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Construction of Adjacent Quaternary and Tertiary Stereocenters via an Organocatalytic Allylic Alkylation of Morita-Baylis-Hillman Carbonates

By D.J.V.C. van Steenis, T. Marcelli, M. Lutz, A.L. Spek, J.H. van Maarseveen and H. Hiemstra


Racemic Baylis-Hillman carbonates can be converted in densely functionalized products by reaction with cyano esters in the presence of a catalytic amount of a modified Cinchona alkaloid in high enantioselectivities and fair diastereoselectivities. A rational for the observed stereoselectivity is presente

Year: 2007
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