Accurate near-field calculation in the rigorous coupled-wave analysis method

The rigorous coupled-wave analysis (RCWA) is one of the most successful and widely used methods for modeling periodic optical structures. It yields fast convergence of the electromagnetic far-field and has been adapted to model various optical devices and wave configurations. In this article, we investigate the accuracy with which the electromagnetic near-field can be calculated by using RCWA and explain the observed slow convergence and numerical artifacts from which it suffers, namely unphysical oscillations at material boundaries due to the Gibb's phenomenon. In order to alleviate these shortcomings, we also introduce a mathematical formulation for accurate near-field calculation in RCWA, for one- and two-dimensional straight and slanted diffraction gratings. This accurate near-field computational approach is tested and evaluated for several representative test-structures and configurations in order to illustrate the advantages provided by the proposed modified formulation of the RCWA.Comment: 13 pages, 12 figure

Theory and simulation of subwavelength high contrast gratings and their applications in vertical-cavity surface-emitting laser devices

This work intends to fully explore the qualities and applications of subwavelength gratings. Subwavelength gratings are diffraction gratings with physical dimensions less than the wavelength of incident light. It has been found that by tailoring specific dimension parameters, a number of different reflection profiles can be attained by these structures including high reflectivity or low reflectivity with broad and narrow spectral responses. In the course of this thesis the physical basis for this phenomenon will be presented as well as a mathematical derivation. After discussion of the mechanics of the reflection behavior, the methods used in modeling subwavelength gratings and designing them for specific functions will be explored. Following this, the fundamentals of vertical-cavity surface-emitting lasers (VCSELs) will be discussed, and the applications of subwavelength gratings when used with these lasers will follow. Several devices, both theoretical proposals and fabricated examples, will be presented in addition to the available performance measurements. Finally, the fabrication challenges that restrict subwavelength gratings from adoption as standard components in VCSEL design will be considered with regard to ongoing fabrication research

Patterned probes for high precision 4D-STEM bragg measurements.

Nanoscale strain mapping by four-dimensional scanning transmission electron microscopy (4D-STEM) relies on determining the precise locations of Bragg-scattered electrons in a sequence of diffraction patterns, a task which is complicated by dynamical scattering, inelastic scattering, and shot noise. These features hinder accurate automated computational detection and position measurement of the diffracted disks, limiting the precision of measurements of local deformation. Here, we investigate the use of patterned probes to improve the precision of strain mapping. We imprint a "bullseye" pattern onto the probe, by using a binary mask in the probe-forming aperture, to improve the robustness of the peak finding algorithm to intensity modulations inside the diffracted disks. We show that this imprinting leads to substantially improved strain-mapping precision at the expense of a slight decrease in spatial resolution. In experiments on an unstrained silicon reference sample, we observe an improvement in strain measurement precision from 2.7% of the reciprocal lattice vectors with standard probes to 0.3% using bullseye probes for a thin sample, and an improvement from 4.7% to 0.8% for a thick sample. We also use multislice simulations to explore how sample thickness and electron dose limit the attainable accuracy and precision for 4D-STEM strain measurements

Collaborative development of diffraction-limited beamline optical systems at US DOE light sources

An ongoing collaboration among four US Department of Energy (DOE) National Laboratories has demonstrated key technology prototypes and software modeling tools required for new high-coherent flux beamline optical systems. New free electron laser (FEL) and diffraction-limited storage ring (DLSR) light sources demand wavefront preservation from source to sample to achieve and maintain optimal performance. Fine wavefront control was achieved using a novel, roomtemperature cooled mirror system called REAL (resistive element adjustable length) that combines cooling with applied, spatially variable auxiliary heating. Single-grating shearing interferometry (also called Talbot interferometry) and Hartmann wavefront sensors were developed and used for optical characterization and alignment on several beamlines, across a range of photon energies. Demonstrations of non-invasive hard x-ray wavefront sensing were performed using a thin diamond single-crystal as a beamsplitter

Manipulating the Interaction between Localized and Delocalized Surface Plasmon Polaritons in Graphene

