24 research outputs found
Non-reciprocal absorption and zero reflection in physically separated dual photonic resonators by traveling-wave-induced indirect coupling
We experimentally explored novel behaviors of non-reciprocal absorption and almost zero reflection in a dual photon resonator system, which is physically separated and composed of two inverted split ring resonators (ISRRs) with varying inter-distances. We also found that an electromagnetically-induced-transparency (EIT)-like peak at a specific inter-distance of d = 18 mm through traveling waves flowing along a shared microstrip line to which the dual ISRRs are dissipatively coupled. With the aid of CST-simulations and analytical modeling, we found that destructive and/or constructive interferences in traveling waves, indirectly coupled to each ISRR, result in a traveling-wave-induced transparency peak within a narrow window. Furthermore, we observed not only strong non-reciprocal responses of reflectivity and absorptivity at individual inter-distances exactly at the corresponding EIT-like peak positions, but also nearly zero reflection and almost perfect absorption for a specific case of d = 20 mm. Finally, the unidirectional absorptions with zero reflection at d = 20 mm are found to be ascribed to a non-Hermitian origin. This work not only provides a better understanding of traveling-wave-induced indirect coupling between two photonic resonators without magnetic coupling, but also suggests potential implications for the resulting non-reciprocal behaviors of absorption and reflection in microwave circuits and quantum information devices
Additional file 1 of msPIPE: a pipeline for the analysis and visualization of whole-genome bisulfite sequencing data
Additional file 1. Supplementary figures
Additional file 2 of msPIPE: a pipeline for the analysis and visualization of whole-genome bisulfite sequencing data
Additional file 2. Supplementary tables
Enhanced Antimalarial and Antisequestration Activity of Methoxybenzenesulfonate-Modified Biopolymers and Nanoparticles for Tackling Severe Malaria
Severe malaria is
a life-threatening condition that is associated
with a high mortality. Severe Plasmodium falciparum infections are mediated primarily by high parasitemia and binding
of infected red blood cells (iRBCs) to the blood vessel endothelial
layer, a process known as sequestration. Here, we show that including
the 5-amino-2-methoxybenzenesulfonate (AMBS) chemical modification
in soluble biopolymers (polyglutamic acid and heparin) and poly(acrylic
acid)-exposing nanoparticles serves as a universal tool to introduce
a potent parasite invasion inhibitory function in these materials.
Importantly, the modification did not add or eliminated (for heparin)
undesired anticoagulation activity. The materials protected RBCs from
invasion by various parasite strains, employing both major entry pathways.
Two further P. falciparum strains, which either expose
ligands for chondroitin sulfate A (CSA) or intercellular adhesion
molecule 1 (ICAM-1) on iRBCs, were tested in antisequestration assays
due to their relevance in placental and cerebral malaria, respectively.
Antisequestration activity was found to be more efficacious with nanoparticles vs gold-standard soluble biopolymers (CSA and heparin) against
both strains, when tested on receptor-coated dishes. The nanoparticles
also efficiently inhibited and reversed the sequestration of iRBCs
on endothelial cells. First, the materials described herein have the
potential to reduce the parasite burden by acting at the key multiplication
stage of reinvasion. Second, the antisequestration ability could help
remove iRBCs from the blood vessel endothelium, which could otherwise
cause vessel obstruction, which in turn can lead to multiple organ
failure in severe malaria infections. This approach represents a further
step toward creation of adjunctive therapies for this devastating
condition to reduce morbidity and mortality
Realizing Electronic Synapses by Defect Engineering in Polycrystalline Two-Dimensional MoS<sub>2</sub> for Neuromorphic Computing
Neuromorphic computing based on two-dimensional transition-metal
dichalcogenides (2D TMDs) has attracted significant attention recently
due to their extraordinary properties generated by the atomic-thick
layered structure. This study presents sulfur-defect-assisted MoS2 artificial synaptic devices fabricated by a simple sputtering
process, followed by a precise sulfur (S) vacancy-engineering process.
While the as-sputtered MoS2 film does not show synaptic
behavior, the S vacancy-controlled MoS2 film exhibits excellent
synapse with remarkable nonvolatile memory characteristics such as
a high switching ratio (∼103), a large memory window,
and long retention time (∼104 s) in addition to
synaptic functions such as paired-pulse facilitation (PPF) and long-term
potentiation (LTP)/depression (LTD). The synaptic device working mechanism
of Schottky barrier height modulation by redistributing S vacancies
was systemically analyzed by electrical, physical, and microscopy
characterizations. The presented MoS2 synaptic device,
based on the precise defect engineering of sputtered MoS2, is a facile, low-cost, complementary metal-oxide semiconductor
(CMOS)-compatible, and scalable method and provides a procedural guideline
for the design of practical 2D TMD-based neuromorphic computing
Quantitative Interpretation of Electromagnetic Interference Shielding Efficiency: Is It Really a Wave Absorber or a Reflector?
As electromagnetic
(EM) pollution continues to increase, electromagnetic
interference (EMI) shielding materials have been intensively evaluated
in terms of two main shielding mechanisms of reflection and absorption.
