Radio frequency and terahertz signals generated by passively mode-locked semiconductor lasers

There are several different approaches to generating periodic signals using semiconductor lasers, for example: Q-switching, gain switching or mode-locking schemes. In general the active or passive mode-locking techniques require the use of a modulator or a saturable absorber in order to achieve the phase synchronisation. The laser diodes studied in this thesis, are demonstrated to operate in the mode-locked regime, while not requiring any direct or external modulation, nor the saturable absorbtion element in order to achieve the phase synchronisation. It has been demonstrated previously, that in a multimode semiconductor laser, the third order nonlinearities of a gain medium resulting in the four-wave-mixing effects, are responsible for the phase synchronisation and lead to phase locking. The repetition rate of the generated signal is fixed by the free-spectral range of the longitudinal spectrum. Therefore, with a passively mode-locked laser (PMLL) it is possible to cover a wide range of frequencies from the Radio-Frequency (RF) to the TeraHertz (THz) domain. Radio frequency signals generated by semiconductor lasers have many applications in optical communications, such as radio-over-fibre, or all-optical clock extraction. Terahertz signals are the focus of many research bodies nowadays, due to their interaction with matter. They have potential applications in areas like: industry, pharmacy, security (military), telecommunication and medicine. With continuous improvement of materials processing and technology, new ways of generation and detection of such types of signals have appeared. The key advantage of the optical RF or THz generation is that this type of device is direct current biased and operates at room temperature. In this thesis, a comprehensive study of various PMLLs, from distributed Bragg reflector bulk laser to quantum dashed Fabry-Perot lasers is given, demonstrating the origin of the phase synchronisation in these structures and some applications for these lasers such as all-optical clock recovery or THz signal generation

Nonlinear polarization effects in optical fibers: polarization attraction and modulation instability [Invited]

We review polarization stabilization techniques based on the polarization attraction effect in low-birefringence fibers. Polarization attraction or pulling may be based on cross-polarization modulation, on parametric amplification, and on Raman or Brillouin scattering. We also review methods for laser frequency conversion based on polarization modulation instabilities in low- and high-birefringence fibers, and photonic crystal fibers. Polarization instabilities in nonlinear fibers may also be exploited for sensing applications

