Analysis of linear long-term trend of aerosol optical thickness derived from SeaWiFS using BAER over Europe and South China

The main purposes of the present paper are not only to investigate linear long-term trends of Aerosol Optical Thickness (AOT) at 443 and 555 nm over regions in Europe and South China, but also to show the uncertainty caused by cloud disturbance in the trend analysis of cloud-free aerosol. These research areas are the densely urbanised and often highly polluted regions. The study uses the Bremen AErosol Retrieval (BAER) and Sea-viewing Wide Field-of-view Sensor (SeaWiFS) data for AOT retrievals in the specified regions from October 1997 to May 2008. In order to validate the individually retrieved AOTs and the corresponding trends, AErosol RObotic NETwork (AERONET) level 2.0 data have been used. The retrieved AOTs were in good agreement with those of AERONET (0.79 ≤ <i>R</i> ≤ 0.88, 0.08 ≤ RMSD ≤ 0.13). The contamination of the aerosol retrievals and/or AERONET observations by thin clouds can significantly degrade the AOT and lead to statistically non-representative monthly-means, especially during cloudy seasons. Therefore an inter-correction method has been developed and applied. The "corrected" trends for both BAER SeaWiFS and AERONET AOT were similar and showed in average a relative difference of ∼25.19%. In general terms, negative trends (decrease of aerosol loading) were mainly observed over European regions, with magnitudes up to −0.00453 and −0.00484 yr<sup>−1</sup> at 443 and 555 nm, respectively. In contrast, the trend in Pearl River Delta was positive, most likely attributed to rapid urbanization and industrialization. The magnitudes of AOT increased by +0.00761 and +0.00625 yr<sup>−1</sup> respectively at 443 and 555 nm

Multi-Decadal Aerosol Variations from 1980 to 2009: A Perspective from Observations and a Global Model

Aerosol variations and trends over different land and ocean regions during 1980-2009 are analyzed with the Goddard Chemistry Aerosol Radiation and Transport (GOCART) model and observations from multiple satellite sensors and ground-based networks. Excluding time periods with large volcanic influences, the tendency of aerosol optical depth (AOD) and surface concentration over polluted land regions is consistent with the anthropogenic emission changes.The largest reduction occurs over Europe, and regions in North America and Russia also exhibit reductions. On the other hand, East Asia and South Asia show AOD increases, although relatively large amount of natural aerosols in Asia makes the total changes less directly connected to the pollutant emission trends. Over major dust source regions, model analysis indicates that the dust emissions over the Sahara and Sahel respond mainly to the near-surface wind speed, but over Central Asia they are largely influenced by ground wetness. The decreasing dust trend in the tropical North Atlantic is most closely associated with the decrease of Sahel dust emission and increase of precipitation over the tropical North Atlantic, likely driven by the sea surface temperature increase. Despite significant regional trends, the model-calculated global annual average AOD shows little changes over land and ocean in the past three decades, because opposite trends in different regions cancel each other in the global average. This highlights the need for regional-scale aerosol assessment, as the global average value conceals regional changes, and thus is not sufficient for assessing changes in aerosol loading

Global and regional trends of Aerosol Optical Thickness derived using satellite- and ground-based observations

Atmospheric aerosol plays a critical role for human health, air quality, long range transport of pollution, and the Earth s radiative balance, thereby influencing global climate change. To test our scientific understanding and provide an evidence base for policymakers, long-term temporal changes of local, regional, and global aerosols are needed. Remote sensing from satellite borne and ground based observations offers unique opportunities to provide such data. However, only a few studies have discussed the limitations, associated with unrepresentative sampling originating from large/persistent cloud disturbance and limited/different sampling (limited orbital periods and different sampling times) in the trend analysis. Using a linear weighted model, the long-term trends of global AOTs from various polar orbiting satellites and ground observations: MODIS (aboard Terra), MISR (Terra), SeaWiFS (OrbView-2), MODIS (Aqua), and AERONET have been analyzed. In this manner, the present study attempts to minimize the influence of unrepresentative sampling in the trend analysis. Throughout terrestrial and marine regions, temporal increase of cloud-free AOTs were dominat over the globe (GL), northern (NH), and southern hemisphere (SH) (up to 0.00348±0.00185 for GL, 0.00514±0.00272 for NH, and 0.00232±0.00124 per year for SH). Generally, consistently in all observations, the weighted trends over Eastern US and OECD Europe showed a strong decreasing AOT (up to -0.00376±0.00174 for Eastern US and -0.00530±0.00304 per year for OECD Europe) attributed to the recent environmental legislation and resulting regulation of emissions. A significant increase was observed over Saharan/Arabian deserts, South, and East Asia (up to 0.00618±0.00326, 0.01452±0.00615, and 0.01939±0.00986 per year, respectively). These in part dramatic increases are caused by the enhanced amount of aerosol transported/emitted from industrialization, urbanization, deforestation, desertification, and climate change. Overall large/persistent cloud disturbance all year round and the limited/different sampling of polar orbiting satellites represent a challenge, which has been addressed successfully in this study for the accurate determination of aerosol amount and its trends

