38 research outputs found
Electron energy loss spectroscopy with parallel readout of energy and momentum
We introduce a high energy resolution electron source that matches the
requirements for parallel readout of energy and momentum of modern
hemispherical electron energy analyzers. The system is designed as an add-on
device to typical photoemission chambers. Due to the multiplex gain, a complete
phonon dispersion of a Cu(111) surface was measured in seven minutes with 4 meV
energy resolution
Orientation Dependence of Step Stiffness: Failure of SOS and Ising Models to Describe Experimental Data
We have investigated the step stiffness on Cu(001) surfaces as a function of
step orientation by two independent methods at several temperatures near 300 K.
Both sets of data agree well and show a substantial dependence of the stiffness
on the angle of orientation. With the exception of steps oriented along
, the experimental stiffness is significantly larger than the stiffness
calculated within the solid-on-solid (SOS) model and the Ising-model, even if
next nearest-neighbor interactions are taken into account. Our results have
considerable consequences for the understanding and for the theoretical
modeling of equilibrium and growth phenomena, such as step meandering
instabilities.Comment: 5 pages, 2 figure
Twisted-light-induced optical transitions in semiconductors: Free-carrier quantum kinetics
We theoretically investigate the interband transitions and quantum kinetics
induced by light carrying orbital angular momentum, or twisted light, in bulk
semiconductors. We pose the problem in terms of the Heisenberg equations of
motion of the electron populations, and inter- and intra-band coherences. Our
theory extends the free-carrier Semiconductor Bloch Equations to the case of
photo-excitation by twisted light. The theory is formulated using cylindrical
coordinates, which are better suited to describe the interaction with twisted
light than the usual cartesian coordinates used to study regular optical
excitation. We solve the equations of motion in the low excitation regime, and
obtain analytical expressions for the coherences and populations; with these,
we calculate the orbital angular momentum transferred from the light to the
electrons and the paramagnetic and diamagnetic electric current densities.Comment: 11 pages, 3 figure
High resolution electron energy loss spectroscopy of spin waves in ultra-thin film â The return of the adiabatic approximation?
The paper reports on recent considerable improvements in electron energy loss spectroscopy (EELS) of spin waves in ultra-thin films. Spin wave spectra with 4 meV resolution are shown. The high energy resolution enables the observation of standing modes in ultra-thin films in the wave vector range of 0.15 Å− 1 < q|| < 0.3 Å− 1. In this range, Landau damping is comparatively small and standing spin wave modes are well-defined Lorentzians for which the adiabatic approximation is well suited, an approximation which was rightly dismissed by Mills and collaborators for spin waves near the Brillouin zone boundary. With the help of published exchange coupling constants, the Heisenberg model, and a simple model for the spectral response function, experimental spectra for Co-films on Cu(100) as well as for Co films capped with further copper layers are successfully simulated. It is shown that, depending on the wave vector and film thickness, the most prominent contribution to the spin wave spectrum may come from the first standing mode, not from the so-called surface mode. In general, the peak position of a low-resolution spin wave spectrum does not correspond to a single mode. A discussion of spin waves based on the “dispersion” of the peak positions in low resolution spectra is therefore subject to errors
Physics of Surfaces and Interfaces
xii;ill.;646hal.;26c