Low-frequency method for magnetothermopower and Nernst effect measurements on single crystal samples at low temperatures and high magnetic fields

We describe an AC method for the measurement of the longitudinal (Sxx) and transverse (Sxy, i.e. Nernst) thermopower of mm-size single crystal samples at low temperatures (T30 T). A low-frequency (33 mHz) heating method is used to increase the resolution, and to determine the temperature gradient reliably in high magnetic fields. Samples are mounted between two thermal blocks which are heated by a sinusoidal frequency f0 with a p/2 phase difference. The phase difference between two heater currents gives a temperature gradient at 2f0. The corresponding thermopower and Nernst effect signals are extracted by using a digital signal processing method due. An important component of the method involves a superconducting link, YBa2Cu3O7+d (YBCO), which is mounted in parallel with sample to remove the background magnetothermopower of the lead wires. The method is demonstrated for the quasi two-dimensional organic conductor a-(BEDT-TTF)2KHg(SCN)4, which exhibits a complex, magnetic field dependent ground state above 22.5 T at low temperatures.Comment: 11 pages, 6 figures, 15 reference

Violation of Kohler's rule by the magnetoresistance of a quasi-two-dimensional organic metal

The interlayer magnetoresistance of the quasi-two-dimensional metal $\alpha$-(BEDT-TTF)$_2$KHg(SCN)$_4$ is considered. In the temperature range from 0.5 to 10 K and for fields up to 10 tesla the magnetoresistance has a stronger temperature dependence than the zero-field resistance. Consequently Kohler's rule is not obeyed for any range of temperatures or fields. This means that the magnetoresistance cannot be described in terms of semiclassical transport on a single Fermi surface with a single scattering time. Possible explanations for the violations of Kohler's rule are considered, both within the framework of semi-classical transport theory and involving incoherent interlayer transport. The issues considered are similar to those raised by the magnetotransport of the cuprate superconductors.Comment: 5 pages, RevTeX + epsf, 2 figures. Slightly revised version to appear in Physical Review B, May 15, 199

Quantum melting of the quasi-two-dimensional vortex lattice in kappa-(ET)2Cu(NCS)2

We report torque magnetization measurements in regions of the mixed state phase diagram (${\bf B}\sim\mu_o{\bf H}_{c2}$ and T$_c$/$10^3$) of the organic superconductor $\kappa-$(ET)$_2$Cu(NCS)$_2$ where quantum fluctuations are expected to dominate thermal effects. Over most of the field range below the irreversibility line (${\bf B}_{irr}$), magneto-thermal instabilities are observed in the form of flux jumps. The abrupt cessation of these instabilities just below ${\bf B}_{irr}$ indicates a quantum melting transition from a quasi-two-dimensional vortex lattice phase to a quantum liquid phase.Comment: 8 pages (inc. Figs), accepted for publication in Phys. Rev. Let