The excitation of localized or delocalized surface plasmon polaritons in nanostructured or extended graphene has attracted a steadily increasing attention due to their promising applications in sensors, switches, and filters. These single resonances may couple and intriguing spectral signatures can be achieved by exploiting the entailing hybridization. Whereas thus far only the coupling between localized or delocalized surface plasmon polaritons has been studied in graphene nanostructures, we consider here the interaction between a localized and a delocalized surface plasmon polariton. This interaction can be achieved by two different schemes that reside on either evanescent near- field coupling or far-field interference. All observable phenomena are corroborated by analytical considerations, providing insight into the physics and paving the way for compact and tunable optical components at infrared and terahertz frequencies.Comment: 6 pages, 4 figure

Characterization and Application of Hard X-Ray Betatron Radiation Generated by Relativistic Electrons from a Laser-Wakefield Accelerator

The necessity for compact table-top x-ray sources with higher brightness, shorter wavelength and shorter pulse duration has led to the development of complementary sources based on laser-plasma accelerators, in contrast to conventional accelerators. Relativistic interaction of short-pulse lasers with underdense plasmas results in acceleration of electrons and in consequence in the emission of spatially coherent radiation, which is known in the literature as betatron radiation. In this article we report on our recent results in the rapidly developing field of secondary x-ray radiation generated by high-energy electron pulses. The betatron radiation is characterized with a novel setup allowing to measure the energy, the spatial energy distribution in the far-field of the beam and the source size in a single laser shot. Furthermore, the polarization state is measured for each laser shot. In this way the emitted betatron x-rays can be used as a non-invasive diagnostic tool to retrieve very subtle information of the electron dynamics within the plasma wave. Parallel to the experimental work, 3D particle-in-cell simulations were performed, proved to be in good agreement with the experimental results.Comment: 38 pages, 19 figures, submitted to the Journal of Plasma Physic

Laser diagnostics and minor species detection in combustion using resonant four-wave mixing

Peer reviewedPostprin

Deep Learning Reveals Underlying Physics of Light-matter Interactions in Nanophotonic Devices

In this paper, we present a deep learning-based (DL-based) algorithm, as a purely mathematical platform, for providing intuitive understanding of the properties of electromagnetic (EM) wave-matter interaction in nanostructures. This approach is based on using the dimensionality reduction (DR) technique to significantly reduce the dimensionality of a generic EM wave-matter interaction problem without imposing significant error. Such an approach implicitly provides useful information about the role of different features (or design parameters such as geometry) of the nanostructure in its response functionality. To demonstrate the practical capabilities of this DL-based technique, we apply it to a reconfigurable optical metadevice enabling dual-band and triple-band optical absorption in the telecommunication window. Combination of the proposed approach with existing commercialized full-wave simulation tools offers a powerful toolkit to extract basic mechanisms of wave-matter interaction in complex EM devices and facilitate the design and optimization of nanostructures for a large range of applications including imaging, spectroscopy, and signal processing. It is worth to mention that the demonstrated approach is general and can be used in a large range of problems as long as enough training data can be provided

High photon flux table-top coherent extreme ultraviolet source

High harmonic generation (HHG) enables extreme ultraviolet radiation with table-top setups. Its exceptional properties, such as coherence and (sub)-femtosecond pulse durations, have led to a diversity of applications. Some of these require a high photon flux and megahertz repetition rates, e.g. to avoid space charge effects in photoelectron spectroscopy. To date this has only been achieved with enhancement cavities. Here, we establish a novel route towards powerful HHG sources. By achieving phase-matched HHG of a megahertz fibre laser we generate a broad plateau (25 eV - 40 eV) of strong harmonics, each containing more than $10^{12}$ photons/s, which constitutes an increase by more than one order of magnitude in that wavelength range. The strongest harmonic (H25, 30 eV) has an average power of 143 $\mu$W ($3\cdot10^{13}$ photons/s). This concept will greatly advance and facilitate applications in photoelectron or coincidence spectroscopy, coherent diffractive imaging or (multidimensional) surface science