Time Minimal Trajectories for a Spin 1/2 Particle in a Magnetic Field

In this paper we consider the minimum time population transfer problem for the $z$-component of the spin of a (spin 1/2) particle driven by a magnetic field, controlled along the x axis, with bounded amplitude. On the Bloch sphere (i.e. after a suitable Hopf projection), this problem can be attacked with techniques of optimal syntheses on 2-D manifolds. Let $(-E,E)$ be the two energy levels, and $|\Omega(t)|\leq M$ the bound on the field amplitude. For each couple of values $E$ and $M$, we determine the time optimal synthesis starting from the level $-E$ and we provide the explicit expression of the time optimal trajectories steering the state one to the state two, in terms of a parameter that can be computed solving numerically a suitable equation. For $M/E<<1$, every time optimal trajectory is bang-bang and in particular the corresponding control is periodic with frequency of the order of the resonance frequency $\omega_R=2E$. On the other side, for $M/E>1$, the time optimal trajectory steering the state one to the state two is bang-bang with exactly one switching. Fixed $E$ we also prove that for $M\to\infty$ the time needed to reach the state two tends to zero. In the case $M/E>1$ there are time optimal trajectories containing a singular arc. Finally we compare these results with some known results of Khaneja, Brockett and Glaser and with those obtained by controlling the magnetic field both on the $x$ and $y$ directions (or with one external field, but in the rotating wave approximation). As byproduct we prove that the qualitative shape of the time optimal synthesis presents different patterns, that cyclically alternate as $M/E\to0$, giving a partial proof of a conjecture formulated in a previous paper.Comment: 31 pages, 10 figures, typos correcte

Geometric optimal control of the contrast imaging problem in Nuclear Magnetic Resonance

The objective of this article is to introduce the tools to analyze the contrast imaging problem in Nuclear Magnetic Resonance. Optimal trajectories can be selected among extremal solutions of the Pontryagin Maximum Principle applied to this Mayer type optimal problem. Such trajectories are associated to the question of extremizing the transfer time. Hence the optimal problem is reduced to the analysis of the Hamiltonian dynamics related to singular extremals and their optimality status. This is illustrated by using the examples of cerebrospinal fluid / water and grey / white matter of cerebrum.Comment: 30 pages, 13 figur

Optimisation of Quantum Trajectories Driven by Strong-field Waveforms

Quasi-free field-driven electron trajectories are a key element of strong-field dynamics. Upon recollision with the parent ion, the energy transferred from the field to the electron may be released as attosecond duration XUV emission in the process of high harmonic generation (HHG). The conventional sinusoidal driver fields set limitations on the maximum value of this energy transfer, and it has been predicted that this limit can be significantly exceeded by an appropriately ramped-up cycleshape. Here, we present an experimental realization of such cycle-shaped waveforms and demonstrate control of the HHG process on the single-atom quantum level via attosecond steering of the electron trajectories. With our optimized optical cycles, we boost the field-ionization launching the electron trajectories, increase the subsequent field-to-electron energy transfer, and reduce the trajectory duration. We demonstrate, in realistic experimental conditions, two orders of magnitude enhancement of the generated XUV flux together with an increased spectral cutoff. This application, which is only one example of what can be achieved with cycle-shaped high-field light-waves, has farreaching implications for attosecond spectroscopy and molecular self-probing