Quantum dichotomies and coherent thermodynamics beyond first-order asymptotics

We address the problem of exact and approximate transformation of quantum dichotomies in the asymptotic regime, i.e., the existence of a quantum channel $\mathcal E$ mapping $\rho_1^{\otimes n}$ into $\rho_2^{\otimes R_nn}$ with an error $\epsilon_n$ (measured by trace distance) and $\sigma_1^{\otimes n}$ into $\sigma_2^{\otimes R_n n}$ exactly, for a large number $n$. We derive second-order asymptotic expressions for the optimal transformation rate $R_n$ in the small, moderate, and large deviation error regimes, as well as the zero-error regime, for an arbitrary pair $(\rho_1,\sigma_1)$ of initial states and a commuting pair $(\rho_2,\sigma_2)$ of final states. We also prove that for $\sigma_1$ and $\sigma_2$ given by thermal Gibbs states, the derived optimal transformation rates in the first three regimes can be attained by thermal operations. This allows us, for the first time, to study the second-order asymptotics of thermodynamic state interconversion with fully general initial states that may have coherence between different energy eigenspaces. Thus, we discuss the optimal performance of thermodynamic protocols with coherent inputs and describe three novel resonance phenomena allowing one to significantly reduce transformation errors induced by finite-size effects. What is more, our result on quantum dichotomies can also be used to obtain, up to second-order asymptotic terms, optimal conversion rates between pure bipartite entangled states under local operations and classical communication.Comment: 51 pages, 6 figures, comments welcom

Overcoming entropic limitations on asymptotic state transformations through probabilistic protocols

The quantum relative entropy is known to play a key role in determining the asymptotic convertibility of quantum states in general resource-theoretic settings, often constituting the unique monotone that is relevant in the asymptotic regime. We show that this is no longer the case when one allows stochastic protocols that may only succeed with some probability, in which case the quantum relative entropy is insufficient to characterize the rates of asymptotic state transformations, and a new entropic quantity based on a regularization of Hilbert's projective metric comes into play. Such a scenario is motivated by a setting where the cost associated with transformations of quantum states, typically taken to be the number of copies of a given state, is instead identified with the size of the quantum memory needed to realize the protocol. Our approach allows for constructing transformation protocols that achieve strictly higher rates than those imposed by the relative entropy. Focusing on the task of resource distillation, we give broadly applicable strong converse bounds on the asymptotic rates of probabilistic distillation protocols, and show them to be tight in relevant settings such as entanglement distillation with non-entangling operations. This generalizes and extends previously known limitations that only apply to deterministic protocols. Our methods are based on recent results for probabilistic one-shot transformations as well as a new asymptotic equipartition property for the projective relative entropy.Comment: 7+16 pages, 2 figure

Sufficiency of R\'enyi divergences

A set of classical or quantum states is equivalent to another one if there exists a pair of classical or quantum channels mapping either set to the other one. For dichotomies (pairs of states) this is closely connected to (classical or quantum) R\'enyi divergences (RD) and the data-processing inequality: If a RD remains unchanged when a channel is applied to the dichotomy, then there is a recovery channel mapping the image back to the initial dichotomy. Here, we prove for classical dichotomies that equality of the RDs alone is already sufficient for the existence of a channel in any of the two directions and discuss some applications. We conjecture that equality of the minimal quantum RDs is sufficient in the quantum case and prove it for special cases. We also show that neither the Petz quantum nor the maximal quantum RDs are sufficient. As a side-result of our techniques we obtain an infinite list of inequalities fulfilled by the classical, the Petz quantum, and the maximal quantum RDs. These inequalities are not true for the minimal quantum RDs.Comment: Comments welcome, 31 pages, v2: Removed insignifcant error; v3: Misupload; v4: Significantly improved presentatio

