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Electrochemical kinetics and dimensional considerations, at the nanoscale

By H. Yamada and P. R. Bandaru

Abstract

It is shown that the consideration of the density of states variation in nanoscale electrochemical systems yields modulations in the rate constant and concomitant electrical currents. The proposed models extend the utility of Marcus-Hush-Chidsey (MHC) kinetics to a larger class of materials and could be used as a test of dimensional character. The implications of the study are of much significance to an understanding and modulation of charge transfer nanostructured electrodes

Topics: Physics, QC1-999
Publisher: AIP Publishing LLC
Year: 2016
DOI identifier: 10.1063/1.4955049
OAI identifier: oai:doaj.org/article:d91d81cf9df54f7abb002ff639727614
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