Large magnetic field-induced spectral weight enhancement of high-energy spin excitations in La1.88Sr0.12CuO4La_{1.88}Sr_{0.12}CuO_{4}

We report electronic Raman scattering experiments on a superconducting ${\rm La_{1.88}Sr_{0.12}CuO_{4}}$ single crystal in a magnetic field. At low temperatures, the spectral weight of the high-energy two-magnon peak increases linearly with field and is amplified by a factor of more than two at 14 T. The effect disappears at elevated temperatures and is not present in undoped ${\rm La_{2}CuO_{4}}$. This observation is discussed in terms of an electronically inhomogeneous state in which the field enhances the volume fraction of a phase with local antiferromagnetic order at the expense of the superconducting phase.Comment: to appear in PR

Spin-Wave Lifetimes Throughout the Brillouin Zone

We use a neutron spin-echo method with $\mu$eV resolution to determine the lifetimes of spin waves in the prototypical antiferromagnet MnF$_2$ over the entire Brillouin zone. A theory based on the interaction of magnons with longitudinal spin fluctuations provides an excellent, parameter-free description of the data, except at the lowest momenta and temperatures. This is surprising, given the prominence of alternative theories based on magnon-magnon interactions in the literature. The results and technique open up a new avenue for the investigation of fundamental concepts in magnetism. The technique also allows measurement of the lifetimes of other elementary excitations (such as lattice vibrations) throughout the Brillouin zone.Comment: 12 pages, 4 figure

Magnetic structure of the edge-sharing copper oxide chain compound NaCu2O2

Single-crystal neutron diffraction has been used to determine the incommensurate magnetic structure of NaCu2O2, a compound built up of chains of edge-sharing CuO4 plaquettes. Magnetic structures compatible with the lattice symmetry were identified by a group-theoretical analysis, and their magnetic structure factors were compared to the experimentally observed Bragg intensities. In conjunction with other experimental data, this analysis yields an elliptical helix structure in which both the helicity and the polarization plane alternate among copper-oxide chains. This magnetic ground state is discussed in the context of the recently reported multiferroic properties of other copper-oxide chain compounds

Neutron spin-echo study of the critical dynamics of spin-5/2 antiferromagnets in two and three dimensions

We report a neutron spin-echo study of the critical dynamics in the $S=5/2$ antiferromagnets MnF$_2$ and Rb$_2$MnF$_4$ with three-dimensional (3D) and two-dimensional (2D) spin systems, respectively, in zero external field. Both compounds are Heisenberg antiferromagnets with a small uniaxial anisotropy resulting from dipolar spin-spin interactions, which leads to a crossover in the critical dynamics close to the N\'eel temperature, $T_N$. By taking advantage of the $\mu\text{eV}$ energy resolution of the spin-echo spectrometer, we have determined the dynamical critical exponents $z$ for both longitudinal and transverse fluctuations. In MnF$_2$, both the characteristic temperature for crossover from 3D Heisenberg to 3D Ising behavior and the exponents $z$ in both regimes are consistent with predictions from the dynamical scaling theory. The amplitude ratio of longitudinal and transverse fluctuations also agrees with predictions. In Rb$_2$MnF$_4$, the critical dynamics crosses over from the expected 2D Heisenberg behavior for $T\gg T_N$ to a scaling regime with exponent $z = 1.387(4)$, which has not been predicted by theory and may indicate the influence of long-range dipolar interactions