Since the shielding effectiveness (SE) is represented in the logarithmic
scale and in a coupled way of transmission (SET), absorption
(SEA), and reflection (SER), often there is
a misinterpretation that the EM wave reflectors are regarded as EM
wave-absorbing materials. Surprisingly, we found that many materials
reported as an EM wave absorber in the literature provide, in fact,
less than 50% of EM wave-absorbing capability, i.e., over 50% of EM
wave-reflecting feature. According to the theory and definition of
EMI SE, the absorption-dominant EMI shielding materials should have
the ratio of absorption to incident energy (A) as A > 0.5, which corresponds to a necessary condition that
SER R subsequently gives
SEA in relation to SET. Using this criterion,
we classified the EMI shielding materials with their shielding mechanism.
The proposed methodology provides significant insight into the evaluation
and development of EMI shielding materials
Near-Field Electrospinning for Three-Dimensional Stacked Nanoarchitectures with High Aspect Ratios
Near-field electrospinning (NFES) was developed to overcome
the
intrinsic instability of traditional electrospinning processes and
to facilitate the controllable deposition of nanofibers under a reduced
electric field. This technique offers a straightforward and versatile
method for the precision patterning of two-dimensional (2D) nanofibers.
However, three-dimensional (3D) stacked structures built by NFES have
been limited to either micron-scale sizes or special shapes. Herein,
we report on a direct-write 3D NFES technique to construct self-aligned,
template-free, 3D stacked nanoarchitectures by simply adding salt
to the polymer solution. Numerical simulations suggested that the
electric field could be tuned to achieve self-aligned nanofibers by
adjusting the conductivity of the polymer solution. This was confirmed
experimentally by using poly(ethylene oxide) (PEO) solutions containing
0.1–1.0 wt% NaCl. Using 0.1 wt% NaCl, nanowalls with a maximum
of 80 layers could be built with a width of 92 ± 3 nm, height
of 6.6 ± 0.1 μm, and aspect ratio (height/width) of 72.
We demonstrate the 3D printing of nanoskyscrapers with various designs,
such as curved “nanowall arrays”, nano “jungle
gyms,” and “nanobridges”. Further, we present
an application of the 3D stacked nanofiber arrays by preparing transparent
and flexible polydimethylsiloxane films embedded with Ag-sputtered
nanowalls as 3D nanoelectrodes. The conductivity of the nanoelectrodes
can be precisely tuned by adjusting the number of 3D printed layers,
without sacrificing transmittance (98.5%). The current NFES approach
provides a simple, reliable route to build 3D stacked nanoarchitectures
with high-aspect ratios for potential application in smart materials,
energy devices, and biomedical applications
Near-Field Electrospinning for Three-Dimensional Stacked Nanoarchitectures with High Aspect Ratios
Near-field electrospinning (NFES) was developed to overcome
the
intrinsic instability of traditional electrospinning processes and
to facilitate the controllable deposition of nanofibers under a reduced
electric field. This technique offers a straightforward and versatile
method for the precision patterning of two-dimensional (2D) nanofibers.
However, three-dimensional (3D) stacked structures built by NFES have
been limited to either micron-scale sizes or special shapes. Herein,
we report on a direct-write 3D NFES technique to construct self-aligned,
template-free, 3D stacked nanoarchitectures by simply adding salt
to the polymer solution. Numerical simulations suggested that the
electric field could be tuned to achieve self-aligned nanofibers by
adjusting the conductivity of the polymer solution. This was confirmed
experimentally by using poly(ethylene oxide) (PEO) solutions containing
0.1–1.0 wt% NaCl. Using 0.1 wt% NaCl, nanowalls with a maximum
of 80 layers could be built with a width of 92 ± 3 nm, height
of 6.6 ± 0.1 μm, and aspect ratio (height/width) of 72.
We demonstrate the 3D printing of nanoskyscrapers with various designs,
such as curved “nanowall arrays”, nano “jungle
gyms,” and “nanobridges”. Further, we present
an application of the 3D stacked nanofiber arrays by preparing transparent
and flexible polydimethylsiloxane films embedded with Ag-sputtered
nanowalls as 3D nanoelectrodes. The conductivity of the nanoelectrodes
can be precisely tuned by adjusting the number of 3D printed layers,
without sacrificing transmittance (98.5%). The current NFES approach
provides a simple, reliable route to build 3D stacked nanoarchitectures
with high-aspect ratios for potential application in smart materials,
energy devices, and biomedical applications
All-Cellulose Paper with High Optical Transmittance and Haze Fabricated via Electrophoretic Deposition
Reducing the thickness of transparent
paper without losing its
outstanding optical haze and transmittance remains a challenge due
to their trade-off relationship. Herein, an all-cellulose transparent
paper composed of cellulose nanofibril (CNF) and carboxymethyl cellulose
(CMC) is developed by electrophoretic deposition (EPD) thanks to the
good film-forming ability of the CMC. The thickness of the paper can
be controlled in the range of 2.4–30 μm depending on
the applied voltage and deposition time. The optical properties and
mechanical strength are adjusted by the sonication time and the ratio
between CNF and CMC, since the CNF works as a light-scattering source
and mechanical reinforcement agent. Consequently, a robust all-cellulose
paper with a thickness of 10 μm exhibiting high transmittance
(up to 96%) and haze (up to 89%) is successfully fabricated. As our
paper has competitive optical properties despite the thinner thickness
than other reported all-cellulose transparent and hazy paper, we achieved
the highest optical haze and transmittance values per unit thickness.
We believe that this all-cellulose paper with outstanding optical
properties has great potential to be applied to many fields that include
flexible devices, environmentally friendly electronics, optoelectronics,
and other functional devices