Merging regional and global aerosol optical depth records from major available satellite products

Satellite instruments provide a vantage point for studying aerosol loading consistently over different regions of the world. However, the typical lifetime of a single satellite platform is on the order of 5-15 years; thus, for climate studies, the use of multiple satellite sensors should be considered. Discrepancies exist between aerosol optical depth (AOD) products due to differences in their information content, spatial and temporal sampling, calibration, cloud masking, and algorithmic assumptions. Users of satellite-based AOD time-series are confronted with the challenge of choosing an appropriate dataset for the intended application. In this study, 16 monthly AOD products obtained from different satellite sensors and with different algorithms were inter-compared and evaluated against Aerosol Robotic Network (AERONET) monthly AOD. Global and regional analyses indicate that products tend to agree qualitatively on the annual, seasonal and monthly timescales but may be offset in magnitude. Several approaches were then investigated to merge the AOD records from different satellites and create an optimised AOD dataset. With few exceptions, all merging approaches lead to similar results, indicating the robustness and stability of the merged AOD products. We introduce a gridded monthly AOD merged product for the period 1995-2017. We show that the quality of the merged product is as least as good as that of individual products. Optimal agreement of the AOD merged product with AERONET further demonstrates the advantage of merging multiple products. This merged dataset provides a long-term perspective on AOD changes over different regions of the world, and users are encouraged to use this dataset

Global aeolian dust variations and trends: a revisit of dust event and visibility observations from surface weather stations

This study revisits the use of horizontal visibility and manually reported present weather (ww) records from the NOAA Integrated Surface Database (ISD) for characterizing the aeolian dust variability and recent trends over the globe and three largest source regions (North Africa, Middle East, and East Asia). Due to its qualitative nature, ww is combined with visibility to derive a new variable, VI, which has higher correlations with the dust emission and burden from satellite observations and global aerosol reanalyses than does the dust event frequency (FR) derived from ww only. Both FR and VI capture the intensive dust activity associated with the prolonged North American drought during the 1950s and Sahelian drought during the 1980s. Correlation analysis suggests soil moisture has a lagged effect on the global dustiness, with a maximum r = −0.3 when soil moisture leads VI by 14 months. Through a critical assessment of the ww continuity and ww-visibility consistency of various report types in ISD, the SYNOP data are used for global dust trend detection from 1986 to 2019. Globally, FR and VI decreased at a rate of −0.23 % yr−1 and −8.0 × 10−4 km−1 yr−1, respectively, from 1986 to 1996/1997 when dust reached a minimum, followed by a slower rebound at a rate of 0.085 % yr−1 and 1.9 × 10−4 km−1 yr−1, respectively. The nonlinear behavior of global dustiness is qualitatively consistent with satellite observations and global aerosol reanalyses. Regionally, North Africa experienced increased dust activity during the past decade after staying below average for most of the 1990s–2000s, in response to reduced soil moisture and increased wind speed following the transition of North Atlantic Oscillation (NAO) from strong negative to recurring positive phases since 2011. In the Middle East, dust has been increasing since 1998 due to a prolonged drought in the Tigris-Euphrates basin associated with strong negative Pacific Decadal Oscillation (PDO) phases. As PDO turned positive and weak negative after 2015, the amelioration of drought has led to decreased dust activity in recent years. The dust variability in East Asia is primarily driven by wind speed, which explains the dust decline from 1986 to 1997, and the absence of dust trends during the past two decades. This study constitutes an initial effort of creating a homogenized weather station-based dust-climate dataset in support of wind erosion monitoring, dust source mapping, and dust-climate analysis at local to global scales

Reducing the Uncertainties in Direct Aerosol Radiative Forcing

Airborne particles, which include desert and soil dust, wildfire smoke, sea salt, volcanic ash, black carbon, natural and anthropogenic sulfate, nitrate, and organic aerosol, affect Earth's climate, in part by reflecting and absorbing sunlight. This paper reviews current status, and evaluates future prospects for reducing the uncertainty aerosols contribute to the energy budget of Earth, which at present represents a leading factor limiting the quality of climate predictions. Information from satellites is critical for this work, because they provide frequent, global coverage of the diverse and variable atmospheric aerosol load. Both aerosol amount and type must be determined. Satellites are very close to measuring aerosol amount at the level-of-accuracy needed, but aerosol type, especially how bright the airborne particles are, cannot be constrained adequately by current techniques. However, satellite instruments can map out aerosol air mass type, which is a qualitative classification rather than a quantitative measurement, and targeted suborbital measurements can provide the required particle property detail. So combining satellite and suborbital measurements, and then using this combination to constrain climate models, will produce a major advance in climate prediction

