Hole Surface Trapping Dynamics Directly Monitored by Electron Spin Manipulation in CdS Nanocrystals

A new detection technique, pump-spin orientation-probe ultrafast spectroscopy, is developed to study the hole trapping dynamics in colloidal CdS nanocrystals. The hole surface trapping process spatially separates the electron–hole pairs excited by the pump pulse, leaves the core negatively charged, and thus enhances the electron spin signal generated by the orientation pulse. The spin enhancement transients as a function of the pump-orientation delay reveal a fast and a slow hole trapping process with respective time constants of sub-10 ps and sub-100 ps, orders of magnitude faster than that of carrier recombination. The power dependence of hole trapping dynamics elucidates the saturation process and relative number of traps, and suggests that there are three subpopulations of nanoparticles related to hole surface trapping, one with the fast trapping pathway only, another with the slow trapping pathway only, and the third with both pathways together

Hole Surface Trapping Dynamics Directly Monitored by Electron Spin Manipulation in CdS Nanocrystals

A new detection technique, pump-spin orientation-probe ultrafast spectroscopy, is developed to study the hole trapping dynamics in colloidal CdS nanocrystals. The hole surface trapping process spatially separates the electron–hole pairs excited by the pump pulse, leaves the core negatively charged, and thus enhances the electron spin signal generated by the orientation pulse. The spin enhancement transients as a function of the pump-orientation delay reveal a fast and a slow hole trapping process with respective time constants of sub-10 ps and sub-100 ps, orders of magnitude faster than that of carrier recombination. The power dependence of hole trapping dynamics elucidates the saturation process and relative number of traps, and suggests that there are three subpopulations of nanoparticles related to hole surface trapping, one with the fast trapping pathway only, another with the slow trapping pathway only, and the third with both pathways together

Twisting Relativistic Electrons Using Ultra-intense Circularly Polarized Lasers in the Radiation-dominated QED Regime

Relativistic vortex particles offer a promising avenue for investigating and manipulating processes in high-energy and nuclear physics, as they provide an additional degree of freedom in the form of orbital-angular-momentum (OAM). Despite the potential benefits, the generation and detection of these particles have proven to be a significant challenge. In this work, we present a new method for producing high-energy vortex electrons and $\gamma$-photons by colliding relativistic electrons with circularly polarized laser pulses in the radiation-dominated quantum electrodynamics (QED) regime. We use the laser-dressed vortex state to develop a nonlinear scattering theory, which allows us to understand the transfer of spin angular momenta (SAM) to intrinsic OAM in the highly nonlinear multi-photon process. The theory shows that electrons in the vortex state carry higher intrinsic OAM when radiation-reaction becomes significant, with the central OAM number proportional to the amount of energy taken by the $\gamma$-photon. This study provides an effective approach to generating high-energy vortex electron beams using laser intensities that are currently achievable. Additionally, the emission spectra of energetic electrons in vortex states are found to exhibit multi-peaks, which sets them apart from plane-wave electrons and makes them easier to distinguish

Single-scan, dual-functional interferometer for fast spatiotemporal characterization of few-cycle pulses

Accurate and fast characterization of spatiotemporal information of high-intensity, ultrashort pulses is crucial in the field of strong-field laser science and technology. While conventional self-referenced interferometers were widely used to retrieve the spatial profile of the relative spectral phase of pulses, additional measurements of temporal and spectral information at a particular position of the laser beam were, however, necessary to remove the indeterminacy, which increases the system complexity. Here we report an advanced, dual-functional interferometer that is able to reconstruct the complete spatiotemporal information of ultrashort pulses with a single scan of the interferometer arm. The set-up integrates an interferometric frequency-resolved optical gating (FROG) with a radial shearing Michelson interferometer. Trough scanning one arm of the interferometer, both cross-correlated FROG trace at the central part of the laser beam and delay-dependent interferograms of the entire laser profile are simultaneously obtained, allowing a fast 3-dimensional reconstruction of few-cycle laser pulses

Polarization sensitive laser intensity inside femtosecond filament in air

Polarization dependence on clamping intensity inside femtosecond filament was experimentally measured in air. By tuning the laser pulse ellipse from linear polarization to circular polarization, the measured clamping intensity inside laser filament is gradually increased up to 1.7 times. The experimental results are in good agreement with the simulation results by solving the extended nonlinear Schrodinger equation (NLSE). The polarization sensitive clamping intensity inside filaments offers an important factor towards fully understanding the polarization related phenomenon observed so far

2.6mJ/100Hz CEP stable near-single-cycle 4{\mu}m laser based on OPCPA and hollow-core-fiber compression

A carrier envelope phase stable near-single cycle mid-infrared laser based on optical parametric chirped pulse amplification and hollow-core-fiber compression is demonstrated. 4 {\mu}m laser pulses with 11.8 mJ energy are delivered from a KTA based OPCPA with 100 Hz repetition rate, and compressed to be ~105 fs by a two-grating compressor with efficiency over 50%. Subsequently, the pulse spectrum is broadened by employing a krypton gas-filled hollow-core-fiber (HCF). Then, the pulse duration is further compressed to 21.5 fs through a CaF2 bulk material with energy of 2.6 mJ and stability of 0.9% RMS, which is about 1.6 cycle for 4 {\mu}m laser pulse. The near-single cycle 4 {\mu}m laser pulse CEP is passively stabilized with ~370 mrad based on a CEP stable 4 {\mu}m OPA injection

Laser guided ionic wind

We report on a method to experimentally generate ionic wind by coupling an external high voltage electric field with an intense femtosecond laser induced air plasma filament. The measured ionic wind velocity could be as strong as >4 m/s. It could be optimized by changing the applied electric field and the laser induced plasma channel. The experimental observation was qualitatively confirmed by a numerical simulation of spatial distribution of the electric field. This technique is robust and free from sharp metallic electrodes for coronas; it opens a way to optically generate ionic wind at a distance