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Nanoscale mechanical control of surface electrical properties of manganite films with magnetic nanoparticles

By Borislav Vasic, Zorica Konstantinovic, Elisa Victoria Pannunzio Miner, Sergio Valencia, Radu Abrudan, Rados Gajic and Alberto Pomar


Mechanical control of electrical properties in complex heterostructures, consisting of magnetic FeOx nanoparticles on top of manganite films, is achieved using atomic force microscope (AFM) based methods. Under applied pressure of the AFM tip, drop of the electrical conductivity is observed inducing an electrically insulating state upon a critical normal load. Current and surface potential maps suggest that the switching process is mainly governed by the flexoelectric field induced at the sample surface. The relaxation process of the electrical surface potential indicates that the diffusion of oxygen vacancies from the bulk of the manganite films towards the sample surface is the dominant relaxation mechanism. The magnetic FeOx nanoparticles, staying attached to the sample surface after the rubbing, protect the underlying manganite films and provide stability of the observed resistive switching effect. The employed mechanical control gives a new freedom in the design of resistive switching devices since it does not depend on the film thickness, and biasing is not needed.Fil: Vasic, Borislav. University Of Belgrade; SerbiaFil: Konstantinovic, Zorica. University Of Belgrade; SerbiaFil: Pannunzio Miner, Elisa Victoria. Consejo Superior de Investigaciones Científicas. Instituto de Ciencia de los Materiales de Barcelona; España. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Centro de Investigaciones en Ciencias de la Tierra. Universidad Nacional de Córdoba. Facultad de Ciencias Exactas Físicas y Naturales. Centro de Investigaciones en Ciencias de la Tierra; ArgentinaFil: Valencia, Sergio. Helmholtz-zentrum Berlin Für Materialien Und Energie (hzb); Berlin; AlemaniaFil: Abrudan, Radu. Ruhr Universität Bochum; AlemaniaFil: Gajic, Rados. University Of Belgrade; SerbiaFil: Pomar, Alberto. Consejo Superior de Investigaciones Científicas. Instituto de Ciencia de los Materiales de Barcelona; Españ

Topics: Thin-films, Oxygen vacancies, SrTiO3, Oxides, Otras Ciencias Químicas, Ciencias Químicas, CIENCIAS NATURALES Y EXACTAS
Publisher: 'Royal Society of Chemistry (RSC)'
Year: 2019
DOI identifier: 10.1039/c8na00301g
OAI identifier:
Provided by: CONICET Digital
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