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Dynamic deformability of individual PbSe nanocrystals during superlattice phase transitions
The behavior of individual nanocrystals during superlattice phase transitions can profoundly affect the structural perfection and electronic properties of the resulting superlattices. However, details of nanocrystal morphological changes during superlattice phase transitions are largely unknown due to the lack of direct observation. Here, we report the dynamic deformability of PbSe semiconductor nanocrystals during superlattice phase transitions that are driven by ligand displacement. Real-time high-resolution imaging with liquid-phase transmission electron microscopy reveals that following ligand removal, the individual PbSe nanocrystals experience drastic directional shape deformation when the spacing between nanocrystals reaches 2 to 4 nm. The deformation can be completely recovered when two nanocrystals move apart or it can be retained when they attach. The large deformation, which is responsible for the structural defects in the epitaxially fused nanocrystal superlattice, may arise from internanocrystal dipole-dipole interactions
Graph States, Pivot Minor, and Universality of (X,Z)-measurements
The graph state formalism offers strong connections between quantum
information processing and graph theory. Exploring these connections, first we
show that any graph is a pivot-minor of a planar graph, and even a pivot minor
of a triangular grid. Then, we prove that the application of measurements in
the (X,Z)-plane over graph states represented by triangular grids is a
universal measurement-based model of quantum computation. These two results are
in fact two sides of the same coin, the proof of which is a combination of
graph theoretical and quantum information techniques
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Generation of Porous Structures Using Fused Deposition
The Fused Deposition Modeling process uses hardware and software machine-level
language that are very similar to that of a pen-plotter. Consequently, the·use of patterns with
poly-lines as basic geometric features, instead of the current method based on filled polygons
(monolithic models), can increase its efficiency.
In the current study, various toolpath planning methods have been developed to fabricate
porous structures. Computational domain decomposition methods can be applied to the physical
or to slice-level domains to generate structured and unstructured grids. Also, textures can be
created using periodic tiling of the layer with unit cells (squares, honeycombs, etc). Methods
'based on curves include fractal space filling curves and.change of effective road width Within a
layer or within a continuous curve. Individual phases can also be placed in binary compositions.
In present investigation, a custom software has been developed and implemented to
generate build files (SML) and slice files (SSL) for the above-mentioned structures, demonstrating the efficient control ofthe size, shape, and distribution ofporosity.Mechanical Engineerin
Hexagonal structure for intelligent vision
Using hexagonal grids to represent digital images have been studied for more than 40 years. Increased processing capabilities of graphic devices and recent improvements in CCD technology have made hexagonal sampling attractive for practical applications and brought new interests on this topic. The hexagonal structure is considered to be preferable to the rectangular structure due to its higher sampling efficiency, consistent connectivity and higher angular resolution and is even proved to be superior to square structure in many applications. Since there is no mature hardware for hexagonal-based image capture and display, square to hexagonal image conversion has to be done before hexagonal-based image processing. Although hexagonal image representation and storage has not yet come to a standard, experiments based on existing hexagonal coordinate systems have never ceased. In this paper, we firstly introduced general reasons that hexagonally sampled images are chosen for research. Then, typical hexagonal coordinates and addressing schemes, as well as hexagonal based image processing and applications, are fully reviewed. © 2005 IEEE
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In Situ TEM Study of the Degradation of PbSe Nanocrystals in Air
PbSe
nanocrystals have attracted widespread attention due to a
variety of potential applications. However, the practical utility
of these nanocrystals has been hindered by their poor air stability,
which induces undesired changes in the optical and electronic properties.
An understanding of the degradation of PbSe nanocrystals when they
are exposed to air is critical for improving the stability and enhancing
their applications. Here, we use in situ transmission electron microscopy
(TEM) with an environmental cell connected to air to study PbSe nanocrystal
degradation triggered by air exposure. We have also conducted a series
of complementary studies, including in situ environmental TEM study
of PbSe nanocrystals exposed to pure oxygen and PbSe nanocrystals
in H2O using a liquid cell, and ex situ experiments, such
as O2 plasma treatment and thermal heating of PbSe nanocrystals
under different air exposure. Our in situ observations reveal that
when PbSe nanocrystals are exposed to air (or oxygen) under electron
beam irradiation, they experience a series of changes, including shape
evolution of individual nanocrystals with the cuboid intermediates,
coalescence between nanocrystals, and formation of PbSe thin films
through drastic solid-state fusion. Further studies show that the
PbSe thin films transform into an amorphous Pb rich phase or eventually
pure Pb, which suggest that Se reacts with oxygen and can be evaporated
under electron beam illumination. These various in situ and ex situ
experimental results indicate that PbSe nanocrystal degradation in
air is initiated by the dissociation and removal of ligands from the
PbSe nanocrystal surface
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