Spin transport and magnetic proximity effect in CoFeB/normal metal/Pt trilayers

We present a study of the damping and spin pumping properties of CoFeB/X/Pt systems with X=Al,Cr, and Ta. We show that the total damping of the CoFeB/Pt systems is strongly reduced when an interlayer is introduced independently of the material. Using a model that considers spin relaxation, we identify the origin of this contribution in the magnetically polarized Pt formed by the magnetic proximity effect (MPE), which is suppressed by the introduction of the interlayer. The induced ferromagnetic order in the Pt layer is confirmed by element-sensitive transverse magneto-optical Kerr spectroscopy at the M2,3 and N7 absorption edges. We discuss the impact of the MPE on parameter extraction in the spin transport model.Peer reviewe

Induced versus intrinsic magnetic moments in ultrafast magnetization dynamics

Ferromagnetic metal alloys are today commonly used in spintronic and magnetic data storage devices. These multicompound structures consist of several magnetic sublattices exhibiting both intrinsic and induced magnetic moments. Here, we study the response of the element-specific magnetization dynamics for thin film systems based on purely intrinsic (CoFeB) and partially induced (FePt) magnetic moments using extreme ultraviolet pulses from high-harmonic generation (HHG) as an element-sensitive probe. In FePt, on the one hand, we observe an identical normalized transient magnetization for Fe and Pt throughout both the ultrafast demagnetization and the subsequent remagnetization. On the other hand, Co and Fe show a clear difference in the asymptotic limit of the remagnetization process in CoFeB, which is supported by calculations for the temperature-dependent behavior of the equilibrium magnetization using a dynamic spin model. Thus, in this work, we provide a vital step toward a comprehensive understanding of ultrafast light-induced magnetization dynamics in ferromagnetic alloys with sublattices of intrinsic and induced magnetic moments.publishe

Efficiency of ultrafast optically induced spin transfer in Hensler compounds

Steil D, Walowski J, Gerhard F, et al. Efficiency of ultrafast optically induced spin transfer in Hensler compounds. Physical Review Research. 2020;2(2): 023199.Optically induced spin transfer (OISTR) is a pathway to control magnetization dynamics in complex materials on femto- to attosecond timescales. The direct interaction of the laser field with the material creates transient nonequilibrium states, which can exhibit an efficient spin transfer between different magnetic subsystems. How far this spin manipulation via OISTR is a general phenomenon or restricted to a subset of materials with specific properties is an open experimental and theoretical question. Using time-resolved magneto-optical Kerr measurements and time-dependent density functional theory we investigate OISTR in Heusler compounds. We show that the half-Heusler materials NiMnSb and CoMnSb exhibit strong signatures of OISTR, whereas this is less pronounced in the full-Heusler compounds Co-2 MnSi, Co2FeSi, and Co2FeAl in agreement with ab initio calculations. Our work opens up a systematic path for coherent manipulation of spin dynamics by direct light-matter interaction

Direct light-induced spin transfer between different elements in a spintronic Heusler material via femtosecond laser excitation

Heusler compounds are exciting materials for future spintronics applications because they display a wide range of tunable electronic and magnetic interactions. Here, we use a femtosecond laser to directly transfer spin polarization from one element to another in a half-metallic Heusler material, Co2MnGe. This spin transfer initiates as soon as light is incident on the material, demonstrating spatial transfer of angular momentum between neighboring atomic sites on time scales < 10 fs. Using ultrafast high harmonic pulses to simultaneously and independently probe the magnetic state of two elements during laser excitation, we find that the magnetization of Co is enhanced, while that of Mn rapidly quenches. Density functional theory calculations show that the optical excitation directly transfers spin from one magnetic sublattice to another through preferred spin-polarized excitation pathways. This direct manipulation of spins via light provides a path toward spintronic devices that can operate on few-femtosecond or faster time scales