Conversion of glassy antiferromagnetic-insulating phase to equilibrium ferromagnetic-metallic phase by devitrification and recrystallization in Al substituted Pr0.5{_{0.5}}Ca0.5_{0.5}MnO3{_3}

We show that Pr${_{0.5}}$Ca$_{0.5}$MnO${_3}$ with 2.5% Al substitution and La${_{0.5}}$Ca$_{0.5}$MnO${_3}$ (LCMO) exhibit qualitatively similar and visibly anomalous M-H curves at low temperature. Magnetic field causes a broad first-order but irreversible antiferromagnetic (AF)-insulating (I) to ferromagnetic (FM)-metallic (M) transition in both and gives rise to soft FM state. However, the low temperature equilibrium state of Pr$_{0.5}$Ca$_{0.5}$Mn$_{0.975}$Al$_{0.025}$O$_3$ (PCMAO) is FM-M whereas that of LCMO is AF-I. In both the systems the respective equilibrium phase coexists with the other phase with contrasting order, which is not in equilibrium, and the cooling field can tune the fractions of the coexisting phases. It is shown earlier that the coexisting FM-M phase behaves like `magnetic glass' in LCMO. Here we show from specially designed measurement protocols that the AF-I phase of PCMAO has all the characteristics of magnetic glassy states. It devitrifies on heating and also recrystallizes to equilibrium FM-M phase after annealing. This glass-like AF-I phase also shows similar intriguing feature observed in FM-M magnetic glassy state of LCMO that when the starting coexisting fraction of glass is larger, successive annealing results in larger fraction of equilibrium phase. This similarity between two manganite systems with contrasting magnetic orders of respective glassy and equilibrium phases points toward a possible universality.Comment: Highlights potential of CHUF (Cooling and Heating in Unequal Fields), a new measurement protoco

Calculation of minor hysteresis loops under metastable to stable transformations in vortex matter

We present a model in which metastable supercooled phase and stable equilibrium phase of vortex matter coexist in different regions of a sample. Minor hysteresis loops are calculated with the simple assumption of the two phases of vortex matter having field-independent critical current densities. We use our earlier published ideas that the free energy barrier separating the metastable and stable phases reduces as the magnetic induction moves farther from the first order phase transition line, and that metastable to stable transformations occur in local regions of the sample when the local energy dissipation exceeds a critical value. Previously reported anomalous features in minor hysteresis loops are reproduced, and calculated field profiles are presented.Comment: 9pages, 7 figure

Vortex Matter and its Phase Transitions

The mixed state of type II superconductors has magnetic flux penetrating the sample in the form of vortices, with each vortex carrying an identical quantum of flux. These vortices generally form a triangular lattice under weak mutually repulsive forces; the lattice spacing can be easily varied over many orders of magnitude by varying the external magnetic field. The elastic moduli of this lattice are small and this soft vortex matter can undergo phase transitions like normal matter, but with thermal fluctuations and underlying defects playing an important role. We discuss experimental studies on vortex matter phase transitions, with some emphasis on DC magnetisation measurements investigating the nature of the phase transition.Comment: 11 pages and 4 figure