Coherent oscillations in a superconducting multi-level quantum system

We have observed coherent time evolution of states in a multi-level quantum system, formed by a current-biased dc SQUID. The manipulation of the quantum states is achieved by resonant microwave pulses of flux. The number of quantum states participating in the coherent oscillations increases with increasing microwave power. Quantum measurement is performed by a nanosecond flux pulse which projects the final state onto one of two different voltage states of the dc SQUID, which can be read out

One-Shot Quantum Measurement Using a Hysteretic dc SQUID

We propose a single shot quantum measurement to determine the state of a Josephson charge quantum bit (qubit). The qubit is a Cooper pair box and the measuring device is a two junction superconducting quantum interference device (dc SQUID). This coupled system exhibits a close analogy with a Rydberg atom in a high Q cavity, except that in the present device we benefit from the additional feature of escape from the supercurrent state by macroscopic quantum tunneling, which provides the final readout. We test the feasibility of our idea against realistic experimental circuit parameters and by analyzing the phase fluctuations of the qubit.Peer reviewe

Addressing single molecular spin with graphene based nano-architectures.

Finding reliable methods to exploit molecular degrees of freedom represents an intriguing problem involving the control of new mechanisms at the nano-scale and several technological challenges. Here we report a novel approach to address single molecular spin embedded in an electronic circuit. Our devices make use of molecules with well-defined magnetic anisotropy (TbPc2) embedded in nano-gapped electrodes obtained by electro-burning graphene layers. Such devices work as molecular spin transistors allowing the detection of the Tb spin flip during the sweep of an external magnetic field. The spin read out is made by the molecular quantum dot that, in turns, is driven by an auxiliary gate voltage. In the general context of (spin-)electronics, these results demonstrate that: 1) molecular quantum dots can be used as ultra-sensitive detectors for spin flip detection and 2) the use of graphene electrodes as platform to contact organo-metallic molecule is a viable route to design more complex nano-architectures

Using a quantum dot as a high-frequency shot noise detector

We present the experimental realization of a Quantum Dot (QD) operating as a high-frequency noise detector. Current fluctuations produced in a nearby Quantum Point Contact (QPC) ionize the QD and induce transport through excited states. The resulting transient current through the QD represents our detector signal. We investigate its dependence on the QPC transmission and voltage bias. We observe and explain a quantum threshold feature and a saturation in the detector signal. This experimental and theoretical study is relevant in understanding the backaction of a QPC used as a charge detector.Comment: 4 pages, 4 figures, accepted for publication in Physical Review Letter

Evidence of two-dimensional macroscopic quantum tunneling of a current-biased DC-SQUID

The escape probability out of the superconducting state of a hysteretic DC-SQUID has been measured at different values of the applied magnetic flux. At low temperature, the escape current and the width of the probability distribution are temperature independent but they depend on flux. Experimental results do not fit the usual one-dimensional (1D) Macroscopic Quantum Tunneling (MQT) law but are perfectly accounted for by the two-dimensional (2D) MQT behaviour as we propose here. Near zero flux, our data confirms the recent MQT observation in a DC-SQUID \cite{Li02}.Comment: 4 pages, 4 figures Accepted to PR

Landau-Zener Transition in a Continuously Measured Single-Molecule Spin Transistor

We monitor the Landau-Zener dynamics of a single-ion magnet inserted into a spin-transistor geometry. For increasing field-sweep rates, the spin reversal probability shows increasing deviations from that of a closed system. In the low-conductance limit, such deviations are shown to result from a dephasing process. In particular, the observed behaviors are successfully simulated by means of an adiabatic master equation, with time averaged dephasing (Lindblad) operators. The time average is tentatively interpreted in terms of the finite time resolution of the continuous measurement

Single-molecule devices with graphene electrodes

Several technological issues have to be faced to realize devices working at the single molecule level. One of the main challenges consists of defining methods to fabricate electrodes to make contact with single molecules. Here, we report the realization of novel spintronic devices made of a TbPc2 single molecule embedded between two nanometer-separated graphene electrodes, obtained by feedback-controlled electroburning. We demonstrate that this approach allows the realisation of devices working at low temperature. With these, we were able to characterize the magnetic exchange coupling between the electronic spin of the Tb3+ magnetic core and the current passing through the molecular system in the Coulomb blockade regime, thus showing that the use of graphene is a promising way forward in addressing single molecules