Strategies for pushing nonlinear microscopy towards its performance limits

The requirement for imaging living structures with higher contrast and resolution has been covered by the inherent advantages offered by nonlinear microscopy (NLM). However, to achieve its full potential there are still several issues that must be addressed. To do so, it is very important to identify and adapt the key elements in a NLM for achieving an optimized interaction among them. These are 1) the laser source 2) the optics and 3) the sample properties for contrast generation. In this thesis, three strategies have been developed for pushing NLM towards its limits based on the light sample interaction optimization. In the first strategy it is experimentally demonstrated how to take advantage of the sample optical properties to generate label-free contrast, eliminating the requirement of modifying the sample either chemically or genetically. This is carried out by implementing third harmonic generation (THG) microscopy. Here, it is shown how the selection of the ultra-short pulsed laser (USPL) operating wavelength (1550 nm) is crucial for generating a signal that matches the peak sensitivity of most commercial detectors. This enables reducing up to seven times the light dose applied to a sample while generating an efficient signal without the requirement of amplification schemes and specialized optics (such as the need of ultraviolet grade). To show the applicability of the technique, a full developmental study of in vivo Caenorhabditis elegans embryos is presented together with the observation of wavelength induced effects. The obtained results demonstrate the potential of the technique at the employed particular wavelength to be used to follow morphogenesis processes in vivo. In the second strategy the limits of NLM are pushed by using a compact, affordable and maintenance free USPL sources. Such device was designed especially for two-photon excited fluorescence (TPEF) imaging of one the most widely used fluorescent markers in bio-imaging research: the green fluorescent protein. The system operating parameters and its emission wavelength enables to demonstrate how matching the employed fluorescent marker two-photon action cross-section is crucial for efficient TPEF signal production at very low powers. This enables relaxing the peak power conditions (40 W) to excite the sample. The enhanced versatility of this strategy is demonstrated by imaging both fixed and in vivo samples containing different dyes. More over the use of this laser is employed to produce second harmonic generation images of different samples. Several applications that can benefit by using such device are outlined. Then a comparison of the employed USPL source is performed versus the Titanium sapphire laser (the most used excitation source in research laboratories). The final goal of this strategy is to continue introducing novel laser devices for future portable NLM applications. In this case, the use of chip-sized semiconductor USPL sources for TPEF imaging is demonstrated. This will allow taking NLM technology towards the sample and make it available for any user. In the last strategy, the light interaction with the optical elements of a NLM workstation and the sample were optimized. The first enhancement was carried out in the laser-microscope optical path using an adaptive element to spatially shape the properties of the incoming beam wavefront. For an efficient light-sample interaction, aberrations caused by the index mismatch between the objective, immersion fluid, cover-glass and the sample were measured. To do so the nonlinear guide-star concept, developed in this thesis, was employed for such task. The correction of optical aberrations in all the NLM workstation enable in some cases to have an improvement of more than one order of magnitude in the total collected signal intensity. The obtained results demonstrate how adapting the interaction among the key elements of a NLM workstation enables pushing it towards its performance limits.La creciente necesidad de observar estructuras complicadas cada vez con mayor contraste y resolución han sido cubiertas por las ventajas inherentes que ofrece la microscopia nolineal. Sin embargo, aun hay ciertos aspectos que deben ser ajustados para obtener su máximo desempeño. Para ello es importante identificar y adaptar los elementos clave que forman un microscopio optimizar la interacción entre estos. Dichos elementos son: 1) el laser, 2) la óptica y 3) las propiedades de la muestra. En esta tesis, se realizan tres estrategias para llevar la eficiencia de la microscopia nolineal hacia sus límites. En la primera estrategia se demuestra de forma experimental como obtener ventaja de las propiedades ópticas de la muestra para generar contraste sin el uso de marcadores mediante la generación de tercer harmónico. Aquí se muestra como la selección de la longitud de onda del láser de pulsos ultracortos es crucial para que la señal obtenida concuerde con la máxima sensibilidad del detector utilizado. Esto permite una reducción de la dosis de luz con la que se expone la muestra, elimina intrínsecamente el requerimiento de esquemas de amplificación de señal y de óptica de tipo ultravioleta (generalmente empleada en este tipo de microscopios). Mediante un estudio comparativo con un sistema convencional se demuestra que los niveles de potencia óptica pueden ser reducidos hasta siete veces. Para demostrar las ventajas de dicha técnica se realiza un estudio completo sobre el desarrollo embrionario de Caenorhabditis elegans y los efectos causados por la exposición de la muestra a dicha longitud de onda. Los resultados demuestran el potencial de la técnica para dar seguimiento a procesos morfogénicos en muestras vivas a la longitud de onda utilizada. En la segunda estrategia se diseñó una fuente de pulsos ultracortos que es compacta, de costo reducido y libre de mantenimiento para excitar mediante la absorción de dos fotones uno de los marcadores más utilizados en el entorno biológico, la proteína verde fluorescente. Los parámetros de operación en conjunto con la longitud de onda emitida por el sistema proporcionan la máxima eficiencia permitiendo el uso de potencias pico muy bajas (40 W), ideales para relajar la exposición de la muestra. La versatilidad de esta estrategia se demuestra empleando muestras fijas y vivas con diferentes marcadores fluorescentes. Este láser también es empleado para la obtención de señal de segundo harmónico en diferentes muestras. Adicionalmente, se llevó a cabo un estudio comparativo entre la fuente desarrollada y un sistema Titanio zafiro (uno de los láseres más utilizados en laboratorios de investigación). El objetivo final de esta estrategia es introducir fuentes novedosas para aplicaciones portátiles basadas en procesos nolineales. En base a esto se demuestra el uso de dispositivos construidos sobre un microchip para generar imágenes de fluorescencia de dos fotones. Esto permitirá llevar la tecnología hacia la muestra biológica y hacerla disponible para cualquier usuario. En la última estrategia se optimiza de la interacción de la luz con los elementos ópticos del microscopio y la muestra. La primera optimización se lleva a cabo en la trayectoria óptica que lleva el láser hacia el microscopio empleando un elemento adaptable que modifica las propiedades espaciales de la luz. Para mejorar la interacción de la luz y la muestra se miden las aberraciones causadas por la diferencia de índices refractivos entre el objetivo, el medio de inmersión y la muestra. Esto se realizo empleando el concepto de la “estrella guía nolineal” desarrollado en esta tesis. Mediante la corrección de las aberraciones en el sistema de microscopia nolineal se obtiene una mejora, en algunos casos de un orden de magnitud, en la intensidad total medida. Los resultados obtenidos en esta tesis demuestran como el adaptar la interacción entre los elementos clave en un microscopio nolineal permiten llevar su desempeño hacia los límites.Postprint (published version

