectronic, and mechanical devices for biointerfaces. The roadmap emphasizes the advantages of semiconductor building blocks in interfacing, monitoring, and manipulating the activity of biological components, and discusses the possibility of using active semiconductor-cell interfaces for discovering new signaling processes in the biological world
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