232,002 research outputs found

    Water activity in lamellar stacks of lipid bilayers: "Hydration forces" revisited

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    Water activity and its relationship with interactions stabilising lamellar stacks of mixed lipid bilayers in their fluid state are investigated by means of osmotic pressure measurements coupled with small-angle x-ray scattering. The (electrically-neutral) bilayers are composed of a mixture in various proportions of lecithin, a zwitterionic phospholipid, and Simulsol, a non-ionic cosurfactant with an ethoxylated polar head. For highly dehydrated samples the osmotic pressure profile always exhibits the "classical" exponential decay as hydration increases but, depending on Simulsol to lecithin ratio, it becomes either of the "bound" or "unbound" types for more water-swollen systems. A simple thermodynamic model is used for interpreting the results without resorting to the celebrated but elusive "hydration forces"Comment: 24 pages, 12 figures. Accepted for publication in The European Physical Journal

    Quantitative scattering theory of near-field response for 1D polaritonic structures

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    Scattering-type scanning near-field optical microscopy is a powerful imaging technique for studying materials beyond the diffraction limit. However, interpreting near-field measurements poses challenges in mapping the response of polaritonic structures to meaningful physical properties. To address this, we propose a theory based on the transfer matrix method to simulate the near-field response of 1D polaritonic structures. Our approach provides a computationally efficient and accurate analytical theory, relating the near-field response to well-defined physical properties. This work enhances the understanding of near-field images and complex polaritonic phenomena. Finally, this scattering theory can extend to other systems like atoms or nanoparticles near a waveguide

    Supramolecular Engineering of Alkylated, Fluorinated, and Mixed Amphiphiles

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    The rational design of perfluorinated amphiphiles to control the supramolecular aggregation in an aqueous medium is still a key challenge for the engineering of supramolecular architectures. Here, the synthesis and physical properties of six novel non-ionic amphiphiles are presented. The effect of mixed alkylated and perfluorinated segments in a single amphiphile is also studied and compared with only alkylated and perfluorinated units. To explore their morphological behavior in an aqueous medium, dynamic light scattering (DLS) and cryogenic transmission electron microscopy/electron microscopy (cryo-TEM/EM) measurements are used. The assembly mechanisms with theoretical investigations are further confirmed, using the Martini model to perform large-scale coarse-grained molecular dynamics simulations. These novel synthesized amphiphiles offer a greater and more systematic understanding of how perfluorinated systems assemble in an aqueous medium and suggest new directions for rational designing of new amphiphilic systems and interpreting their assembly process

    Using think-aloud interviews to characterize model-based reasoning in electronics for a laboratory course assessment

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    Models of physical systems are used to explain and predict experimental results and observations. The Modeling Framework for Experimental Physics describes the process by which physicists revise their models to account for the newly acquired observations, or change their apparatus to better represent their models when they encounter discrepancies between actual and expected behavior of a system. While modeling is a nationally recognized learning outcome for undergraduate physics lab courses, no assessments of students' model-based reasoning exist for upper-division labs. As part of a larger effort to create two assessments of students' modeling abilities, we used the Modeling Framework to develop and code think-aloud problem-solving activities centered on investigating an inverting amplifier circuit. This study is the second phase of a multiphase assessment instrument development process. Here, we focus on characterizing the range of modeling pathways students employ while interpreting the output signal of a circuit functioning far outside its recommended operation range. We end by discussing four outcomes of this work: (1) Students engaged in all modeling subtasks, and they spent the most time making measurements, making comparisons, and enacting revisions; (2) Each subtask occurred in close temporal proximity to all over subtasks; (3) Sometimes, students propose causes that do not follow logically from observed discrepancies; (4) Similarly, students often rely on their experiential knowledge and enact revisions that do not follow logically from articulated proposed causes.Comment: 18 pages, 5 figure

    Andreev bound states versus Majorana bound states in quantum dot-nanowire-superconductor hybrid structures: Trivial versus topological zero-bias conductance peaks

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    Motivated by an important recent experiment [Deng et al., Science 354, 1557 (2016)], we theoretically consider the interplay between Andreev bound states(ABSs) and Majorana bound states(MBSs) in quantum dot-nanowire semiconductor systems with proximity-induced superconductivity(SC), spin-orbit coupling and Zeeman splitting. The dot induces ABSs in the SC nanowire which show complex behavior as a function of Zeeman splitting and chemical potential, and the specific question is whether two such ABSs can come together forming a topological MBS. We consider physical situations involving the dot being non-SC, SC, or partially SC. We find that the ABSs indeed tend to coalesce together producing near-zero-energy midgap states as Zeeman splitting and/or chemical potential are increased, but this mostly happens in the non-topological regime although there are situations where the ABSs could come together forming a topological MBS. The two scenarios(two ABSs forming a near-zero-energy non-topological ABS or a zero-energy topological MBS) are difficult to distinguish by tunneling conductance spectroscopy due to essentially the same signatures. Theoretically we distinguish them by knowing the critical Zeeman splitting for the topological quantum phase transition or by calculating the topological visibility. We find that the "sticking together" propensity of ABSs to produce a zero-energy midgap state is generic in class D systems, and by itself says nothing about the topological nature of the underlying SC nanowire. One must use caution in interpreting tunneling conductance measurements where the midgap sticking-together behavior of ABSs cannot be construed as definitive evidence for topological SC with non-Abelian MBSs. We also suggest some experimental techniques for distinguishing between trivial and topological ZBCPs.Comment: 32 pages, 29 figure
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