Relative Entropy and Catalytic Relative Majorization

Given two pairs of quantum states, a fundamental question in the resource theory of asymmetric distinguishability is to determine whether there exists a quantum channel converting one pair to the other. In this work, we reframe this question in such a way that a catalyst can be used to help perform the transformation, with the only constraint on the catalyst being that its reduced state is returned unchanged, so that it can be used again to assist a future transformation. What we find here, for the special case in which the states in a given pair are commuting, and thus quasi-classical, is that this catalytic transformation can be performed if and only if the relative entropy of one pair of states is larger than that of the other pair. This result endows the relative entropy with a fundamental operational meaning that goes beyond its traditional interpretation in the setting of independent and identical resources. Our finding thus has an immediate application and interpretation in the resource theory of asymmetric distinguishability, and we expect it to find application in other domains.Comment: v3: 18 pages, 1 figure, accepted for publication in Physical Review Researc

The Semiring of Dichotomies and Asymptotic Relative Submajorization

We study quantum dichotomies and the resource theory of asymmetric distinguishability using a generalization of Strassen's theorem on preordered semirings. We find that an asymptotic variant of relative submajorization, defined on unnormalized dichotomies, is characterized by real-valued monotones that are multiplicative under the tensor product and additive under the direct sum. These strong constraints allow us to classify and explicitly describe all such monotones, leading to a rate formula expressed as an optimization involving sandwiched Rényi divergences. As an application we give a new derivation of the strong converse error exponent in quantum hypothesis testing

The semiring of dichotomies and asymptotic relative submajorization

We study quantum dichotomies and the resource theory of asymmetric distinguishability using a generalization of Strassen's theorem on preordered semirings. We find that an asymptotic variant of relative submajorization, defined on unnormalized dichotomies, is characterized by real-valued monotones that are multiplicative under the tensor product and additive under the direct sum. These strong constraints allow us to classify and explicitly describe all such monotones, leading to a rate formula expressed as an optimization involving sandwiched R\'enyi divergences. As an application we give a new derivation of the strong converse error exponent in quantum hypothesis testing.Comment: 21 page

Variance of Relative Surprisal as Single-Shot Quantifier

The variance of (relative) surprisal, also known as varentropy, so far mostly plays a role in information theory as quantifying the leading-order corrections to asymptotic independent and identically distributed (IID) limits. Here, we comprehensively study the use of it to derive single-shot results in (quantum) information theory. We show that it gives genuine sufficient and necessary conditions for approximate state transitions between pairs of quantum states in the single-shot setting, without the need for further optimization. We also clarify its relation to smoothed min and max entropies, and construct a monotone for resource theories using only the standard (relative) entropy and variance of (relative) surprisal. This immediately gives rise to enhanced lower bounds for entropy production in random processes. We establish certain properties of the variance of relative surprisal, which will be useful for further investigations, such as uniform continuity and upper bounds on the violation of subadditivity. Motivated by our results, we further derive a simple and physically appealing axiomatic single-shot characterization of (relative) entropy, which we believe to be of independent interest. We illustrate our results with several applications, ranging from interconvertibility of ergodic states, over Landauer erasure to a bound on the necessary dimension of the catalyst for catalytic state transitions and Boltzmann’s H theorem

Benchmarking one-shot distillation in general quantum resource theories

We study the one-shot distillation of general quantum resources, providing a unified quantitative description of the maximal fidelity achievable in this task, and revealing similarities shared by broad classes of resources. We establish fundamental quantitative and qualitative limitations on resource distillation applicable to all convex resource theories. We show that every convex quantum resource theory admits a meaningful notion of a pure maximally resourceful state which maximizes several monotones of operational relevance and finds use in distillation. We endow the generalized robustness measure with an operational meaning as an exact quantifier of performance in distilling such maximal states in many classes of resources including bi- and multipartite entanglement, multi-level coherence, as well as the whole family of affine resource theories, which encompasses important examples such as asymmetry, coherence, and thermodynamics.Comment: 8+5 pages, 1 figure. v3: fixed (inconsequential) error in Lemma 1