Destabilization of a flow focused suspension of magnetotactic bacteria

Active matter is a new class of material, intrinsically out-of equilibrium with intriguing properties. So far, the recent upsurge of studies has mostly focused on the spontaneous behavior of these systems --in the absence of external constraints or driving--. Yet, many real life systems evolve under constraints, being both submitted to flow and various taxis. In the present work, we demonstrate a new experimental system which opens up the way for quantitative investigations, and discriminating examinations, of the challenging theoretical description of such systems. We explore the behavior of magnetotactic bacteria as a particularly rich and versatile class of driven matter, which behavior can be studied under contrasting and contradicting stimuli. In particular we demonstrate that the competing driving of an orienting magnetic field and hydrodynamic flow lead not only to jetting, but also unveils a new pearling instability. This illustrates new structuring capabilities of driven active matter

Sedimentation of self-propelled Janus colloids: polarization and pressure

We study experimentally-using Janus colloids-and theoretically-using Active Brownian Particles- the sedimentation of dilute active colloids. We first confirm the existence of an exponential density profile. We show experimentally the emergence of a polarized steady state outside the effective equilibrium regime, i.e. when v_s is not much smaller than the propulsion speed. The experimental distribution of polarization is very well described by the theoretical prediction with no fitting parameter. We then discuss and compare three different definitions of pressure for sedimenting particles: the weight of particles above a given height, the flux of momentum and active impulse, and the force density measured by pressure gauges

Diffusiophoresis at the macroscale

Diffusiophoresis, a ubiquitous phenomenon that induces particle transport whenever solute concentration gradients are present, was recently observed in the context of microsystems and shown to strongly impact colloidal transport (patterning and mixing) at such scales. In the present work, we show experimentally that this nanoscale mechanism can induce changes in the macroscale mixing of colloids by chaotic advection. Rather than the decay of the standard deviation of concentration, which is a global parameter commonly employed in studies of mixing, we instead use multiscale tools adapted from studies of chaotic flows or intermittent turbulent mixing: concentration spectra and second and fourth moments of the probability density functions of scalar gradients. Not only can these tools be used in open flows, but they also allow for scale-by-scale analysis. Strikingly, diffusiophoresis is shown to affect all scales, although more particularly the small ones, resulting in a change of scalar intermittency and in an unusual scale bridging spanning more than seven orders of magnitude. By quantifying the averaged impact of diffusiophoresis on the macroscale mixing, we explain why the effects observed are consistent with the introduction of an effective P\'eclet number.Comment: 13 page

Continuous Manipulation and Characterization of Colloidal Beads and Liposomes via Diffusiophoresis in Single- and Double-Junction Microchannels

International audienc

Dataset for "Enhanced Accumulation of Colloidal Particles in Microgrooved Channels via Diffusiophoresis and Steady-State Electrolyte Flows"

Experimental particle concentration fields used to generate the results shown in Fig. 2, Fig. 3 and Fig. 4 of "Enhanced Accumulation of Colloidal Particles in Microgrooved Channels via Diffusiophoresis and Steady-State Electrolyte Flows" by N. Singh, G. Vladisavljevic, F. Nadal, C. Cottin-Bizonne, C. Pirat, G. Bolognesi Capitalized keywords are from Loterre's Chemistry Vocabulary.</p

Reversible trapping of colloids in microgrooved channels by diffusiophoresis

Symposium abstract