Ab initio investigation of intermolecular interactions in solid benzene

A computational strategy for the evaluation of the crystal lattice constants and cohesive energy of the weakly bound molecular solids is proposed. The strategy is based on the high level ab initio coupled-cluster determination of the pairwise additive contribution to the interaction energy. The zero-point-energy correction and non-additive contributions to the interaction energy are treated using density functional methods. The experimental crystal lattice constants of the solid benzene are reproduced, and the value of 480 meV/molecule is calculated for its cohesive energy

Assessing the vulnerability of stream communities and the consistency and use of biotic indices in least-disturbed streams

The need in freshwater conservation is to understand the current status of aquatic biota so that we can recognize when degradation or changes occur. Because stream habitats and communities are dynamic, it is important to understand the natural variability through time and space so that departures may be used to make inferences on stability or instability. Additionally, attempting to predict aquatic communities that are more likely to experience a change in diversity, abundance, and function from anthropogenic impacts may help to prioritize locations for management action. Finally, assessing the consistency of various biotic indices (quantitative tools used to convey lotic ecosystem health) will aid in conveying a more holistic depiction of stream condition and to prioritize locations and biota for management action. To address each of the aforementioned data gaps, we used fish and aquatic invertebrate community data collected from 1988 to 2013 from 88 sites within seven National Park Service (NPS) units represented within the Heartland Inventory and Monitoring Network. The fish community (Index of Biotic Integrity) at each of the seven NPS units was less temporally variable than spatially variable. This relationship was not found with aquatic invertebrate community (Hilsenhoff Biotic Index) in that only three of the seven NPS units were less temporally variable than spatially variable

Low-Energy Scale Excitations in the Spectral Function of Organic Monolayer Systems

Using high-resolution photoemission spectroscopy we demonstrate that the electronic structure of several organic monolayer systems, in particular 1,4,5,8-naphthalene tetracarboxylic dianhydride and Copper-phtalocyanine on Ag(111), is characterized by a peculiar excitation feature right at the Fermi level. This feature displays a strong temperature dependence and is immediatly connected to the binding energy of the molecular states, determined by the coupling between the molecule and the substrate. At low temperatures, the line-width of this feature, appearing on top of the partly occupied lowest unoccupied molecular orbital of the free molecule, amounts to only $\approx 25$ meV, representing an unusually small energy scale for electronic excitations in these systems. We discuss possible origins, related e.g. to many-body excitations in the organic-metal adsorbate system, in particular a generalized Kondo scenario based on the single impurity Anderson model.Comment: 6 pages, 3 figures, accepted as PRB Rapid Communication

Measurement of Magnetic-Field Structures in a Laser-Wakefield Accelerator

Experimental measurements of magnetic fields generated in the cavity of a self-injecting laser-wakefield accelerator are presented. Faraday rotation is used to determine the existence of multi-megagauss fields, constrained to a transverse dimension comparable to the plasma wavelength and several plasma wavelengths longitudinally. The fields are generated rapidly and move with the driving laser. In our experiment, the appearance of the magnetic fields is correlated to the production of relativistic electrons, indicating that they are inherently tied to the growth and wavebreaking of the nonlinear plasma wave. This evolution is confirmed by numerical simulations, showing that these measurements provide insight into the wakefield evolution with high spatial and temporal resolution

All-optical measurement of the hot electron sheath driving laser ion acceleration from thin foils

We present experimental results from an all-optical diagnostic method to directly measure the evolution of the hot-electron distribution driving the acceleration of ions from thin foils using high-intensity lasers. Central parameters of laser ion acceleration such as the hot-electron density, the temperature distribution and the conversion efficiency from laser pulse energy into hot electrons become comprehensively accessible with this technique.Deutsche Forschungsgemeinschaft (DFG) (contract number TR18)Germany. Bundesministerium für Bildung und Forschung (contract number 03ZIK445)Germany. Bundesministerium für Bildung und Forschung (contract number 03ZIK052

Recent results on the Higgs boson candidate in the two-photon decay channel at ATLAS

This paper is intended to give an overview of the results of the ATLAS experiment at the LHC presented in December 2012 for the H → γγ channel using 4.8 fb−1 of data taken in 2011 at √s = 7TeV and 13.0 fb−1 of data taken in 2012 at √s = 8TeV

Coulomb implosion mechanism of negative ion acceleration in laser plasmas

Coulomb implosion mechanism of the negatively charged ion acceleration in laser plasmas is proposed. When a cluster target is irradiated by an intense laser pulse and the Coulomb explosion of positively charged ions occurs, the negative ions are accelerated inward. The maximum energy of negative ions is several times lower than that of positive ions. The theoretical description and Particle-in-Cell simulation of the Coulomb implosion mechanism and the evidence of the negative ion acceleration in the experiments on the high intensity laser pulse interaction with the cluster targets are presented.Comment: 4 page

Spectral shaping of laser generated proton beams

The rapid progress in the field of laser particle acceleration has stimulated a debate about the promising perspectives of laser based ion beam sources. For a long time, the beams produced exhibited quasi-thermal spectra. Recent proof-of-principle experiments demonstrated that ion beams with narrow energy distribution can be generated from special target geometries. However, the achieved spectra were strongly limited in terms of monochromacity and reproducibility. We show that microstructured targets can be used to reliably produce protons with monoenergetic spectra above 2 MeV with less than 10% energy spread. Detailed investigations of the effects of laser ablation on the target resulted in a significant improvement of the reproducibility. Based on statistical analysis, we derive a scaling law between proton peak position and laser energy, underlining the suitability of this method for future applications. Both the quality of the spectra and the scaling law are well reproduced by numerical simulations

Nuclear Inelastic X-Ray Scattering of FeO to 48 GPa

The partial density of vibrational states has been measured for Fe in compressed FeO (w\"ustite) using nuclear resonant inelastic x-ray scattering. Substantial changes have been observed in the overall shape of the density of states close to the magnetic transiton around 20 GPa from the paramagnetic (low pressure) to the antiferromagnetic (high pressure) state. Our data indicate a substantial softening of the aggregate sound velocities far below the transition, starting between 5 and 10 GPa. This is consistent with recent radial x-ray diffraction measurements of the elastic constants in FeO. The results indicate that strong magnetoelastic coupling in FeO is the driving force behind the changes in the phonon spectrum of FeO.Comment: 4 pages, 4 figure

Phonons and related properties of extended systems from density-functional perturbation theory

This article reviews the current status of lattice-dynamical calculations in crystals, using density-functional perturbation theory, with emphasis on the plane-wave pseudo-potential method. Several specialized topics are treated, including the implementation for metals, the calculation of the response to macroscopic electric fields and their relevance to long wave-length vibrations in polar materials, the response to strain deformations, and higher-order responses. The success of this methodology is demonstrated with a number of applications existing in the literature.Comment: 52 pages, 14 figures, submitted to Review of Modern Physic