19,151 research outputs found
Probing the inter-layer exciton physics in a MoS/MoSe/MoS van der Waals heterostructure
Stacking atomic monolayers of semiconducting transition metal dichalcogenides
(TMDs) has emerged as an effective way to engineer their properties. In
principle, the staggered band alignment of TMD heterostructures should result
in the formation of inter-layer excitons with long lifetimes and robust valley
polarization. However, these features have been observed simultaneously only in
MoSe/WSe heterostructures. Here we report on the observation of long
lived inter-layer exciton emission in a MoS/MoSe/MoS trilayer van
der Waals heterostructure. The inter-layer nature of the observed transition is
confirmed by photoluminescence spectroscopy, as well as by analyzing the
temporal, excitation power and temperature dependence of the inter-layer
emission peak. The observed complex photoluminescence dynamics suggests the
presence of quasi-degenerate momentum-direct and momentum-indirect bandgaps. We
show that circularly polarized optical pumping results in long lived valley
polarization of inter-layer exciton. Intriguingly, the inter-layer exciton
photoluminescence has helicity opposite to the excitation. Our results show
that through a careful choice of the TMDs forming the van der Waals
heterostructure it is possible to control the circular polarization of the
inter-layer exciton emission.Comment: 19 pages, 3 figures. Just accepted for publication in Nano Letters
(http://pubs.acs.org/doi/10.1021/acs.nanolett.7b03184
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Airborne measurement of inorganic ionic components of fine aerosol particles using the particle-into-liquid sampler coupled to ion chromatography technique during ACE-Asia and TRACE-P
Quantum-fluid dynamics of microcavity polaritons
Semiconductor microcavities offer a unique system to investigate the physics
of weakly interacting bosons. Their elementary excitations, polaritons--a
mixture of excitons and photons--behave, in the low density limit, as bosons
that can undergo a phase transition to a regime characterised by long range
coherence. Condensates of polaritons have been advocated as candidates for
superfluidity; and the formation of vortices as well as elementary excitations
with a linear dispersion are actively sought after. In this work, we have
created and set in motion a macroscopically degenerate state of polaritons and
let it collide with a variety of defects present in the sample. Our experiments
show striking manifestations of a coherent light-matter packet that displays
features of a superfluid, although one of a highly unusual character as it
involves an out-of-equilibrium dissipative system where it travels at
ultra-fast velocity of the order of 1% the speed of light. Our main results are
the observation of i) a linear polariton dispersion accompanied with
diffusion-less motion, ii) flow without resistance when crossing an obstacle,
iii) suppression of Rayleigh scattering and iv) splitting into two fluids when
the size of the obstacle is comparable with the size of the wavepacket. This
work opens the way to the investigation of new phenomenology of
out-of-equilibrium condensates.Comment: 22 pages, 5 figure
On the cavity method for decimated random constraint satisfaction problems and the analysis of belief propagation guided decimation algorithms
We introduce a version of the cavity method for diluted mean-field spin
models that allows the computation of thermodynamic quantities similar to the
Franz-Parisi quenched potential in sparse random graph models. This method is
developed in the particular case of partially decimated random constraint
satisfaction problems. This allows to develop a theoretical understanding of a
class of algorithms for solving constraint satisfaction problems, in which
elementary degrees of freedom are sequentially assigned according to the
results of a message passing procedure (belief-propagation). We confront this
theoretical analysis to the results of extensive numerical simulations.Comment: 32 pages, 24 figure
Nanoparticle enhanced evaporation of liquids: A case study of silicone oil and water
Evaporation is a fundamental physical phenomenon, of which many challenging
questions remain unanswered. Enhanced evaporation of liquids in some occasions
is of enormous practical significance. Here we report the enhanced evaporation
of the nearly permanently stable silicone oil by dispersing with nanopariticles
including CaTiO3, anatase and rutile TiO2. The results can inspire the research
of atomistic mechanism for nanoparticle enhanced evaporation and exploration of
evaporation control techniques for treatment of oil pollution and restoration
of dirty water
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