Spatially resolved femtosecond pump-probe study of topological insulator Bi2Se3

Carrier and phonon dynamics in Bi2Se3 crystals are studied by a spatially resolved ultrafast pump-probe technique. Pronounced oscillations in differential reflection are observed with two distinct frequencies, and are attributed to coherent optical and acoustic phonons, respectively. The rising time of the signal indicates that the thermalization and energy relaxation of hot carriers are both sub-ps in this material. We found that the thermalization and relaxation time decreases with the carrier density. The expansion of the differential reflection profile allows us to estimate an ambipolar carrier diffusion coefficient on the order of 500 square centimeters per second. A long-term slow expansion of the profile shows a thermal diffusion coefficient of 1.2 square centimeters per second.Comment: 8 pages, 6 figure

Superconductivity and magnetism in platinum-substituted SrFe2As2 single crystals

Single crystals of SrFe2-xPtxAs2 (0 < x < 0.36) were grown using the self flux solution method and characterized using x-ray crystallography, electrical transport, magnetic susceptibility, and specific heat measurements. The magnetic/structural transition is suppressed with increasing Pt concentration, with superconductivity seen over the range 0.08 < x < 0.36 with a maximum transition temperature Tc of 16 K at x = 0.16. The shape of the phase diagram and the changes to the lattice parameters are similar to the effects of other group VIII elements Ni and Pd, however the higher transition temperature and extended range of superconductivity suggest some complexity beyond the simple electron counting picture that has been discussed thus far.Comment: 6 pages, 6 figure

On the resistivity at low temperatures in electron-doped cuprate superconductors

We measured the magnetoresistance as a function of temperature down to 20mK and magnetic field for a set of underdoped PrCeCuO (x=0.12) thin films with controlled oxygen content. This allows us to access the edge of the superconducting dome on the underdoped side. The sheet resistance increases with increasing oxygen content whereas the superconducting transition temperature is steadily decreasing down to zero. Upon applying various magnetic fields to suppress superconductivity we found that the sheet resistance increases when the temperature is lowered. It saturates at very low temperatures. These results, along with the magnetoresistance, cannot be described in the context of zero temperature two dimensional superconductor-to-insulator transition nor as a simple Kondo effect due to scattering off spins in the copper-oxide planes. We conjecture that due to the proximity to an antiferromagnetic phase magnetic droplets are induced. This results in negative magnetoresistance and in an upturn in the resistivity.Comment: Accepted in Phys. Rev.

The suppression of magnetism and the development of superconductivity within the collapsed tetragonal phase of Ca0.67Sr0.33Fe2As2 at high pressure

Structural and electronic characterization of (Ca0.67Sr0.33)Fe2As2 has been performed as a func- tion of pressure up to 12 GPa using conventional and designer diamond anvil cells. The compound (Ca0.67Sr0.33)Fe2As2 behaves intermediate between its end members-CaFe2As2 and SrFe2As2- displaying a suppression of magnetism and the onset of superconductivity. Like other members of the AEFe2As2 family, (Ca0.67Sr0.33)Fe2As2 undergoes a pressure-induced isostructural volume collapse, which we associate with the development of As-As bonding across the mirror plane of the structure. This collapsed tetragonal phase abruptly cuts off the magnetic state, giving rise to superconductivity with a maximum Tc=22.2 K. The maximum Tc of the superconducting phase is not strongly correlated with any structural parameter, but its proximity to the abrupt suppression of magnetism as well as the volume collapse transition suggests that magnetic interactions and structural inhomogeneity may play a role in its development. The pressure-dependent evolution of the ordered states and crystal structures in (Ca,Sr)Fe2As2 provides an avenue to understand the generic behavior of the other members of the AEFe2As2 family.Comment: 9 pages, 9 figure

Magnetothermoelectric properties of Bi2Se3

We present a study of entropy transport in Bi2Se3 at low temperatures and high magnetic fields. In the zero-temperature limit, the magnitude of the Seebeck coefficient quantitatively tracks the Fermi temperature of the 3D Fermi surface at \Gamma-point as the carrier concentration changes by two orders of magnitude (10$^{17}$ to 10$^{19}$cm$^{-3}$). In high magnetic fields, the Nernst response displays giant quantum oscillations indicating that this feature is not exclusive to compensated semi-metals. A comprehensive analysis of the Landau Level spectrum firmly establishes a large $g$-factor in this material and a substantial decrease of the Fermi energy with increasing magnetic field across the quantum limit. Thus, the presence of bulk carriers significantly affects the spectrum of the intensively debated surface states in Bi2Se3 and related materials.Comment: 10 pages, 9 figure

Towards spin injection from silicon into topological insulators: Schottky barrier between Si and Bi2Se3

A scheme is proposed to electrically measure the spin-momentum coupling in the topological insulator surface state by injection of spin polarized electrons from silicon. As a first approach, devices were fabricated consisting of thin (<100nm) exfoliated crystals of Bi2Se3 on n-type silicon with independent electrical contacts to silicon and Bi2Se3. Analysis of the temperature dependence of thermionic emission in reverse bias indicates a barrier height of 0.34 eV at the Si-Bi2Se3 interface. This robust Schottky barrier opens the possibility of novel device designs based on sub-band gap internal photoemission from Bi2Se3 into Si