Spin-phonon coupling in Gd(Co1/2Mn1/2)O3 perovskite

We have investigated the temperature-dependent Raman-active phonons and the magnetic properties of Gd(Co1/2Mn1/2)O3 perovskite ceramics in the temperature range from 40 K to 300 K. The samples crystallized in an orthorhombic distorted simple perovskite, whose symmetry belongs to the Pnma space group. The data reveals spin-phonon coupling near the ferromagnetic transition occurring at around 120 K. The correlation of the Raman and magnetization data suggests that the structural order influences the magnitude of the spin-phonon coupling.Comment: 3 Figures, suplementary materia

A library of ab initio Raman spectra for automated identification of 2D materials

Raman spectroscopy is frequently used to identify composition, structure and layer thickness of 2D materials. Here, we describe an efficient first-principles workflow for calculating resonant first-order Raman spectra of solids within third-order perturbation theory employing a localized atomic orbital basis set. The method is used to obtain the Raman spectra of 733 different monolayers selected from the computational 2D materials database (C2DB). We benchmark the computational scheme against available experimental data for 15 known monolayers. Furthermore, we propose an automatic procedure for identifying a material based on an input experimental Raman spectrum and illustrate it for the cases of MoS$_2$ (H-phase) and WTe$_2$ (T$^\prime$-phase). The Raman spectra of all materials at different excitation frequencies and polarization configurations are freely available from the C2DB. Our comprehensive and easily accessible library of \textit{ab initio} Raman spectra should be valuable for both theoreticians and experimentalists in the field of 2D materialsComment: 17 pages, 7 figure

Architectures for a quantum random access memory

A random access memory, or RAM, is a device that, when interrogated, returns the content of a memory location in a memory array. A quantum RAM, or qRAM, allows one to access superpositions of memory sites, which may contain either quantum or classical information. RAMs and qRAMs with n-bit addresses can access 2^n memory sites. Any design for a RAM or qRAM then requires O(2^n) two-bit logic gates. At first sight this requirement might seem to make large scale quantum versions of such devices impractical, due to the difficulty of constructing and operating coherent devices with large numbers of quantum logic gates. Here we analyze two different RAM architectures (the conventional fanout and the "bucket brigade") and propose some proof-of-principle implementations which show that in principle only O(n) two-qubit physical interactions need take place during each qRAM call. That is, although a qRAM needs O(2^n) quantum logic gates, only O(n) need to be activated during a memory call. The resulting decrease in resources could give rise to the construction of large qRAMs that could operate without the need for extensive quantum error correction.Comment: 10 pages, 7 figures. Updated version includes the answers to the Refere

Vibro-Acoustic FE Analyses of the Saab 2000 Aircraft

A finite element model of the Saab 2000 fuselage structure and interior cavity has been created in order to compute the noise level in the passenger cabin due to propeller noise. Areas covered in viewgraph format include the following: coupled acoustic/structural noise; data base creation; frequency response analysis; model validation; and planned analyses

Event notification services: analysis and transformation of profile definition languages

The integration of event information from diverse event notification sources is, as with meta-searching over heterogeneous search engines, a challenging task. Due to the complexity of profile definition languages, known solutions for heterogeneous searching cannot be applied for event notification. In this technical report, we propose transformation rules for profile rewriting. We transform each profile defined at a meta-service into a profile expressed in the language of each event notification source. Due to unavoidable asymmetry in the semantics of different languages, some superfluous information may be delivered to the meta-service. These notifications are then post-processed to reduce the number of spurious messages. We present a survey and classification of profile definition languages for event notification, which serves as basis for the transformation rules. The proposed rules are implemented in a prototype transformation module for a Meta-Service for event notification

A theoretical and experimental investigation into multilayered piezoelectric composite transducers

The behaviour of a number of 3-1 connectivity piezoelectric composite plate transducers is presented. The fundamental thickness mode resonance of such devices is found to be contaminated by lateral resonant activity; this is evidenced in the measured and predicted electrical impedance profile and the surface displacement data at the,fundamental thickness mode. Measurements taken on the 3-1 devices infer that they are not acting as true composites. In addition to this the finite element technique is applied to a number of stacked 3-1 and 1-3 connectivity devices to predict the mechanical Q-factor, and hence bandwidth, as a function of polymer filler properties

Normal Mode Determination of Perovskite Crystal Structures with Octahedral Rotations: Theory and Applications

Nuclear site analysis methods are used to enumerate the normal modes of $ABX_{3}$ perovskite polymorphs with octahedral rotations. We provide the modes of the fourteen subgroups of the cubic aristotype describing the Glazer octahedral tilt patterns, which are obtained from rotations of the $BX_{6}$ octahedra with different sense and amplitude about high symmetry axes. We tabulate all normal modes of each tilt system and specify the contribution of each atomic species to the mode displacement pattern, elucidating the physical meaning of the symmetry unique modes. We have systematically generated 705 schematic atomic displacement patterns for the normal modes of all 15 (14 rotated + 1 unrotated) Glazer tilt systems. We show through some illustrative examples how to use these tables to identify the octahedral rotations, symmetric breathing, and first-order Jahn-Teller anti-symmetric breathing distortions of the $BX_{6}$ octahedra, and the associated Raman selection rules. We anticipate that these tables and schematics will be useful in understanding the lattice dynamics of bulk perovskites and would serve as reference point in elucidating the atomic origin of a wide range of physical properties in synthetic perovskite thin films and superlattices.Comment: 17 pages, 3 figures, 17 tables. Supporting information accessed through link specified within manuscrip