Stable Optical Frequency Comb Generation And Applications In Arbitrary Waveform Generation, Signal Processing And Optical Data M

This thesis focuses on the generation and applications of stable optical frequency combs. Optical frequency combs are defined as equally spaced optical frequencies with a fixed phase relation among themselves. The conventional source of optical frequency combs is the optical spectrum of the modelocked lasers. In this work, we investigated alternative methods for optical comb generation, such as dual sine wave phase modulation, which is more practical and cost effective compared to modelocked lasers stabilized to a reference. Incorporating these comblines, we have generated tunable RF tones using the serrodyne technique. The tuning range was ±1 MHz, limited by the electronic waveform generator, and the RF carrier frequency is limited by the bandwidth of the photodetector. Similarly, using parabolic phase modulation together with time division multiplexing, RF chirp extension has been realized. Another application of the optical frequency combs studied in this thesis is real time data mining in a bit stream. A novel optoelectronic logic gate has been developed for this application and used to detect an 8 bit long target pattern. Also another approach based on orthogonal Hadamard codes have been proposed and explained in detail. Also novel intracavity modulation schemes have been investigated and applied for various applications such as a) improving rational harmonic modelocking for repetition rate multiplication and pulse to pulse amplitude equalization, b) frequency skewed pulse generation for ranging and c) intracavity active phase modulation in amplitude modulated modelocked lasers for supermode noise spur suppression and integrated jitter reduction. The thesis concludes with comments on the future work and next steps to improve some of the results presented in this work

Nano-optical studies of superconducting nanowire single-photon detectors

uperconducting single-photon detectors based on superconducting nanowires offer broadband single-photon sensitivity, from visible to mid-infrared wavelengths. They have attracted particular attention due to their promising performance at telecommunications wavelengths. The additional benefits of superconducting nanowire single-photon detectors (SNSPDs) include low dark count rates (Hz) and low timing jitter (sub 100 ps). SNSPDs have been employed in practical photon-counting applications such as quantum key distribution (QKD), operation of quantum waveguide circuits and quantum emitter characterisation. Major challenges in the development of SNSPDs are the improvement of device uniformity and achieving efficient optical coupling. Nano-optical techniques such as confocal microscopy can be used to image localised areas of SNSPDs providing a direct measurement of the device uniformity. The work in this thesis describes both initial nano-optical testing at visible wavelengths in liquid helium and the construction of a fibre based miniature confocal microscope configuration operating at telecommunications wavelengths for use in a closed cycle refrigerator. In both cases localised areas of SNSPDs can be studied whilst maintaining efficient optical coupling. The miniature confocal microscope configuration has sub-nanometre position resolution over a 30 μm x 30 μm area by way of a piezoelectric X-Y scanner. A full width at half maximum (FWHM) optical resolution of 1305 nm at a wavelength of 1550 nm is achieved. SNSPDs based upon niobium nitride (NbN) nanowires fabricated on magnesium oxide (MgO) have been studied. The microscope system has allowed us to map the temporal response (timing jitter and output pulse timing delay) of constricted (non-uniform) SNSPDs. By fitting to a theoretical model, the variations in output pulse timing delay have been shown to be caused by variations in hotspot resistances across the device. This observation has provided insights into the underlying physics of SNSPDs and especially the origins of timing jitter in SNSPDs. This provides a pathway to exploitation of this effect in next-generation device designs for applications such as imaging