Spatial distribution of dust's optical properties over the Sahara and Asia inferred from Moderate Resolution Imaging Spectroradiometer

There is great uncertainty regarding the role of mineral dust aerosols in Earth’s climate system. One reason for this uncertainty is that the optical properties of mineral dust, such as its single scattering albedo (the ratio of scattering to total extinction), are poorly constrained because ground observations are limited to a few locations and satellite standard products are not available due to the excessively bright surface of the desert in the visible wavelength, which makes robust retrievals difficult. Here, we develop a method to estimate the spatial distributions of the aerosol single scattering albedo (ω0) and optical depth (τa), with daily 1◦ × 1 ◦ spatial resolution using data from the Moderate Resolution Imaging Spectroradiometer (MODIS) as well as model simulations of radiative transfer. This approach is based on the “critical surface reflectance” method developed in the literature, which estimates ω0 from the top of the atmospheric radiance. We estimate the uncertainties in ω0 over the Sahara (Asia) to be approximately 0.020 and 0.010 (0.023 and 0.017) for bands 9 and 1, respectively, while the uncertainty in τa is approximately 0.235 and 0.228 (0.464 and 0.370) for bands 9 and 1, respectively. The 5–95 % range of the spatial distribution of ω0 over the Sahara (Asia) is approximately 0.90–0.94 and 0.96–0.99 (0.87–0.94 and 0.89–0.97) for bands 9 and 1, respectively, and that of τa over the Sahara (Asia) is approximately 0.8–1.4 and 0.8–1.7 (0.7–2.0 and 0.7–1.9) for bands 9 and 1, respectively. The results for the Sahara indicate a good correlation between ω0 and the surface reflectance, and between ω0 and τa. However, the relationships between ω0, τa, and surface reflectance are less clear in Asia than in the Sahara, and the ω0 values are smaller than those in the Sahara. The regions with small ω0 values are consistent with the regions where coal-burning smoke and carbonaceous aerosols are reported to be transported in previous studies. Because the coal-burning and carbonaceous aerosols are known to be more absorptive and have smaller ω0 values than dust aerosols, our results indicate that the dust aerosols in Asia are contaminated by these anthropogenic aerosols. The spatial distribution of dust optical properties obtained in our work could be useful in understanding the role of dust aerosols in Earth’s climate system, most likely through future collaboration with regional and global modelling studies.The authors are grateful to the Open CLASTER project for allowing us to use the RSTAR package for this research. We would like to thank the AERONET project and its staff for establishing and maintaining the Tamanrasset, Agoufou, Banizoumbou and Saada sites considered in this investigation. We would also like to thank the SKYNET project and its staff for establishing and maintaining the Dunhuang site. Finally, we appreciate the valuable discussions and support provided by Ben Johnson, Satoru Fukuda, Yosuke Sato, Eiji Oikawa, Makiko Hashimoto, Yasushi Mitomi and Matthew Collins. One of the authors was supported by projects by JAXA/EarthCARE and GCOM/C, MEXT/VL for Climate System Diagnostics, MOE/Global Environment Research Fund A-1101, NIES/GOSAT, and MEXT/RECCA/SALSA

Melting of Major Glaciers in Himalayas: Role of Desert Dust and Anthropogenic Aerosols

The Himalayan and Tibet Glaciers, that are among the largest bodies of ice and fresh water resource outside of the polar ice caps, face a significant threat of accelerated meltdown in coming decades due to climate variability and change. The rate of retreat of these glaciers and changes in their terminus (frontal dynamics) is highly variable across the Himalayan range. These large freshwater sources are critical to human activities for food production, human consumption and a whole host of other applications, especially over the Indo-Gangetic (IG) plains. They are also situated in a geo-politically sensitive area surrounded by China, India, Pakistan, Nepal and Bhutan where more than a billion people depend on them. The major rivers of the Asian continent such as the Ganga (also known as Ganges), Brahmaputra, Indus, Yamuna, Sutluj etc., originate and pass through these regions and they have greater importance due to their multi-use downstream: hydro power, agriculture, aquaculture, flood control, and as a freshwater resource. Recent studies over the Himalayan Glaciers using ground-based and space-based observations, and computer models indicate a long-term trend of climate variability and change that may accelerate melting of the Himalayan Glaciers.https://digitalcommons.chapman.edu/sees_books/1001/thumbnail.jp