16,321 research outputs found

    Kinetically-controlled thin-film growth of layered β\beta- and γ\gamma-Nax_{x}CoO2_{2} cobaltate

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    We report growth characteristics of epitaxial β\beta-Na0.6_{0.6}CoO2_{2} and γ\gamma-Na0.7_{0.7}CoO2_{2} thin films on (001) sapphire substrates grown by pulsed-laser deposition. Reduction of deposition rate could change structure of Nax_{x}CoO2_{2} thin film from β\beta-phase with island growth mode to γ\gamma-phase with layer-by-layer growth mode. The γ\gamma-Na0.7_{0.7}CoO2_{2} thin film exhibits spiral surface growth with multiterraced islands and highly crystallized texture compared to that of the β\beta-Na0.6_{0.6}CoO2_{2} thin film. This heterogeneous epitaxial film growth can give opportunity of strain effect of physical properties and growth dynamics of Nax_{x}CoO2_{2} as well as subtle nature of structural change.Comment: accepted for publication in Applied Physics Letter

    Infrared Hall conductivity of Na0.7_{0.7}CoO2_2

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    We report infrared Hall conductivity σxy(ω)\sigma_{xy}(\omega) of Na0.7_{0.7}CoO2_2 thin films determined from Faraday rotation angle θF\theta_{F} measurements. σxy(ω)\sigma_{xy}(\omega) exhibits two types of hole conduction, Drude and incoherent carriers. The coherent Drude carrier shows a large renormalized mass and Fermi liquid-like behavior of Hall scattering rate, γHaT2\gamma_{H} \sim aT^{2}. The spectral weight is suppressed and disappears at T = 120K. The incoherent carrier response is centered at mid-IR frequency and shifts to lower energy with increasing T. Infrared Hall constant is positive and almost independent of temperature in sharp contrast with the dc-Hall constant.Comment: 5 Pages, 5 Figures. Author list corrected in metadata only, paper is unchange

    Mean Field Theoretical Structure of He and Be Isotopes

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    The structures of He and Be even-even isotopes are investigated using an axially symmetric Hartree-Fock approach with a Skyrme-IIIls mean field potential. In these simple HF calculations, He and Be isotopes appear to be prolate in their ground states and Be isotopes have oblate shape isomeric states. It is also shown that there exists a level crossing when the nuclear shape changes from the prolate state to the oblate state. The single neutron levels of Be isotopes exhibit a neutron magic number 6 instead of 8 and show that the level inversion between 1/2- and 1/2+ levels occurs only for a largely deformed isotope. Protons are bound stronger in the isotope with more neutrons while neutron levels are somewhat insensitive to the number of neutrons and thus the nuclear size and also the neutron skin become larger as the neutron number increases. In these simple calculations with Skyrme-IIIls interaction no system with a clear indication of neutron halo was found among He and Be isotopes. Instead of it we have found 8He+2n, 2n+8He+2n, and 16Be+2n like chain structures with clusters of two correlated neutrons. It is also shown that 8He and 14Be in their ground states are below the neutron drip line in which all nucleons are bound with negative energy and that 16Be in its ground state is beyond the neutron drip line with two neutrons in positive energy levels.Comment: CM energy correction, 1 figure and more discussions adde

    Signature of Carrier-Induced Ferromagnetism in Ti_{1-x}Co_{x}O_{2-delta}: Exchange Interaction Between High-Spin Co 2+ and the Ti 3d Conduction Band

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    X-ray photoemission spectroscopy measurements were performed on thin-film samples of rutile Ti_{1-x}Co_{x}O_{2-delta} to reveal the electronic structure. The Co 2p core level spectra indicate that the Co ions take the high-spin Co 2+ configuration, consistent with substitution on the Ti site. The high spin state and the shift due to the exchange splitting of the conduction band suggest strong hybridization between carriers in the Ti 3d t2g band and the t2g states of the high-spin Co 2+. These observations support the argument that room temperature ferromagnetism in Ti_{1-x}Co_{x}O_{2-delta} is intrinsic.Comment: 4 pages, 5 figures. Accepted for publication in Physical Review Letter

    Unusual superexchange pathways in a Ni triangular lattice of NiGa2_2S4_4 with negative charge-transfer energy

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    We have studied the electronic structure of the Ni triangular lattice in NiGa2_2S4_4 using photoemission spectroscopy and subsequent model calculations. The cluster-model analysis of the Ni 2pp core-level spectrum shows that the S 3pp to Ni 3dd charge-transfer energy is \sim -1 eV and the ground state is dominated by the d9Ld^9L configuration (LL is a S 3pp hole). Cell perturbation analysis for the NiS2_2 triangular lattice indicates that the strong S 3pp hole character of the ground state provides the enhanced superexchange interaction between the third nearest neighbor sites.Comment: 10 pages, 5 figures, accepted to PR

    The Dropping of In-Medium Hadron Mass in Holographic QCD

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    We study the baryon density dependence of the vector meson spectrum using the D4/D6 system together with the compact D4 baryon vertex. We find that the vector meson mass decreases almost linearly in density at low density for small quark mass, but saturates to a finite non-zero value for large density. We also compute the density dependence of the η\eta\prime mass and the η\eta\prime velocity. We find that in medium, our model is consistent with the GMOR relation up to a few times the normal nuclear density. We compare our hQCD predictions with predictions made based on hidden local gauge theory that is constructed to model QCD.Comment: 20 pages, 7 figure

    (Non)-Renormalization of the Chiral Vortical Effect Coefficient

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    We show using diagramtic arguments that in some (but not all) cases, the temperature dependent part of the chiral vortical effect coefficient is independent of the coupling constant. An interpretation of this result in terms of quantization in the effective 3 dimensional Chern-Simons theory is also given. In the language of 3D dimensionally reduced theory, the value of the chiral vortical coefficient is related to the formula n=1n=1/12\sum_{n=1}^\infty n=-1/12. We also show that in the presence of dynamical gauge fields, the CVE coefficient is not protected from renormalization, even in the large NN limit.Comment: 11 pages, 3 figures. Version 2 corrects an error and calculates leading radiative correctio

    Half-Metallic Graphene Nanoribbons

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    Electrical current can be completely spin polarized in a class of materials known as half-metals, as a result of the coexistence of metallic nature for electrons with one spin orientation and insulating for electrons with the other. Such asymmetric electronic states for the different spins have been predicted for some ferromagnetic metals - for example, the Heusler compounds- and were first observed in a manganese perovskite. In view of the potential for use of this property in realizing spin-based electronics, substantial efforts have been made to search for half-metallic materials. However, organic materials have hardly been investigated in this context even though carbon-based nanostructures hold significant promise for future electronic device. Here we predict half-metallicity in nanometre-scale graphene ribbons by using first-principles calculations. We show that this phenomenon is realizable if in-plane homogeneous electric fields are applied across the zigzag-shaped edges of the graphene nanoribbons, and that their magnetic property can be controlled by the external electric fields. The results are not only of scientific interests in the interplay between electric fields and electronic spin degree of freedom in solids but may also open a new path to explore spintronics at nanometre scale, based on graphene
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