1.55 μm integrated modelocked semiconductor lasers

This thesis presents research on, and the realization of compact InP/InGaAsP integrated passively modelocked lasers (MLL) operating in the 1.55 µm wavelength range. The goal of this work was to obtain modelocked laser designs at a repetition rate of several tens of GHz that can be integrated with other devices on a single semiconductor wafer. These modelocked lasers should be usable as optical pulse sources in an all-optical clock recovery application in optical time domain multiplexing (OTDM) systems. The integration of the modelocked laser on a single chip is achieved using the active-passive integration technique. This technique allows one to integrate active components such as optical amplifiers and saturable absorbers, with passive components such as waveguides and optical power splitters. The modelocking mechanism of the integrated lasers is passive modelocking using a slow saturable absorber. The saturable absorber is a short optical amplifier section that is reversely biased. The work was largely concentrated on ring laser type cavities. Such a configuration has many advantages. Firstly it allows one to fix the repetition rate of the laser by photolithography. It also provides better performance thanks to the two counter-propagating pulses which collide in the saturable absorber. Finally the output of the laser can be directly interconnected on the same wafer with other devices such as an all-optical switch or a pulse compressor. From the first realization of integrated ring modelocked lasers (RMLLs) using active-passive integration and a demonstration of a device at 27 GHz, many issues came up and have been addressed in this thesis. First, the understanding of the modelocking mechanism and other dynamics needed to be better understood. To address this issue, a simulation tool of RMLL was developed. Simulation results showed that symmetrical cavities show a much wider operating range for stable modelocking. The transitions from a modelocked state of the laser to another operating regime have been explored with the model. The simulation tool requires parameters describing the gain properties of the material. These have been accurately measured using a new type of high resolution spectrum analyzer. Another important issue which came out from the first RMLL realization was the necessity to reduce all the reflections inside the modelocked laser cavity and in particular the reflections at the active-passive interfaces. Special efforts have therefore been made to characterize the optical losses and reflections at those interfaces and to minimize them to a sufficiently low value of less than -50 dB. To validate techniques of fabrication and materials required to achieve high repetition rate RMLL designs, the realization of more compact devices through the use of deep etching has been investigated in this thesis. Results are presented on, at that time, the world’s most compact AWG using a double-etch technique, and the world’s first InAs/InP quantum dot (QD) lasers employing narrow deeply etched ridge active waveguides in the 1.55 µm wavelength region. Before realizing a final RMLL design on an active-passive wafer, a series of allactive devices has been designed, fabricated and characterized. These all-active chips provided material for the gain measurements and allowed to look further into short pulse laser characterization techniques and to test designs for reducing reflections from other intra-cavity components. The results of the all-active MLLs have been obtained in different configurations. Firstly, 20 GHz and 40 GHz linear all active Fabry-Pérot MLL (FPMLL) lasers have been successfully fabricated. Modelocking has been achieved with these lasers in the colliding pulse modelocked (CPM) and self CPM configurations. Pulse lengths down to 1.6 ps (at 20 GHz) have been observed. A 40 GHz repetition rate was demonstrated in a CPM laser with a Saturable Absorber (SA) positioned in the center of the FP cavity. All-active 15 GHz RMLLs have also been successfully fabricated. These lasers show a relatively good timing stability due to the ring configuration. Measured output pulses are highly chirped and an FWHM bandwidth of up to 4.5 nm was obtained. Such lasers with high bandwidth pulses and compatible with active-passive integration are of great interest for optical code division multiple access applications, where information is coded in the spectrum. Finally, first results from MLLs realized on an active-passive wafer are presented. Passive modelocking has been demonstrated in these integrated Extended Cavity FPMLLs with minimized intra-cavity reflections. Pulses of 2.1 ps duration and with a small pedestal have been observed. The pulses are close to transform-limited. The longer timescale dynamics of the EC-FPMLLs are reduced compared to the all-active FPMLLs, which is understood to be due to the short amplifier section. The use of a MLL at 20 GHz for the all optical clock recovery (AOCR) application and a special RMLL design for AOCR at 40 GHz are presented in the last chapter of this thesis. Many characteristics of the AOCR at 20 GHz could be quantified. The design of the 40 GHz RMLL laser is for an active-passive wafer. The design utilizes all the minimizations of small intra-cavity reflections. For the AOCR application a novel way to couple the optical input signal into the MLL via a separate waveguide is presented. Based on the accumulated results presented in this thesis the timing jitter of the clock recovered from this laser is expected to be sufficiently low to comply with the telecom requirements at 40 GHz